Exposing hidden periodic orbits in scanning force microscopy

Abstract The nonlinear interaction between the tip of a scanning probe microscope (SPM) and a sample is manifested in the emergence of bifurcations and unstable branches in the frequency response of a driven cantilever. While extensively investigated theoretically, exploring the unstable branch in a...

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Main Authors: Lukas Böttcher, Hannes Wallner, Niklas Kruse, Wolfram Just, Ingo Barke, Jens Starke, Sylvia Speller
Format: Article
Language:English
Published: Nature Portfolio 2025-02-01
Series:Communications Physics
Online Access:https://doi.org/10.1038/s42005-025-01958-w
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author Lukas Böttcher
Hannes Wallner
Niklas Kruse
Wolfram Just
Ingo Barke
Jens Starke
Sylvia Speller
author_facet Lukas Böttcher
Hannes Wallner
Niklas Kruse
Wolfram Just
Ingo Barke
Jens Starke
Sylvia Speller
author_sort Lukas Böttcher
collection DOAJ
description Abstract The nonlinear interaction between the tip of a scanning probe microscope (SPM) and a sample is manifested in the emergence of bifurcations and unstable branches in the frequency response of a driven cantilever. While extensively investigated theoretically, exploring the unstable branch in an actual SPM experiment is lacking so far, reflecting the broader challenge in studying mechanical nanojunction oscillators under strongly varying external forces. Here we demonstrate experimental tracking of unstable periodic orbits between two saddle-node bifurcation points in the attractive regime, revealing the full set of stationary oscillatory states. This is achieved by a minimally invasive control scheme based on fast adaptive phase extraction and Fourier discretisation of the tip dynamics. Stabilization of unstable branches of oscillating AFM cantilevers opens avenues for novel experimental modes, potentially enabling ultrasensitive surface detection at considerably large amplitudes with minimal tip-surface interaction, new insights in tip-surface interaction mechanisms, as well as new AFM modes enabling arbitrary setpoint choice while inherently avoiding discontinuities.
format Article
id doaj-art-8bad2c71432b40d6881188c954eef00e
institution Kabale University
issn 2399-3650
language English
publishDate 2025-02-01
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series Communications Physics
spelling doaj-art-8bad2c71432b40d6881188c954eef00e2025-02-09T12:40:41ZengNature PortfolioCommunications Physics2399-36502025-02-01811910.1038/s42005-025-01958-wExposing hidden periodic orbits in scanning force microscopyLukas Böttcher0Hannes Wallner1Niklas Kruse2Wolfram Just3Ingo Barke4Jens Starke5Sylvia Speller6Institute of Physics, University of RostockInstitute of Mathematics, University of RostockInstitute of Mathematics, University of RostockInstitute of Mathematics, University of RostockInstitute of Physics, University of RostockInstitute of Mathematics, University of RostockInstitute of Physics, University of RostockAbstract The nonlinear interaction between the tip of a scanning probe microscope (SPM) and a sample is manifested in the emergence of bifurcations and unstable branches in the frequency response of a driven cantilever. While extensively investigated theoretically, exploring the unstable branch in an actual SPM experiment is lacking so far, reflecting the broader challenge in studying mechanical nanojunction oscillators under strongly varying external forces. Here we demonstrate experimental tracking of unstable periodic orbits between two saddle-node bifurcation points in the attractive regime, revealing the full set of stationary oscillatory states. This is achieved by a minimally invasive control scheme based on fast adaptive phase extraction and Fourier discretisation of the tip dynamics. Stabilization of unstable branches of oscillating AFM cantilevers opens avenues for novel experimental modes, potentially enabling ultrasensitive surface detection at considerably large amplitudes with minimal tip-surface interaction, new insights in tip-surface interaction mechanisms, as well as new AFM modes enabling arbitrary setpoint choice while inherently avoiding discontinuities.https://doi.org/10.1038/s42005-025-01958-w
spellingShingle Lukas Böttcher
Hannes Wallner
Niklas Kruse
Wolfram Just
Ingo Barke
Jens Starke
Sylvia Speller
Exposing hidden periodic orbits in scanning force microscopy
Communications Physics
title Exposing hidden periodic orbits in scanning force microscopy
title_full Exposing hidden periodic orbits in scanning force microscopy
title_fullStr Exposing hidden periodic orbits in scanning force microscopy
title_full_unstemmed Exposing hidden periodic orbits in scanning force microscopy
title_short Exposing hidden periodic orbits in scanning force microscopy
title_sort exposing hidden periodic orbits in scanning force microscopy
url https://doi.org/10.1038/s42005-025-01958-w
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