Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification

Abstract Ferrate (Fe(VI)) is a prospective green oxidant owing to producing highly reactive Fe(IV)/Fe(V) for micropollutant degradation. However, the performance is significantly compromised by the severe side reaction of Fe(VI) self-decay with H2O, generating H2O2 byproduct that quickly quenches Fe...

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Main Authors: Yundan Chen, Xiaofei Ge, Jun Li, Zishuai Bill Zhang, Zhenshan Li
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-62930-4
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author Yundan Chen
Xiaofei Ge
Jun Li
Zishuai Bill Zhang
Zhenshan Li
author_facet Yundan Chen
Xiaofei Ge
Jun Li
Zishuai Bill Zhang
Zhenshan Li
author_sort Yundan Chen
collection DOAJ
description Abstract Ferrate (Fe(VI)) is a prospective green oxidant owing to producing highly reactive Fe(IV)/Fe(V) for micropollutant degradation. However, the performance is significantly compromised by the severe side reaction of Fe(VI) self-decay with H2O, generating H2O2 byproduct that quickly quenches Fe(IV)/Fe(V). In this study, we synthesized a single-ruthenium-atom catalyst (RuGN) to activate Fe(VI) to selectively produce Fe(IV)/Fe(V)/Ru(V) for antibiotic degradation, with record-fast ciprofloxacin (CIP) degradation kinetics (~18.7 min−1 g−1 L). Since Fe(VI) preferentially reacts with RuGN rather than H2O, RuGN inhibits Fe(VI) self-decay, thus decreasing the H2O2 production. Moreover, RuGN consumes H2O2 (that quenches Fe(IV)/Fe(V)/Ru(V)) in the reaction system, which significantly improves the Fe(VI) utilization rate. Compared with other typical transition metal single-atom catalysts, RuGN exhibits moderate interactions with Fe(VI) and thus facilitates the electron transfer via Ru-O-Fe coordination to activate Fe(VI) for efficient CIP degradation. The RuGN/Fe(VI) system resists interference from background substances coexisting in water, achieving efficient CIP degradation under complex water chemistry conditions and in real water samples. The system can also efficiently degrade CIP in continuous-flow reactors. This work develops a promising strategy for improving Fe(VI) activation via regulating the interaction between the metal site and Fe(VI), holding immense potential for deep wastewater purification.
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spelling doaj-art-85874f5de2194dda809cd6942cb7d6062025-08-20T03:05:14ZengNature PortfolioNature Communications2041-17232025-08-0116111210.1038/s41467-025-62930-4Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purificationYundan Chen0Xiaofei Ge1Jun Li2Zishuai Bill Zhang3Zhenshan Li4The Key Laboratory of Water and Sediment Sciences, Ministry of Education, College of Environmental Sciences and Engineering, Peking UniversityThe Key Laboratory of Water and Sediment Sciences, Ministry of Education, College of Environmental Sciences and Engineering, Peking UniversityFrontiers Science Center for Transformative Molecules, Shanghai Jiao tong UniversityThe Key Laboratory of Water and Sediment Sciences, Ministry of Education, College of Environmental Sciences and Engineering, Peking UniversityThe Key Laboratory of Water and Sediment Sciences, Ministry of Education, College of Environmental Sciences and Engineering, Peking UniversityAbstract Ferrate (Fe(VI)) is a prospective green oxidant owing to producing highly reactive Fe(IV)/Fe(V) for micropollutant degradation. However, the performance is significantly compromised by the severe side reaction of Fe(VI) self-decay with H2O, generating H2O2 byproduct that quickly quenches Fe(IV)/Fe(V). In this study, we synthesized a single-ruthenium-atom catalyst (RuGN) to activate Fe(VI) to selectively produce Fe(IV)/Fe(V)/Ru(V) for antibiotic degradation, with record-fast ciprofloxacin (CIP) degradation kinetics (~18.7 min−1 g−1 L). Since Fe(VI) preferentially reacts with RuGN rather than H2O, RuGN inhibits Fe(VI) self-decay, thus decreasing the H2O2 production. Moreover, RuGN consumes H2O2 (that quenches Fe(IV)/Fe(V)/Ru(V)) in the reaction system, which significantly improves the Fe(VI) utilization rate. Compared with other typical transition metal single-atom catalysts, RuGN exhibits moderate interactions with Fe(VI) and thus facilitates the electron transfer via Ru-O-Fe coordination to activate Fe(VI) for efficient CIP degradation. The RuGN/Fe(VI) system resists interference from background substances coexisting in water, achieving efficient CIP degradation under complex water chemistry conditions and in real water samples. The system can also efficiently degrade CIP in continuous-flow reactors. This work develops a promising strategy for improving Fe(VI) activation via regulating the interaction between the metal site and Fe(VI), holding immense potential for deep wastewater purification.https://doi.org/10.1038/s41467-025-62930-4
spellingShingle Yundan Chen
Xiaofei Ge
Jun Li
Zishuai Bill Zhang
Zhenshan Li
Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
Nature Communications
title Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
title_full Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
title_fullStr Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
title_full_unstemmed Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
title_short Anchored atomic Ru-O4 architecture enables ultra-effective Fe(VI) activation via avoiding Fe(VI) self-decay for water purification
title_sort anchored atomic ru o4 architecture enables ultra effective fe vi activation via avoiding fe vi self decay for water purification
url https://doi.org/10.1038/s41467-025-62930-4
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AT xiaofeige anchoredatomicruo4architectureenablesultraeffectivefeviactivationviaavoidingfeviselfdecayforwaterpurification
AT junli anchoredatomicruo4architectureenablesultraeffectivefeviactivationviaavoidingfeviselfdecayforwaterpurification
AT zishuaibillzhang anchoredatomicruo4architectureenablesultraeffectivefeviactivationviaavoidingfeviselfdecayforwaterpurification
AT zhenshanli anchoredatomicruo4architectureenablesultraeffectivefeviactivationviaavoidingfeviselfdecayforwaterpurification