ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance

This study investigates the photocatalytic degradation of Methyl orange (MO) dye using ZnO/CdS nanocomposites synthesized by the hydrothermal technique. Using XRD, FTIR, FESEM-EDS, TEM, UV-Vis DRS, BET, and XPS, the chemically produced chalcogenide hybrid nanocomposites were thoroughly characterized...

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Main Authors: Anupam Sarker, Shahriar Atik Fahim, Rupna Akther Putul, Humayra Gazi, Shah Md. Masum, Md. Ashraful Islam Molla
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Next Nanotechnology
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Online Access:http://www.sciencedirect.com/science/article/pii/S2949829525000154
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author Anupam Sarker
Shahriar Atik Fahim
Rupna Akther Putul
Humayra Gazi
Shah Md. Masum
Md. Ashraful Islam Molla
author_facet Anupam Sarker
Shahriar Atik Fahim
Rupna Akther Putul
Humayra Gazi
Shah Md. Masum
Md. Ashraful Islam Molla
author_sort Anupam Sarker
collection DOAJ
description This study investigates the photocatalytic degradation of Methyl orange (MO) dye using ZnO/CdS nanocomposites synthesized by the hydrothermal technique. Using XRD, FTIR, FESEM-EDS, TEM, UV-Vis DRS, BET, and XPS, the chemically produced chalcogenide hybrid nanocomposites were thoroughly characterized. The 5 % ZnO/CdS nanocomposite photocatalyst exhibited a crystallite size of 5.63 nm, a bandgap energy of 2.35 eV, and a larger surface area of 118.47 m2/g, indicating excellent photocatalytic performance compared to pristine ZnO and CdS. The best MO removal efficiency of 98.67 % within 60 min is demonstrated by the 5 % ZnO/CdS photocatalyst under UV-C irradiation. The photocatalytic MO degradation reaction maintains a pseudo-first-order kinetic law. The rate constant (k) and half-life (t1/2) are found to be 0.065 min−1 and 10.66 min, respectively. The reusability of the 5 % ZnO/CdS photocatalyst was investigated, and the MO removal efficiency remained acceptable after three cycles. These findings suggest that the synthesized ZnO/CdS nanocomposite is a promising photocatalyst for efficiently and sustainably removing organic pollutants from wastewater.
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spelling doaj-art-8829277983944d3bb0e52bef00da5d222025-08-20T03:15:16ZengElsevierNext Nanotechnology2949-82952025-01-01810014610.1016/j.nxnano.2025.100146ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performanceAnupam Sarker0Shahriar Atik Fahim1Rupna Akther Putul2Humayra Gazi3Shah Md. Masum4Md. Ashraful Islam Molla5Department of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, Bangladesh; Department of Chemistry, American International University-Bangladesh, Dhaka 1229, BangladeshDepartment of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Applied Chemistry and Chemical Engineering, Faculty of Engineering and Technology, University of Dhaka, Dhaka 1000, Bangladesh; Corresponding author.This study investigates the photocatalytic degradation of Methyl orange (MO) dye using ZnO/CdS nanocomposites synthesized by the hydrothermal technique. Using XRD, FTIR, FESEM-EDS, TEM, UV-Vis DRS, BET, and XPS, the chemically produced chalcogenide hybrid nanocomposites were thoroughly characterized. The 5 % ZnO/CdS nanocomposite photocatalyst exhibited a crystallite size of 5.63 nm, a bandgap energy of 2.35 eV, and a larger surface area of 118.47 m2/g, indicating excellent photocatalytic performance compared to pristine ZnO and CdS. The best MO removal efficiency of 98.67 % within 60 min is demonstrated by the 5 % ZnO/CdS photocatalyst under UV-C irradiation. The photocatalytic MO degradation reaction maintains a pseudo-first-order kinetic law. The rate constant (k) and half-life (t1/2) are found to be 0.065 min−1 and 10.66 min, respectively. The reusability of the 5 % ZnO/CdS photocatalyst was investigated, and the MO removal efficiency remained acceptable after three cycles. These findings suggest that the synthesized ZnO/CdS nanocomposite is a promising photocatalyst for efficiently and sustainably removing organic pollutants from wastewater.http://www.sciencedirect.com/science/article/pii/S2949829525000154PhotocatalysisZnO/CdS nanocompositeHydrothermalMethyl orangeUV-C irradiation
spellingShingle Anupam Sarker
Shahriar Atik Fahim
Rupna Akther Putul
Humayra Gazi
Shah Md. Masum
Md. Ashraful Islam Molla
ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
Next Nanotechnology
Photocatalysis
ZnO/CdS nanocomposite
Hydrothermal
Methyl orange
UV-C irradiation
title ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
title_full ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
title_fullStr ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
title_full_unstemmed ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
title_short ZnO/CdS nanocomposites: Synthesis, characterization and assessment of photocatalytic performance
title_sort zno cds nanocomposites synthesis characterization and assessment of photocatalytic performance
topic Photocatalysis
ZnO/CdS nanocomposite
Hydrothermal
Methyl orange
UV-C irradiation
url http://www.sciencedirect.com/science/article/pii/S2949829525000154
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