High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations

Abstract Cancer genomics aims to personalize treatments by identifying genetic abnormalities in cancer cells. However, current analytical techniques face limitations in simplicity and cost-effectiveness. To address these issues, we developed an enhanced capillary gel electrophoresis (CE) sequencer u...

Full description

Saved in:
Bibliographic Details
Main Authors: Nobue Tamamura, Yoshihiko Hagiwara, Hirokazu Kato, Yusuke Ono, Kenji Takahashi, Kazuya Koyama, Hiroki Sato, Tetsuhiro Okada, Hidemasa Kawabata, Yu Ohtaki, Chiho Maeda, Miyuki Mori, Shin-ichi Chiba, Mishie Tanino, Kenzui Taniue, Takashi Anazawa, Ryoji Inaba, Yusuke Mizukami
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Scientific Reports
Subjects:
Online Access:https://doi.org/10.1038/s41598-025-01884-5
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849768822782820352
author Nobue Tamamura
Yoshihiko Hagiwara
Hirokazu Kato
Yusuke Ono
Kenji Takahashi
Kazuya Koyama
Hiroki Sato
Tetsuhiro Okada
Hidemasa Kawabata
Yu Ohtaki
Chiho Maeda
Miyuki Mori
Shin-ichi Chiba
Mishie Tanino
Kenzui Taniue
Takashi Anazawa
Ryoji Inaba
Yusuke Mizukami
author_facet Nobue Tamamura
Yoshihiko Hagiwara
Hirokazu Kato
Yusuke Ono
Kenji Takahashi
Kazuya Koyama
Hiroki Sato
Tetsuhiro Okada
Hidemasa Kawabata
Yu Ohtaki
Chiho Maeda
Miyuki Mori
Shin-ichi Chiba
Mishie Tanino
Kenzui Taniue
Takashi Anazawa
Ryoji Inaba
Yusuke Mizukami
author_sort Nobue Tamamura
collection DOAJ
description Abstract Cancer genomics aims to personalize treatments by identifying genetic abnormalities in cancer cells. However, current analytical techniques face limitations in simplicity and cost-effectiveness. To address these issues, we developed an enhanced capillary gel electrophoresis (CE) sequencer using a fluorescence-acquisition technique called “HiDy” (High Dynamic range) (HiDy-CE). The HiDy-CE reduces the hardware binning region size and increases the number of regions on a charge-coupled device image sensor, expanding the dynamic range and reducing saturation risk. By applying the multi-base primer extension method to the HiDy-CE with control DNA containing known mutations, we detected variant allele frequencies (VAFs) as low as 0.5% for major KRAS hotspot mutation at codon 12 and 13. With 10 ng of DNA from small tissues obtained via fine-needle biopsy from patients with suspected pancreaticoduodenal tumors, HiDy-CE produced equivalent VAFs in KRAS compared with targeted amplicon sequencing. This demonstrated the world’s first capability of detecting mutations below 1% on CE using pathological specimens, leveraging its wide dynamic range. With only 2 ng of input DNA, the HiDy-CE provided results highly concordant with digital PCR with minimal non-specific noise. These findings underscore the HiDy-CE’s potential for sensitive detection of oncogenes such as KRAS, facilitating pre-testing before comprehensive genome profiling.
format Article
id doaj-art-87f584461afd42ce8226ecf23ae9e2ff
institution DOAJ
issn 2045-2322
language English
publishDate 2025-07-01
publisher Nature Portfolio
record_format Article
series Scientific Reports
spelling doaj-art-87f584461afd42ce8226ecf23ae9e2ff2025-08-20T03:03:40ZengNature PortfolioScientific Reports2045-23222025-07-0115111110.1038/s41598-025-01884-5High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutationsNobue Tamamura0Yoshihiko Hagiwara1Hirokazu Kato2Yusuke Ono3Kenji Takahashi4Kazuya Koyama5Hiroki Sato6Tetsuhiro Okada7Hidemasa Kawabata8Yu Ohtaki9Chiho Maeda10Miyuki Mori11Shin-ichi Chiba12Mishie Tanino13Kenzui Taniue14Takashi Anazawa15Ryoji Inaba16Yusuke Mizukami17Department of Advanced Genomic Community Healthcare, Asahikawa Medical UniversityNaka Diagnostic Products Division, Bio Systems Design 1st Department, Hitachi High-Tech CorporationNaka Diagnostic Products Division, Bio Systems Design 1st Department, Hitachi High-Tech CorporationDepartment of Advanced Genomic Community Healthcare, Asahikawa Medical UniversityDepartment of Advanced Genomic Community Healthcare, Asahikawa Medical UniversityDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityInstitute of Biomedical Research, Sapporo-Higashi Tokushukai HospitalInstitute of Biomedical Research, Sapporo-Higashi Tokushukai HospitalCenter for Advanced Research and Education, Asahikawa Medical UniversityDepartment of Diagnostic Pathology, Asahikawa Medical University HospitalDivision of Gastroenterology, Department of Medicine, Asahikawa Medical UniversityHitachi, Ltd.Naka Diagnostic Products Division, Bio Systems Design 1st Department, Hitachi High-Tech CorporationDepartment of Advanced Genomic Community Healthcare, Asahikawa Medical UniversityAbstract Cancer genomics aims to personalize treatments by identifying genetic abnormalities in cancer cells. However, current analytical techniques face limitations in simplicity and cost-effectiveness. To address these issues, we developed an enhanced capillary gel electrophoresis (CE) sequencer using a fluorescence-acquisition technique called “HiDy” (High Dynamic range) (HiDy-CE). The HiDy-CE reduces the hardware binning region size and increases the number of regions on a charge-coupled device image sensor, expanding the dynamic range and reducing saturation risk. By applying the multi-base primer extension method to the HiDy-CE with control DNA containing known mutations, we detected variant allele frequencies (VAFs) as low as 0.5% for major KRAS hotspot mutation at codon 12 and 13. With 10 ng of DNA from small tissues obtained via fine-needle biopsy from patients with suspected pancreaticoduodenal tumors, HiDy-CE produced equivalent VAFs in KRAS compared with targeted amplicon sequencing. This demonstrated the world’s first capability of detecting mutations below 1% on CE using pathological specimens, leveraging its wide dynamic range. With only 2 ng of input DNA, the HiDy-CE provided results highly concordant with digital PCR with minimal non-specific noise. These findings underscore the HiDy-CE’s potential for sensitive detection of oncogenes such as KRAS, facilitating pre-testing before comprehensive genome profiling.https://doi.org/10.1038/s41598-025-01884-5HiDyCapillary gel electrophoresisDynamic rangeLow-frequency mutationKRASFragment analysis
spellingShingle Nobue Tamamura
Yoshihiko Hagiwara
Hirokazu Kato
Yusuke Ono
Kenji Takahashi
Kazuya Koyama
Hiroki Sato
Tetsuhiro Okada
Hidemasa Kawabata
Yu Ohtaki
Chiho Maeda
Miyuki Mori
Shin-ichi Chiba
Mishie Tanino
Kenzui Taniue
Takashi Anazawa
Ryoji Inaba
Yusuke Mizukami
High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
Scientific Reports
HiDy
Capillary gel electrophoresis
Dynamic range
Low-frequency mutation
KRAS
Fragment analysis
title High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
title_full High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
title_fullStr High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
title_full_unstemmed High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
title_short High dynamic range capillary electrophoresis method for sensitive detection of low-frequency driver mutations
title_sort high dynamic range capillary electrophoresis method for sensitive detection of low frequency driver mutations
topic HiDy
Capillary gel electrophoresis
Dynamic range
Low-frequency mutation
KRAS
Fragment analysis
url https://doi.org/10.1038/s41598-025-01884-5
work_keys_str_mv AT nobuetamamura highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT yoshihikohagiwara highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT hirokazukato highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT yusukeono highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT kenjitakahashi highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT kazuyakoyama highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT hirokisato highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT tetsuhirookada highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT hidemasakawabata highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT yuohtaki highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT chihomaeda highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT miyukimori highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT shinichichiba highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT mishietanino highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT kenzuitaniue highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT takashianazawa highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT ryojiinaba highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations
AT yusukemizukami highdynamicrangecapillaryelectrophoresismethodforsensitivedetectionoflowfrequencydrivermutations