Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion

Carbon-based nanomaterials have been explored as effective adsorbents to remove bilirubin in hemoperfusion therapy. However, developing carbon-based absorbents with both high adsorption capacity and good hemocompatibility remains a challenge in clinical applications. In this study, an efficient adso...

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Main Authors: Futao Wang, Xiangyun Zheng, Qi Zhao, Yuchen Feng, Guanyue Gao, Dalibor M. Stanković, Jinfang Zhi
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Functional Diamond
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Online Access:http://dx.doi.org/10.1080/26941112.2023.2300475
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author Futao Wang
Xiangyun Zheng
Qi Zhao
Yuchen Feng
Guanyue Gao
Dalibor M. Stanković
Jinfang Zhi
author_facet Futao Wang
Xiangyun Zheng
Qi Zhao
Yuchen Feng
Guanyue Gao
Dalibor M. Stanković
Jinfang Zhi
author_sort Futao Wang
collection DOAJ
description Carbon-based nanomaterials have been explored as effective adsorbents to remove bilirubin in hemoperfusion therapy. However, developing carbon-based absorbents with both high adsorption capacity and good hemocompatibility remains a challenge in clinical applications. In this study, an efficient adsorbent for bilirubin removal was fabricated by grafting polyaniline (PANI) onto nanodiamonds (NDs). The nanocomposite ND-PANI had negligible effect on the hemolytic activity, confirming its excellent blood compatibility. The adsorption results revealed that the ND-PANI had high adsorption capacities (947 mg/g) and rapid adsorption rate toward bilirubin. Moreover, it exhibited efficient bilirubin adsorption in bovine serum albumin (BSA) solution, indicating its potential for practical application. Additionally, the adsorption kinetics and isotherms were systematically analyzed and modeled, thereby offering insights into the possible adsorption mechanism. Our findings suggest that the ND-PANI could be used as an efficient sorbent for the bilirubin removal, offering a promising avenue for blood purification application.
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id doaj-art-893ec3b4e3c9490c983079f1315fcbb1
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issn 2694-1120
language English
publishDate 2024-12-01
publisher Taylor & Francis Group
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series Functional Diamond
spelling doaj-art-893ec3b4e3c9490c983079f1315fcbb12025-08-20T03:14:58ZengTaylor & Francis GroupFunctional Diamond2694-11202024-12-014110.1080/26941112.2023.23004752300475Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusionFutao Wang0Xiangyun Zheng1Qi Zhao2Yuchen Feng3Guanyue Gao4Dalibor M. Stanković5Jinfang Zhi6Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesKey Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesKey Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesKey Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesKey Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesInnovation Center of the Faculty of Chemistry, University of BelgradeKey Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of SciencesCarbon-based nanomaterials have been explored as effective adsorbents to remove bilirubin in hemoperfusion therapy. However, developing carbon-based absorbents with both high adsorption capacity and good hemocompatibility remains a challenge in clinical applications. In this study, an efficient adsorbent for bilirubin removal was fabricated by grafting polyaniline (PANI) onto nanodiamonds (NDs). The nanocomposite ND-PANI had negligible effect on the hemolytic activity, confirming its excellent blood compatibility. The adsorption results revealed that the ND-PANI had high adsorption capacities (947 mg/g) and rapid adsorption rate toward bilirubin. Moreover, it exhibited efficient bilirubin adsorption in bovine serum albumin (BSA) solution, indicating its potential for practical application. Additionally, the adsorption kinetics and isotherms were systematically analyzed and modeled, thereby offering insights into the possible adsorption mechanism. Our findings suggest that the ND-PANI could be used as an efficient sorbent for the bilirubin removal, offering a promising avenue for blood purification application.http://dx.doi.org/10.1080/26941112.2023.2300475nanodiamondsbilirubinadsorptionhemoperfusion
spellingShingle Futao Wang
Xiangyun Zheng
Qi Zhao
Yuchen Feng
Guanyue Gao
Dalibor M. Stanković
Jinfang Zhi
Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
Functional Diamond
nanodiamonds
bilirubin
adsorption
hemoperfusion
title Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
title_full Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
title_fullStr Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
title_full_unstemmed Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
title_short Fabrication of nanodiamonds/polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
title_sort fabrication of nanodiamonds polyaniline nanocomposite for bilirubin adsorption in hemoperfusion
topic nanodiamonds
bilirubin
adsorption
hemoperfusion
url http://dx.doi.org/10.1080/26941112.2023.2300475
work_keys_str_mv AT futaowang fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT xiangyunzheng fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT qizhao fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT yuchenfeng fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT guanyuegao fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT dalibormstankovic fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion
AT jinfangzhi fabricationofnanodiamondspolyanilinenanocompositeforbilirubinadsorptioninhemoperfusion