Simulation on Vapor Liquid Equilibria of R1234yf/R290/R134a Ternary System

Based on the Peng Robinson (PR) equation of state combined with the Wong-Sandler (WS) mixing rule, and combined with the UNIFAC group contribution method used in the Predictive Soave Redlich Kwong (PSRK) equation, a gas-liquid equilibrium prediction model of the mixture (PRWS-UNIFAC-PSRK) was constr...

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Bibliographic Details
Main Authors: Qin Yanbin, Zhang Hua, Wu Yinlong
Format: Article
Language:zho
Published: Journal of Refrigeration Magazines Agency Co., Ltd. 2017-01-01
Series:Zhileng xuebao
Subjects:
Online Access:http://www.zhilengxuebao.com/thesisDetails#10.3969/j.issn.0253-4339.2017.05.029
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Summary:Based on the Peng Robinson (PR) equation of state combined with the Wong-Sandler (WS) mixing rule, and combined with the UNIFAC group contribution method used in the Predictive Soave Redlich Kwong (PSRK) equation, a gas-liquid equilibrium prediction model of the mixture (PRWS-UNIFAC-PSRK) was constructed. The results indicate that for the R32/R1234yf binary mixture, the deviations between the experimental and calculated data for the pressure and vapor phase mass fraction are within ±2.5% and 0.02, respectively. For R134a/R1234yf/R600a ternary mixture, the relative deviation between the measured pressures and calculated results are within ±3% and the absolute deviation of vapor phase mass fraction is within ±0.04. In ternary phase equilibria diagram of R1234yf/R290/R134a, the mass fraction of R1234yf/R290/R134a at around 0.25/0.7/0.05 has an azeotropic point. The VLE (vapor liquid equilibria) prediction model can be further improved by using the multi-parameter equation of states, improving the activity coefficient models and obtaining more accurate binary interaction coefficient.
ISSN:0253-4339