Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods

The geometry, electronic structure and stability of endohedral complexes Pdn@C60, n=1,…,4, were investigated by a quantum chemistry method (DFT/PBE). The heat of formation ΔНf of a complex consisting of C60 and n Pd atoms was used as a measure of complex stability. In particular, it was is establish...

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Main Authors: G. E. Gal’pern, I. V. Stankevich, M. I. Skvortsova
Format: Article
Language:Russian
Published: MIREA - Russian Technological University 2011-12-01
Series:Тонкие химические технологии
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Online Access:https://www.finechem-mirea.ru/jour/article/view/1181
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author G. E. Gal’pern
I. V. Stankevich
M. I. Skvortsova
author_facet G. E. Gal’pern
I. V. Stankevich
M. I. Skvortsova
author_sort G. E. Gal’pern
collection DOAJ
description The geometry, electronic structure and stability of endohedral complexes Pdn@C60, n=1,…,4, were investigated by a quantum chemistry method (DFT/PBE). The heat of formation ΔНf of a complex consisting of C60 and n Pd atoms was used as a measure of complex stability. In particular, it was is established that this reaction is exothermal for n=1-3 and endothermal for n=4.
format Article
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institution Kabale University
issn 2410-6593
2686-7575
language Russian
publishDate 2011-12-01
publisher MIREA - Russian Technological University
record_format Article
series Тонкие химические технологии
spelling doaj-art-862dafc19d8e4b6d867a343a5bb394682025-08-20T03:56:23ZrusMIREA - Russian Technological UniversityТонкие химические технологии2410-65932686-75752011-12-016619221175Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methodsG. E. Gal’pern0I. V. Stankevich1M. I. Skvortsova2M.V. Lomonosov Moscow State University of Fine Chemical Technologies, 86, Vernadskogo pr., Moscow 119571M.V. Lomonosov Moscow State University of Fine Chemical Technologies, 86, Vernadskogo pr., Moscow 119571Институт элементоорганических соединений им. А.Н. Несмеянова РАНThe geometry, electronic structure and stability of endohedral complexes Pdn@C60, n=1,…,4, were investigated by a quantum chemistry method (DFT/PBE). The heat of formation ΔНf of a complex consisting of C60 and n Pd atoms was used as a measure of complex stability. In particular, it was is established that this reaction is exothermal for n=1-3 and endothermal for n=4.https://www.finechem-mirea.ru/jour/article/view/1181fullerenespalladiumendohedral complexesquantum chemistrydft/pbe methodelectron density functionalaffinity to electronatom charges
spellingShingle G. E. Gal’pern
I. V. Stankevich
M. I. Skvortsova
Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
Тонкие химические технологии
fullerenes
palladium
endohedral complexes
quantum chemistry
dft/pbe method
electron density functional
affinity to electron
atom charges
title Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
title_full Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
title_fullStr Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
title_full_unstemmed Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
title_short Investigation of the geometry and electronic structure of endohedral complexes Pd<sub>n</sub>@C<sub>60</sub>, n=1,…,4, by quantum chemistry methods
title_sort investigation of the geometry and electronic structure of endohedral complexes pd sub n sub c sub 60 sub n 1 4 by quantum chemistry methods
topic fullerenes
palladium
endohedral complexes
quantum chemistry
dft/pbe method
electron density functional
affinity to electron
atom charges
url https://www.finechem-mirea.ru/jour/article/view/1181
work_keys_str_mv AT gegalpern investigationofthegeometryandelectronicstructureofendohedralcomplexespdsubnsubcsub60subn14byquantumchemistrymethods
AT ivstankevich investigationofthegeometryandelectronicstructureofendohedralcomplexespdsubnsubcsub60subn14byquantumchemistrymethods
AT miskvortsova investigationofthegeometryandelectronicstructureofendohedralcomplexespdsubnsubcsub60subn14byquantumchemistrymethods