Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling

Abstract Altermagnets, a recently identified class of collinear magnets, exhibit unique properties such as zero net magnetization and spin polarization dictated by lattice symmetry, making them a subject of intense research. In contrast to conventional strategies for inducing altermagnetism in antif...

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Main Authors: Wei Sun, Wenxuan Wang, Changhong Yang, Shifeng Huang, Ning Ding, Shuai Dong, Zhenxiang Cheng
Format: Article
Language:English
Published: Wiley 2025-08-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202503235
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author Wei Sun
Wenxuan Wang
Changhong Yang
Shifeng Huang
Ning Ding
Shuai Dong
Zhenxiang Cheng
author_facet Wei Sun
Wenxuan Wang
Changhong Yang
Shifeng Huang
Ning Ding
Shuai Dong
Zhenxiang Cheng
author_sort Wei Sun
collection DOAJ
description Abstract Altermagnets, a recently identified class of collinear magnets, exhibit unique properties such as zero net magnetization and spin polarization dictated by lattice symmetry, making them a subject of intense research. In contrast to conventional strategies for inducing altermagnetism in antiferromagnets that rely on manipulating real‐space symmetry, this work introduces a novel and general approach to achieving altermagnetism by modulating spin‐space symmetry. Through a combination of tight‐binding models and first‐principles calculations, the microscopic origin of altermagnetism driven by spin‐space symmetry is uncovered, and the mechanism underlying enhanced spin splitting is identified. Furthermore, it is demonstrated that this spin‐space modulation can synergistically interact with ferroelectricity, enabling a spin symmetry‐dependent magnetoelectric coupling mechanism that is distinct from conventional multiferroics. This unique coupling is validated by the magneto‐optical Kerr effect, providing a robust theoretical foundation for the development of next‐generation spintronic devices that harness the potential of altermagnetism.
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institution Kabale University
issn 2198-3844
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publishDate 2025-08-01
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series Advanced Science
spelling doaj-art-8b7a7aeeaa05466b8da5dca34bdb88172025-08-20T11:56:10ZengWileyAdvanced Science2198-38442025-08-011230n/an/a10.1002/advs.202503235Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric CouplingWei Sun0Wenxuan Wang1Changhong Yang2Shifeng Huang3Ning Ding4Shuai Dong5Zhenxiang Cheng6Shandong Provincial Key Laboratory of Green and Intelligent Building Materials University of Jinan Jinan 250022 ChinaSchool of Material Science and Engineering University of Jinan Jinan Shandong 250022 ChinaShandong Provincial Key Laboratory of Green and Intelligent Building Materials University of Jinan Jinan 250022 ChinaShandong Provincial Key Laboratory of Green and Intelligent Building Materials University of Jinan Jinan 250022 ChinaKey Laboratory of Quantum Materials and Devices of Ministry of Education School of Physics Southeast University Nanjing 211189 ChinaKey Laboratory of Quantum Materials and Devices of Ministry of Education School of Physics Southeast University Nanjing 211189 ChinaInstitute for Superconducting & Electronic Materials Australian Institute of Innovative Materials University of Wollongong Innovation Campus, Squires Way North Wollongong New South Wales 2500 AustraliaAbstract Altermagnets, a recently identified class of collinear magnets, exhibit unique properties such as zero net magnetization and spin polarization dictated by lattice symmetry, making them a subject of intense research. In contrast to conventional strategies for inducing altermagnetism in antiferromagnets that rely on manipulating real‐space symmetry, this work introduces a novel and general approach to achieving altermagnetism by modulating spin‐space symmetry. Through a combination of tight‐binding models and first‐principles calculations, the microscopic origin of altermagnetism driven by spin‐space symmetry is uncovered, and the mechanism underlying enhanced spin splitting is identified. Furthermore, it is demonstrated that this spin‐space modulation can synergistically interact with ferroelectricity, enabling a spin symmetry‐dependent magnetoelectric coupling mechanism that is distinct from conventional multiferroics. This unique coupling is validated by the magneto‐optical Kerr effect, providing a robust theoretical foundation for the development of next‐generation spintronic devices that harness the potential of altermagnetism.https://doi.org/10.1002/advs.202503235altermagnetismmagnetoelectric couplingmultiferroicssliding ferroelectricity
spellingShingle Wei Sun
Wenxuan Wang
Changhong Yang
Shifeng Huang
Ning Ding
Shuai Dong
Zhenxiang Cheng
Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
Advanced Science
altermagnetism
magnetoelectric coupling
multiferroics
sliding ferroelectricity
title Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
title_full Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
title_fullStr Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
title_full_unstemmed Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
title_short Designing Spin Symmetry for Altermagnetism with Strong Magnetoelectric Coupling
title_sort designing spin symmetry for altermagnetism with strong magnetoelectric coupling
topic altermagnetism
magnetoelectric coupling
multiferroics
sliding ferroelectricity
url https://doi.org/10.1002/advs.202503235
work_keys_str_mv AT weisun designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT wenxuanwang designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT changhongyang designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT shifenghuang designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT ningding designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT shuaidong designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling
AT zhenxiangcheng designingspinsymmetryforaltermagnetismwithstrongmagnetoelectriccoupling