Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications

Thin Nb2O5 films with tunable porosity are deposited by the sol-gel and evaporation induced self-assembly methods using organic template Pluronic PE6100 with different molar fractions with respect to NbCl5 used as a precursor for synthesis of Nb sol. Surface morphology and structure of the films are...

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Main Authors: Rosen Georgiev, Biliana Georgieva, Marina Vasileva, Petar Ivanov, Tsvetanka Babeva
Format: Article
Language:English
Published: Wiley 2015-01-01
Series:Advances in Condensed Matter Physics
Online Access:http://dx.doi.org/10.1155/2015/403196
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author Rosen Georgiev
Biliana Georgieva
Marina Vasileva
Petar Ivanov
Tsvetanka Babeva
author_facet Rosen Georgiev
Biliana Georgieva
Marina Vasileva
Petar Ivanov
Tsvetanka Babeva
author_sort Rosen Georgiev
collection DOAJ
description Thin Nb2O5 films with tunable porosity are deposited by the sol-gel and evaporation induced self-assembly methods using organic template Pluronic PE6100 with different molar fractions with respect to NbCl5 used as a precursor for synthesis of Nb sol. Surface morphology and structure of the films are studied by Transmission Electron Microscopy and Selected Area Electron Diffraction. The optical characterization of the films is carried out through reflectance spectra measurements of the films deposited on silicon substrates and theoretical modeling in order to obtain refractive index, extinction coefficient, and thickness of the films. The overall porosity of the films and the amount of adsorbed acetone vapors in the pores are quantified by means of Bruggeman effective medium approximation using already determined optical constants. The sensing properties of the samples are studied by measuring both the reflectance spectra and room-temperature photoluminescence spectra prior to and after exposure to acetone vapors and liquid, respectively. The potential of using the studied mesoporous Nb2O5 films for chemooptical sensing is demonstrated and discussed.
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spelling doaj-art-8b6ee43ebece4e8399ae6dc2c0334d872025-08-20T02:09:25ZengWileyAdvances in Condensed Matter Physics1687-81081687-81242015-01-01201510.1155/2015/403196403196Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing ApplicationsRosen Georgiev0Biliana Georgieva1Marina Vasileva2Petar Ivanov3Tsvetanka Babeva4Institute of Optical Materials and Technologies “Acad. J. Malinowski”, Bulgarian Academy of Sciences, Acad. G. Bonchev Street, Block 109, 1113 Sofia, BulgariaInstitute of Optical Materials and Technologies “Acad. J. Malinowski”, Bulgarian Academy of Sciences, Acad. G. Bonchev Street, Block 109, 1113 Sofia, BulgariaInstitute of Optical Materials and Technologies “Acad. J. Malinowski”, Bulgarian Academy of Sciences, Acad. G. Bonchev Street, Block 109, 1113 Sofia, BulgariaInstitute of Optical Materials and Technologies “Acad. J. Malinowski”, Bulgarian Academy of Sciences, Acad. G. Bonchev Street, Block 109, 1113 Sofia, BulgariaInstitute of Optical Materials and Technologies “Acad. J. Malinowski”, Bulgarian Academy of Sciences, Acad. G. Bonchev Street, Block 109, 1113 Sofia, BulgariaThin Nb2O5 films with tunable porosity are deposited by the sol-gel and evaporation induced self-assembly methods using organic template Pluronic PE6100 with different molar fractions with respect to NbCl5 used as a precursor for synthesis of Nb sol. Surface morphology and structure of the films are studied by Transmission Electron Microscopy and Selected Area Electron Diffraction. The optical characterization of the films is carried out through reflectance spectra measurements of the films deposited on silicon substrates and theoretical modeling in order to obtain refractive index, extinction coefficient, and thickness of the films. The overall porosity of the films and the amount of adsorbed acetone vapors in the pores are quantified by means of Bruggeman effective medium approximation using already determined optical constants. The sensing properties of the samples are studied by measuring both the reflectance spectra and room-temperature photoluminescence spectra prior to and after exposure to acetone vapors and liquid, respectively. The potential of using the studied mesoporous Nb2O5 films for chemooptical sensing is demonstrated and discussed.http://dx.doi.org/10.1155/2015/403196
spellingShingle Rosen Georgiev
Biliana Georgieva
Marina Vasileva
Petar Ivanov
Tsvetanka Babeva
Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
Advances in Condensed Matter Physics
title Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
title_full Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
title_fullStr Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
title_full_unstemmed Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
title_short Optical Properties of Sol-Gel Nb2O5 Films with Tunable Porosity for Sensing Applications
title_sort optical properties of sol gel nb2o5 films with tunable porosity for sensing applications
url http://dx.doi.org/10.1155/2015/403196
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AT marinavasileva opticalpropertiesofsolgelnb2o5filmswithtunableporosityforsensingapplications
AT petarivanov opticalpropertiesofsolgelnb2o5filmswithtunableporosityforsensingapplications
AT tsvetankababeva opticalpropertiesofsolgelnb2o5filmswithtunableporosityforsensingapplications