Toward Attosecond Vortices in Semiconductor Materials

We present theoretical results on the generation of short-wavelength vortex beams in semiconductors through their interaction with an intense Laguerre–Gauss (LG) beam, in the regime where nonperturbative high-order harmonics are generated. Our approach leverages key aspects of the microscopic mechan...

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Bibliographic Details
Main Authors: Camilo Granados, Bikash K. Das, Christian Heide, Shambhu Ghimire, Marcelo F. Ciappina
Format: Article
Language:English
Published: American Association for the Advancement of Science (AAAS) 2025-01-01
Series:Ultrafast Science
Online Access:https://spj.science.org/doi/10.34133/ultrafastscience.0100
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Summary:We present theoretical results on the generation of short-wavelength vortex beams in semiconductors through their interaction with an intense Laguerre–Gauss (LG) beam, in the regime where nonperturbative high-order harmonics are generated. Our approach leverages key aspects of the microscopic mechanism for high-order harmonic generation (HHG) in condensed matter, including the incorporation of dephasing time in the semiconductor Bloch equations (SBEs), the integration of the SBE model with the thin-slab model, and the application of experimentally validated scaling laws for different harmonic orders. For our simulations, we use a zinc oxide crystal interacting with an LG vortex beam characterized by a topological charge of [Formula: see text]. Time-domain analysis reveals that this is a feasible route, by synthesizing several harmonics, toward the generation of twisted attosecond pulse trains. These findings contribute to advancing the understanding of solid-state media interacting with structured light.
ISSN:2765-8791