AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma

Abstract Background Lymphoma is a malignant tumor of the immune system and its incidence is increasing year after year, causing a major threat to people's health. Conventional diagnosis of lymphoma basically depends on histological images consuming long-time and tedious manipulations (e.g., 7–1...

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Main Authors: Haiting Cao, Xiaofeng Wu, Huayi Shi, Binbin Chu, Yao He, Houyu Wang, Fenglin Dong
Format: Article
Language:English
Published: BMC 2025-04-01
Series:Journal of Nanobiotechnology
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Online Access:https://doi.org/10.1186/s12951-025-03339-5
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author Haiting Cao
Xiaofeng Wu
Huayi Shi
Binbin Chu
Yao He
Houyu Wang
Fenglin Dong
author_facet Haiting Cao
Xiaofeng Wu
Huayi Shi
Binbin Chu
Yao He
Houyu Wang
Fenglin Dong
author_sort Haiting Cao
collection DOAJ
description Abstract Background Lymphoma is a malignant tumor of the immune system and its incidence is increasing year after year, causing a major threat to people's health. Conventional diagnosis of lymphoma basically depends on histological images consuming long-time and tedious manipulations (e.g., 7–15 days) and large-field view (e.g., > 1000 × 1000 μm2). Artificial intelligence has recently revolutionized cancer diagnosis by training pathological image databases via deep learning. Current approaches, however, remain dependent on analyzing wide-field pathological images to detect distinct nuclear, cytologic, and histomorphologic traits for diagnostic categorization, limiting their applicability to minimally invasive lesion. Results Herein, we develop a molecular imaging strategy for minimally invasive lymphoma diagnosis. By spreading lymphoma tissue sections tightly on a surface-enhanced Raman scattering (SERS) chip, label-free images of DNA double strand breaks (DSBs) in 30 × 30 μm2 tissue sections could be achieved in ~ 15 min. To establish a proof of concept, the Raman image datasets collected from clinical samples of normal lymphatic tissues and non-Hodgkin's lymphoma (NHL) tissues were well organized and trained in a deep convolutional neural network model, finally achieving a recognition rate of ~ 91.7 ± 2.1%. Conclusions The molecular imaging strategy for minimally invasive lymphoma diagnosis that can achieve a recognition rate of ~ 91.7 ± 2.1%. We anticipate that these results will catalyze the development of a series of histological SERS-AI technologies for diagnosing various diseases, including other types of cancer. In this work, we present a reliable tool to facilitate clinicians in the diagnosis of lymphoma. Graphical Abstract
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spelling doaj-art-8655a7f631aa4b51995802ff515052bb2025-08-20T03:18:42ZengBMCJournal of Nanobiotechnology1477-31552025-04-0123111110.1186/s12951-025-03339-5AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphomaHaiting Cao0Xiaofeng Wu1Huayi Shi2Binbin Chu3Yao He4Houyu Wang5Fenglin Dong6Suzhou Key Laboratory of Nanotechnology and Biomedicine, Institute of Functional Nano & Soft Materials (FUNSOM), and Collaborative Innovation Center of Suzhou Nano Science and Technology (NANO-CIC), Soochow UniversityDepartment of Ultrasound, The First Affiliated Hospital of Soochow UniversitySuzhou Key Laboratory of Nanotechnology and Biomedicine, Institute of Functional Nano & Soft Materials (FUNSOM), and Collaborative Innovation Center of Suzhou Nano Science and Technology (NANO-CIC), Soochow UniversitySuzhou Key Laboratory of Nanotechnology and Biomedicine, Institute of Functional Nano & Soft Materials (FUNSOM), and Collaborative Innovation Center of Suzhou Nano Science and Technology (NANO-CIC), Soochow UniversitySuzhou Key Laboratory of Nanotechnology and Biomedicine, Institute of Functional Nano & Soft Materials (FUNSOM), and Collaborative Innovation Center of Suzhou Nano Science and Technology (NANO-CIC), Soochow UniversitySuzhou Key Laboratory of Nanotechnology and Biomedicine, Institute of Functional Nano & Soft Materials (FUNSOM), and Collaborative Innovation Center of Suzhou Nano Science and Technology (NANO-CIC), Soochow UniversityDepartment of Ultrasound, The First Affiliated Hospital of Soochow UniversityAbstract Background Lymphoma is a malignant tumor of the immune system and its incidence is increasing year after year, causing a major threat to people's health. Conventional diagnosis of lymphoma basically depends on histological images consuming long-time and tedious manipulations (e.g., 7–15 days) and large-field view (e.g., > 1000 × 1000 μm2). Artificial intelligence has recently revolutionized cancer diagnosis by training pathological image databases via deep learning. Current approaches, however, remain dependent on analyzing wide-field pathological images to detect distinct nuclear, cytologic, and histomorphologic traits for diagnostic categorization, limiting their applicability to minimally invasive lesion. Results Herein, we develop a molecular imaging strategy for minimally invasive lymphoma diagnosis. By spreading lymphoma tissue sections tightly on a surface-enhanced Raman scattering (SERS) chip, label-free images of DNA double strand breaks (DSBs) in 30 × 30 μm2 tissue sections could be achieved in ~ 15 min. To establish a proof of concept, the Raman image datasets collected from clinical samples of normal lymphatic tissues and non-Hodgkin's lymphoma (NHL) tissues were well organized and trained in a deep convolutional neural network model, finally achieving a recognition rate of ~ 91.7 ± 2.1%. Conclusions The molecular imaging strategy for minimally invasive lymphoma diagnosis that can achieve a recognition rate of ~ 91.7 ± 2.1%. We anticipate that these results will catalyze the development of a series of histological SERS-AI technologies for diagnosing various diseases, including other types of cancer. In this work, we present a reliable tool to facilitate clinicians in the diagnosis of lymphoma. Graphical Abstracthttps://doi.org/10.1186/s12951-025-03339-5SERSConvolutional neural networkLymphomaMinimally invasive diagnosis
spellingShingle Haiting Cao
Xiaofeng Wu
Huayi Shi
Binbin Chu
Yao He
Houyu Wang
Fenglin Dong
AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
Journal of Nanobiotechnology
SERS
Convolutional neural network
Lymphoma
Minimally invasive diagnosis
title AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
title_full AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
title_fullStr AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
title_full_unstemmed AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
title_short AI-assisted SERS imaging method for label-free and rapid discrimination of clinical lymphoma
title_sort ai assisted sers imaging method for label free and rapid discrimination of clinical lymphoma
topic SERS
Convolutional neural network
Lymphoma
Minimally invasive diagnosis
url https://doi.org/10.1186/s12951-025-03339-5
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