Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs

Most novel active pharmaceutical ingredients have low water solubility; therefore, solubility-enhancing methods are applied. The aim of the present investigation is to study the impact of nine commonly used pharmaceutical excipients (fillers, surfactants, cyclodextrins, polymers) on solubility, perm...

Full description

Saved in:
Bibliographic Details
Main Authors: Vivien Bárdos, Rita Szolláth, Petra Tőzsér, Arash Mirzahosseini, Bálint Sinkó, Réka Angi, Krisztina Takács-Novák
Format: Article
Language:English
Published: MDPI AG 2025-04-01
Series:Scientia Pharmaceutica
Subjects:
Online Access:https://www.mdpi.com/2218-0532/93/2/19
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849425316195336192
author Vivien Bárdos
Rita Szolláth
Petra Tőzsér
Arash Mirzahosseini
Bálint Sinkó
Réka Angi
Krisztina Takács-Novák
author_facet Vivien Bárdos
Rita Szolláth
Petra Tőzsér
Arash Mirzahosseini
Bálint Sinkó
Réka Angi
Krisztina Takács-Novák
author_sort Vivien Bárdos
collection DOAJ
description Most novel active pharmaceutical ingredients have low water solubility; therefore, solubility-enhancing methods are applied. The aim of the present investigation is to study the impact of nine commonly used pharmaceutical excipients (fillers, surfactants, cyclodextrins, polymers) on solubility, permeability and their relationship. This is crucial for ensuring optimal bioavailability. Carbamazepine, naproxen and pimobendan were chosen as model compounds due to their different acid–base properties. Equilibrium solubility was measured by the traditional shake flask method. Effective permeability was determined by the PAMPA model. Measurements of ionizable compounds were carried out at three pH values. The pH-dependent change in the investigated parameters is maintained even in the presence of excipients. Fillers resulted in a slight or no effect, while the impact of other excipients showed a significant concentration dependence. The impact of excipients was influenced by the structure and ionization state of the molecules. The dominance of the ionized form moderates the impact of excipients. The changes in solubility were more pronounced than in the case of permeability. By examining the effect of the ionization state and interactions with excipients, this work supports the development of formulations that enhance solubility with minimal impacts on permeability. Additionally, it can serve as good basis for preformulation studies and design optimization.
format Article
id doaj-art-8a824afefabb4b669c0f06b14cc20d64
institution Kabale University
issn 0036-8709
2218-0532
language English
publishDate 2025-04-01
publisher MDPI AG
record_format Article
series Scientia Pharmaceutica
spelling doaj-art-8a824afefabb4b669c0f06b14cc20d642025-08-20T03:29:48ZengMDPI AGScientia Pharmaceutica0036-87092218-05322025-04-019321910.3390/scipharm93020019Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II DrugsVivien Bárdos0Rita Szolláth1Petra Tőzsér2Arash Mirzahosseini3Bálint Sinkó4Réka Angi5Krisztina Takács-Novák6Department of Pharmaceutical Chemistry, Semmelweis University, 9 Hőgyes Endre Street, H-1092 Budapest, HungaryDepartment of Pharmaceutical Chemistry, Semmelweis University, 9 Hőgyes Endre Street, H-1092 Budapest, HungaryDepartment of Organic Chemistry and Technology, Faculty of Chemical Technology and Biotechnology, Budapest University of Technology and Economics, 3 Műegyetem rkp., H-1111 Budapest, HungaryDepartment of Pharmaceutical Chemistry, Semmelweis University, 9 Hőgyes Endre Street, H-1092 Budapest, HungaryPion Inc., 10 Cook Street, Billerica, MA 01821, USADepartment of Pharmaceutical Chemistry, Semmelweis University, 9 Hőgyes Endre Street, H-1092 Budapest, HungaryDepartment of Pharmaceutical Chemistry, Semmelweis University, 9 Hőgyes Endre Street, H-1092 Budapest, HungaryMost novel active pharmaceutical ingredients have low water solubility; therefore, solubility-enhancing methods are applied. The aim of the present investigation is to study the impact of nine commonly used pharmaceutical excipients (fillers, surfactants, cyclodextrins, polymers) on solubility, permeability and their relationship. This is crucial for ensuring optimal bioavailability. Carbamazepine, naproxen and pimobendan were chosen as model compounds due to their different acid–base properties. Equilibrium solubility was measured by the traditional shake flask method. Effective permeability was determined by the PAMPA model. Measurements of ionizable compounds were carried out at three pH values. The pH-dependent change in the investigated parameters is maintained even in the presence of excipients. Fillers resulted in a slight or no effect, while the impact of other excipients showed a significant concentration dependence. The impact of excipients was influenced by the structure and ionization state of the molecules. The dominance of the ionized form moderates the impact of excipients. The changes in solubility were more pronounced than in the case of permeability. By examining the effect of the ionization state and interactions with excipients, this work supports the development of formulations that enhance solubility with minimal impacts on permeability. Additionally, it can serve as good basis for preformulation studies and design optimization.https://www.mdpi.com/2218-0532/93/2/19BCS II APIspharmaceutical excipientsSSFPAMPAequilibrium solubilityintestinal permeability
spellingShingle Vivien Bárdos
Rita Szolláth
Petra Tőzsér
Arash Mirzahosseini
Bálint Sinkó
Réka Angi
Krisztina Takács-Novák
Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
Scientia Pharmaceutica
BCS II APIs
pharmaceutical excipients
SSF
PAMPA
equilibrium solubility
intestinal permeability
title Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
title_full Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
title_fullStr Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
title_full_unstemmed Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
title_short Study of the Influence of Pharmaceutical Excipients on the Solubility and Permeability of BCS Class II Drugs
title_sort study of the influence of pharmaceutical excipients on the solubility and permeability of bcs class ii drugs
topic BCS II APIs
pharmaceutical excipients
SSF
PAMPA
equilibrium solubility
intestinal permeability
url https://www.mdpi.com/2218-0532/93/2/19
work_keys_str_mv AT vivienbardos studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT ritaszollath studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT petratozser studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT arashmirzahosseini studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT balintsinko studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT rekaangi studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs
AT krisztinatakacsnovak studyoftheinfluenceofpharmaceuticalexcipientsonthesolubilityandpermeabilityofbcsclassiidrugs