Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma

Polysulfone/polyethylene glycol (PSF/PEG) membranes were prepared by dry/wet phase inversion method. Effects of direct current glow discharge plasma using argon as working gas on morphological structures and gas separation properties of membranes were studied. Alteration of membrane characteristics...

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Main Authors: Chalad Yuenyao, Thawat Chittrakarn, Yutthana Tirawanichakul, Suksawat Sirijarukul
Format: Article
Language:English
Published: Wiley 2016-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2016/4759150
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author Chalad Yuenyao
Thawat Chittrakarn
Yutthana Tirawanichakul
Suksawat Sirijarukul
author_facet Chalad Yuenyao
Thawat Chittrakarn
Yutthana Tirawanichakul
Suksawat Sirijarukul
author_sort Chalad Yuenyao
collection DOAJ
description Polysulfone/polyethylene glycol (PSF/PEG) membranes were prepared by dry/wet phase inversion method. Effects of direct current glow discharge plasma using argon as working gas on morphological structures and gas separation properties of membranes were studied. Alteration of membrane characteristics were analyzed by various techniques like contact angle, scanning electron microscope, Fourier transform infrared spectroscopy, and dynamic mechanical thermal analysis. Gas separation properties were measured in terms of permeation and ideal O2/N2 selectivity. Results showed that hydrophilic and gas separation properties of PSF/PEG membranes increased by plasma surface modification. It was also shown that the dosage of PEG and plasma treatment affected the morphological structures and mechanical and gas separation properties. The macro voids and transmembrane structure disappeared with a little amount of PEG dosage. Pore size and mechanical strength tend to decrease with increasing PEG dosage up to 10 wt%. Glass transition temperature (Tg) receded from 201.8 to 143.7°C for pure PSF and PSF/PEG with PEG dosage of 10 wt%. O2 and N2 gases permeation through the 10-minute plasma treated membranes tend to increase. However, the permeation strongly dispersed when treatment time was more extended.
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institution OA Journals
issn 1687-9422
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language English
publishDate 2016-01-01
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series International Journal of Polymer Science
spelling doaj-art-8900d243fc134c488ed27e1c5b5baa0d2025-08-20T02:09:10ZengWileyInternational Journal of Polymer Science1687-94221687-94302016-01-01201610.1155/2016/47591504759150Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge PlasmaChalad Yuenyao0Thawat Chittrakarn1Yutthana Tirawanichakul2Suksawat Sirijarukul3National Research University Project 2014, Prince of Songkla University, Hat Yai, Songkhla 90112, ThailandDepartment of Physics, Faculty of Science, Prince of Songkla University, Hat Yai, Songkhla 90112, ThailandNational Research University Project 2014, Prince of Songkla University, Hat Yai, Songkhla 90112, ThailandDepartment of Physics, Faculty of Science, Prince of Songkla University, Hat Yai, Songkhla 90112, ThailandPolysulfone/polyethylene glycol (PSF/PEG) membranes were prepared by dry/wet phase inversion method. Effects of direct current glow discharge plasma using argon as working gas on morphological structures and gas separation properties of membranes were studied. Alteration of membrane characteristics were analyzed by various techniques like contact angle, scanning electron microscope, Fourier transform infrared spectroscopy, and dynamic mechanical thermal analysis. Gas separation properties were measured in terms of permeation and ideal O2/N2 selectivity. Results showed that hydrophilic and gas separation properties of PSF/PEG membranes increased by plasma surface modification. It was also shown that the dosage of PEG and plasma treatment affected the morphological structures and mechanical and gas separation properties. The macro voids and transmembrane structure disappeared with a little amount of PEG dosage. Pore size and mechanical strength tend to decrease with increasing PEG dosage up to 10 wt%. Glass transition temperature (Tg) receded from 201.8 to 143.7°C for pure PSF and PSF/PEG with PEG dosage of 10 wt%. O2 and N2 gases permeation through the 10-minute plasma treated membranes tend to increase. However, the permeation strongly dispersed when treatment time was more extended.http://dx.doi.org/10.1155/2016/4759150
spellingShingle Chalad Yuenyao
Thawat Chittrakarn
Yutthana Tirawanichakul
Suksawat Sirijarukul
Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
International Journal of Polymer Science
title Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
title_full Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
title_fullStr Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
title_full_unstemmed Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
title_short Surface Modification of Asymmetric Polysulfone/Polyethylene Glycol Membranes by DC Ar-Glow Discharge Plasma
title_sort surface modification of asymmetric polysulfone polyethylene glycol membranes by dc ar glow discharge plasma
url http://dx.doi.org/10.1155/2016/4759150
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AT thawatchittrakarn surfacemodificationofasymmetricpolysulfonepolyethyleneglycolmembranesbydcarglowdischargeplasma
AT yutthanatirawanichakul surfacemodificationofasymmetricpolysulfonepolyethyleneglycolmembranesbydcarglowdischargeplasma
AT suksawatsirijarukul surfacemodificationofasymmetricpolysulfonepolyethyleneglycolmembranesbydcarglowdischargeplasma