Tutorial on high-performance liquid chromatography of isotopologues of organic compounds

Separation of isotopologues or chemical species having different number of neutrons in one or more atoms of specific compound represents an important but difficult task. Application of high-performance liquid chromatography (HPLC) provides some flexibility in various separation modes of isotopologue...

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Main Authors: P.N. Nesterenko, V.D. Kazakova
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Journal of Chromatography Open
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2772391725000052
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author P.N. Nesterenko
V.D. Kazakova
author_facet P.N. Nesterenko
V.D. Kazakova
author_sort P.N. Nesterenko
collection DOAJ
description Separation of isotopologues or chemical species having different number of neutrons in one or more atoms of specific compound represents an important but difficult task. Application of high-performance liquid chromatography (HPLC) provides some flexibility in various separation modes of isotopologues via different isotopic effects. This tutorial describes basic isotopic effects (hydrophobicity, polarizability, acid-base properties, size difference, etc.), which can influence HPLC performance in the separation of isotopologues. The article is focused on separation selectivity of deuterated organic compounds, for which different properties are considered. The use of advanced adsorption materials and techniques is discussed.
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spelling doaj-art-8b0c29e6fb594458bc8f19c977eb11cb2025-08-20T03:00:50ZengElsevierJournal of Chromatography Open2772-39172025-05-01710020710.1016/j.jcoa.2025.100207Tutorial on high-performance liquid chromatography of isotopologues of organic compoundsP.N. Nesterenko0V.D. Kazakova1Corresponding author.; Department of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1/3, GSP-1, Moscow, 119991, RussiaDepartment of Chemistry, Lomonosov Moscow State University, Leninskie Gory, 1/3, GSP-1, Moscow, 119991, RussiaSeparation of isotopologues or chemical species having different number of neutrons in one or more atoms of specific compound represents an important but difficult task. Application of high-performance liquid chromatography (HPLC) provides some flexibility in various separation modes of isotopologues via different isotopic effects. This tutorial describes basic isotopic effects (hydrophobicity, polarizability, acid-base properties, size difference, etc.), which can influence HPLC performance in the separation of isotopologues. The article is focused on separation selectivity of deuterated organic compounds, for which different properties are considered. The use of advanced adsorption materials and techniques is discussed.http://www.sciencedirect.com/science/article/pii/S2772391725000052Liquid chromatographyIsotopologuesRetention mechanismSeparation selectivityIsotope effects
spellingShingle P.N. Nesterenko
V.D. Kazakova
Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
Journal of Chromatography Open
Liquid chromatography
Isotopologues
Retention mechanism
Separation selectivity
Isotope effects
title Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
title_full Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
title_fullStr Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
title_full_unstemmed Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
title_short Tutorial on high-performance liquid chromatography of isotopologues of organic compounds
title_sort tutorial on high performance liquid chromatography of isotopologues of organic compounds
topic Liquid chromatography
Isotopologues
Retention mechanism
Separation selectivity
Isotope effects
url http://www.sciencedirect.com/science/article/pii/S2772391725000052
work_keys_str_mv AT pnnesterenko tutorialonhighperformanceliquidchromatographyofisotopologuesoforganiccompounds
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