Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts

Abstract Around 80% of the world’s hard-rock lithium supply comes from pegmatites formed in the Archean Eon, yet our understanding of how Lithium-pegmatites form assumes magma source compositions not relevant to those Archean cratons hosting most of the giant Lithium-pegmatites. These models emphasi...

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Main Authors: Robert H. Smithies, Yongjun Lu, David C. Champion, Marcus T. Sweetapple, Jack R. Lowrey, Nathan H. Bowman, Kevin F. Cassidy, Tim J. Ivanic, Anthony I. S. Kemp, Rose E. Turnbull, Klaus Gessner, Fawna J. Korhonen
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Communications Earth & Environment
Online Access:https://doi.org/10.1038/s43247-025-02622-5
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author Robert H. Smithies
Yongjun Lu
David C. Champion
Marcus T. Sweetapple
Jack R. Lowrey
Nathan H. Bowman
Kevin F. Cassidy
Tim J. Ivanic
Anthony I. S. Kemp
Rose E. Turnbull
Klaus Gessner
Fawna J. Korhonen
author_facet Robert H. Smithies
Yongjun Lu
David C. Champion
Marcus T. Sweetapple
Jack R. Lowrey
Nathan H. Bowman
Kevin F. Cassidy
Tim J. Ivanic
Anthony I. S. Kemp
Rose E. Turnbull
Klaus Gessner
Fawna J. Korhonen
author_sort Robert H. Smithies
collection DOAJ
description Abstract Around 80% of the world’s hard-rock lithium supply comes from pegmatites formed in the Archean Eon, yet our understanding of how Lithium-pegmatites form assumes magma source compositions not relevant to those Archean cratons hosting most of the giant Lithium-pegmatites. These models emphasize extraction of residual pegmatitic liquids from granitic magmas formed through melting sedimentary sequences. However, there is no evidence that such sequences provided the source to Lithium-rich granites and related giant Lithium-pegmatites in the Archean cratons of Western Australia. Economically important Lithium-pegmatites in these terrains form near faulted contacts between regional granites and basalt-dominated greenstone belts. Where spatially associated granites are Lithium-rich, they also contain unusually radiogenic Neodymium, resembling earlier, but spatially associated hydrated high-Magnesium diorites of mantle origin (sanukitoid). Intrusion of sanukitoids along crustal-scale structures prior to granitic magmatism induced Lithium-rich biotite alteration of the felsic basement beneath greenstone belts. Analogous to melting metasomatized lithospheric mantle to produce sanukitoids, melting of sanukitoid-infused basement beneath greenstone roots produced Lithium-rich granites and ultimately Lithium-pegmatite. Melting buried metasediments might produce Lithium-pegmatites, but most of the world’s giant Lithium-pegmatites formed along major crustal boundaries in response to the transfer of hydrous mantle-derived magma from metasomatized deep lithospheric domains in the Archean.
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spelling doaj-art-8c3e8e62740f40d3b4e9137b71d3ab872025-08-20T03:43:30ZengNature PortfolioCommunications Earth & Environment2662-44352025-08-016111110.1038/s43247-025-02622-5Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone beltsRobert H. Smithies0Yongjun Lu1David C. Champion2Marcus T. Sweetapple3Jack R. Lowrey4Nathan H. Bowman5Kevin F. Cassidy6Tim J. Ivanic7Anthony I. S. Kemp8Rose E. Turnbull9Klaus Gessner10Fawna J. Korhonen11Geological Survey of Western AustraliaGeological Survey of Western AustraliaGeological Survey of Western AustraliaCentre for Exploration Targeting and School of Earth and Oceans, University of Western AustraliaGeological Survey of Western AustraliaGeological Survey of Western AustraliaCentre for Exploration Targeting and School of Earth and Oceans, University of Western AustraliaGeological Survey of Western AustraliaARC Centre for Critical Resources of the Future, School of Earth and Oceans, University of Western AustraliaGeological Survey of Western AustraliaGeological Survey of Western AustraliaGeological Survey of Western AustraliaAbstract Around 80% of the world’s hard-rock lithium supply comes from pegmatites formed in the Archean Eon, yet our understanding of how Lithium-pegmatites form assumes magma source compositions not relevant to those Archean cratons hosting most of the giant Lithium-pegmatites. These models emphasize extraction of residual pegmatitic liquids from granitic magmas formed through melting sedimentary sequences. However, there is no evidence that such sequences provided the source to Lithium-rich granites and related giant Lithium-pegmatites in the Archean cratons of Western Australia. Economically important Lithium-pegmatites in these terrains form near faulted contacts between regional granites and basalt-dominated greenstone belts. Where spatially associated granites are Lithium-rich, they also contain unusually radiogenic Neodymium, resembling earlier, but spatially associated hydrated high-Magnesium diorites of mantle origin (sanukitoid). Intrusion of sanukitoids along crustal-scale structures prior to granitic magmatism induced Lithium-rich biotite alteration of the felsic basement beneath greenstone belts. Analogous to melting metasomatized lithospheric mantle to produce sanukitoids, melting of sanukitoid-infused basement beneath greenstone roots produced Lithium-rich granites and ultimately Lithium-pegmatite. Melting buried metasediments might produce Lithium-pegmatites, but most of the world’s giant Lithium-pegmatites formed along major crustal boundaries in response to the transfer of hydrous mantle-derived magma from metasomatized deep lithospheric domains in the Archean.https://doi.org/10.1038/s43247-025-02622-5
spellingShingle Robert H. Smithies
Yongjun Lu
David C. Champion
Marcus T. Sweetapple
Jack R. Lowrey
Nathan H. Bowman
Kevin F. Cassidy
Tim J. Ivanic
Anthony I. S. Kemp
Rose E. Turnbull
Klaus Gessner
Fawna J. Korhonen
Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
Communications Earth & Environment
title Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
title_full Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
title_fullStr Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
title_full_unstemmed Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
title_short Giant lithium-rich pegmatites in Archean cratons form by remelting refertilised roots of greenstone belts
title_sort giant lithium rich pegmatites in archean cratons form by remelting refertilised roots of greenstone belts
url https://doi.org/10.1038/s43247-025-02622-5
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