Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines

The problem of searching biologically active compounds amidst xanthine derivatives is a crucial one and is an issue for long-term investigation. Aim. In order to find new biologically active compounds among xanthine derivatives, undescribed earlier 8-benzylidenhydrazino-1-p-methylbenzyltheobromin...

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Main Author: D. G. Ivanchenko
Format: Article
Language:English
Published: Zaporizhzhia State Medical and Pharmaceutical University 2015-10-01
Series:Zaporožskij Medicinskij Žurnal
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Online Access:http://zmj.zsmu.edu.ua/article/view/53768/50333
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author D. G. Ivanchenko
author_facet D. G. Ivanchenko
author_sort D. G. Ivanchenko
collection DOAJ
description The problem of searching biologically active compounds amidst xanthine derivatives is a crucial one and is an issue for long-term investigation. Aim. In order to find new biologically active compounds among xanthine derivatives, undescribed earlier 8-benzylidenhydrazino-1-p-methylbenzyltheobromines have been synthesized. Methods and results. Reaction of 1-p-methylbenzyl-8-bromoxanthine with the excess of hydrazine hydrate in the aqueous dioxane is implemented through formation of 8-hydrazine-1(4-methylbenzyl)theobromine. Through the interaction of 8-hydrazinetheobromine with aldehydes in aqueous propan-2-ol respective 8-benzylidenhydrazino-1-p-methylbenzyltheobromines have been obtained. Structure of synthesized compounds has been definitely proved by NMR-spectroscopy. Conclusions. Molecular and pharmacological descriptors of obtained substances have been calculated. The antioxidant activity of the obtained compounds has been explored. Priorities for further search of biologically active compounds in a range of xanthine derivatives have been set out.
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spelling doaj-art-89da6f8d04024347bb3cb4fefd49bc5c2025-08-20T01:58:12ZengZaporizhzhia State Medical and Pharmaceutical UniversityZaporožskij Medicinskij Žurnal2306-41452310-12102015-10-0158992http://dx.doi.org/10.14739/2310-1210.2015.5.53768Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobrominesD. G. IvanchenkoThe problem of searching biologically active compounds amidst xanthine derivatives is a crucial one and is an issue for long-term investigation. Aim. In order to find new biologically active compounds among xanthine derivatives, undescribed earlier 8-benzylidenhydrazino-1-p-methylbenzyltheobromines have been synthesized. Methods and results. Reaction of 1-p-methylbenzyl-8-bromoxanthine with the excess of hydrazine hydrate in the aqueous dioxane is implemented through formation of 8-hydrazine-1(4-methylbenzyl)theobromine. Through the interaction of 8-hydrazinetheobromine with aldehydes in aqueous propan-2-ol respective 8-benzylidenhydrazino-1-p-methylbenzyltheobromines have been obtained. Structure of synthesized compounds has been definitely proved by NMR-spectroscopy. Conclusions. Molecular and pharmacological descriptors of obtained substances have been calculated. The antioxidant activity of the obtained compounds has been explored. Priorities for further search of biologically active compounds in a range of xanthine derivatives have been set out.http://zmj.zsmu.edu.ua/article/view/53768/50333XanthineOrganic SynthesisNMR-spectroscopyAcute ToxicityAntioxidant Effect
spellingShingle D. G. Ivanchenko
Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
Zaporožskij Medicinskij Žurnal
Xanthine
Organic Synthesis
NMR-spectroscopy
Acute Toxicity
Antioxidant Effect
title Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
title_full Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
title_fullStr Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
title_full_unstemmed Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
title_short Synthesis, physical-chemical and biological properties of 1.8-disubstituted of theobromine. V. 8-Benzylidenhydrazino-1-p-methylbenzyltheobromines
title_sort synthesis physical chemical and biological properties of 1 8 disubstituted of theobromine v 8 benzylidenhydrazino 1 p methylbenzyltheobromines
topic Xanthine
Organic Synthesis
NMR-spectroscopy
Acute Toxicity
Antioxidant Effect
url http://zmj.zsmu.edu.ua/article/view/53768/50333
work_keys_str_mv AT dgivanchenko synthesisphysicalchemicalandbiologicalpropertiesof18disubstitutedoftheobrominev8benzylidenhydrazino1pmethylbenzyltheobromines