Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity

Abstract The immunomodulation of the tumor microenvironment is critical for effective cancer immunotherapy, particularly for tumors that exhibit limited responses to conventional treatments. However, current immune agonists developed for tumor immunomodulation face several challenges, such as poor i...

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Main Authors: Huilan He, Liang Liu, Yun Zheng, Jinlong Ji, Li Cao, Chunlian Ye, Yu Sun, Ying Zhang, Zhiyuan Zhong
Format: Article
Language:English
Published: Wiley 2025-04-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202414110
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author Huilan He
Liang Liu
Yun Zheng
Jinlong Ji
Li Cao
Chunlian Ye
Yu Sun
Ying Zhang
Zhiyuan Zhong
author_facet Huilan He
Liang Liu
Yun Zheng
Jinlong Ji
Li Cao
Chunlian Ye
Yu Sun
Ying Zhang
Zhiyuan Zhong
author_sort Huilan He
collection DOAJ
description Abstract The immunomodulation of the tumor microenvironment is critical for effective cancer immunotherapy, particularly for tumors that exhibit limited responses to conventional treatments. However, current immune agonists developed for tumor immunomodulation face several challenges, such as poor intratumoral retention, inadequate biocompatibility, and restricted cellular targets, which ultimately hamper their therapeutic efficacy and clinical application. In this study, a tumor‐adhesive chitosan‐tethered immune agonist construct (TACTIC) is introduced, which demonstrates good biocompatibility and robust immunostimulatory effects, enhancing the immunogenicity of tumor cells while simultaneously stimulating pro‐inflammatory responses in various immune cell populations. Mechanistic investigations reveal that TACTIC targets multiple signaling pathways, conferring it to effectively remodel the irradiated tumor microenvironment, improve tumor control on murine cancer models post‐radiotherapy, and elicit systemic immune responses with memory effects. The findings highlight the potential of TACTIC as a powerful macromolecular immune adjuvant, paving the way for its broader application in innovative cancer immunotherapies.
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id doaj-art-8a982e29b89a497b8a0ffb2673ed6ff3
institution OA Journals
issn 2198-3844
language English
publishDate 2025-04-01
publisher Wiley
record_format Article
series Advanced Science
spelling doaj-art-8a982e29b89a497b8a0ffb2673ed6ff32025-08-20T02:18:32ZengWileyAdvanced Science2198-38442025-04-011216n/an/a10.1002/advs.202414110Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer ImmunityHuilan He0Liang Liu1Yun Zheng2Jinlong Ji3Li Cao4Chunlian Ye5Yu Sun6Ying Zhang7Zhiyuan Zhong8College of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaCollege of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaCollege of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaBiomedical Polymers LaboratoryCollege of Chemistry, Chemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123 ChinaCollege of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaBiomedical Polymers LaboratoryCollege of Chemistry, Chemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123 ChinaBiomedical Polymers LaboratoryCollege of Chemistry, Chemical Engineering and Materials ScienceSoochow UniversitySuzhou 215123 ChinaCollege of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaCollege of Pharmaceutical Sciences and State Key Laboratory of Radiation Medicine and Protection Soochow University Suzhou 215123 ChinaAbstract The immunomodulation of the tumor microenvironment is critical for effective cancer immunotherapy, particularly for tumors that exhibit limited responses to conventional treatments. However, current immune agonists developed for tumor immunomodulation face several challenges, such as poor intratumoral retention, inadequate biocompatibility, and restricted cellular targets, which ultimately hamper their therapeutic efficacy and clinical application. In this study, a tumor‐adhesive chitosan‐tethered immune agonist construct (TACTIC) is introduced, which demonstrates good biocompatibility and robust immunostimulatory effects, enhancing the immunogenicity of tumor cells while simultaneously stimulating pro‐inflammatory responses in various immune cell populations. Mechanistic investigations reveal that TACTIC targets multiple signaling pathways, conferring it to effectively remodel the irradiated tumor microenvironment, improve tumor control on murine cancer models post‐radiotherapy, and elicit systemic immune responses with memory effects. The findings highlight the potential of TACTIC as a powerful macromolecular immune adjuvant, paving the way for its broader application in innovative cancer immunotherapies.https://doi.org/10.1002/advs.202414110cancer therapyimmune agonistimmunomodulationmulti‐targetsradiotherapy
spellingShingle Huilan He
Liang Liu
Yun Zheng
Jinlong Ji
Li Cao
Chunlian Ye
Yu Sun
Ying Zhang
Zhiyuan Zhong
Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
Advanced Science
cancer therapy
immune agonist
immunomodulation
multi‐targets
radiotherapy
title Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
title_full Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
title_fullStr Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
title_full_unstemmed Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
title_short Tumor‐Adhesive Chitosan‐Derived Multi‐Immune Agonist Unleashes Strong and Durable Anti‐Cancer Immunity
title_sort tumor adhesive chitosan derived multi immune agonist unleashes strong and durable anti cancer immunity
topic cancer therapy
immune agonist
immunomodulation
multi‐targets
radiotherapy
url https://doi.org/10.1002/advs.202414110
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