Direction‐Dependent Conduction Polarity in Altermagnetic CrSb

Abstract CrSb has recently gained immense attention as an altermagnetic candidate. This work reports on the experimental observation of direction‐dependent conduction polarity (DDCP) in altermagnetic CrSb through Hall and Seebeck thermopower measurements. Conduction is dominated by holes along the c...

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Main Authors: Banik Rai, Krishnendu Patra, Satyabrata Bera, Sk Kalimuddin, Kakan Deb, Mintu Mondal, Priya Mahadevan, Nitesh Kumar
Format: Article
Language:English
Published: Wiley 2025-07-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202502226
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author Banik Rai
Krishnendu Patra
Satyabrata Bera
Sk Kalimuddin
Kakan Deb
Mintu Mondal
Priya Mahadevan
Nitesh Kumar
author_facet Banik Rai
Krishnendu Patra
Satyabrata Bera
Sk Kalimuddin
Kakan Deb
Mintu Mondal
Priya Mahadevan
Nitesh Kumar
author_sort Banik Rai
collection DOAJ
description Abstract CrSb has recently gained immense attention as an altermagnetic candidate. This work reports on the experimental observation of direction‐dependent conduction polarity (DDCP) in altermagnetic CrSb through Hall and Seebeck thermopower measurements. Conduction is dominated by holes along the c‐axis and by electrons in the ab‐plane of the hexagonal crystal of CrSb. Density functional theory (DFT) calculations indicate that DDCP in CrSb arises from a multicarrier mechanism, where electrons and holes living in distinct bands dominate conduction along different crystallographic directions. Furthermore, DFT predicts that DDCP exists within a narrow energy window near the Fermi level and is sensitive to small doping levels. This prediction is experimentally validated by the loss of DDCP in hole‐doped Cr0.98V0.02Sb. These findings highlight the potential for tunable electronic behavior in CrSb, offering promising avenues for applications in devices that require both p‐type and n‐type functionalities within a single material.
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spelling doaj-art-83fbf10d2a7f4e47aed474bfd062229d2025-08-20T03:12:04ZengWileyAdvanced Science2198-38442025-07-011227n/an/a10.1002/advs.202502226Direction‐Dependent Conduction Polarity in Altermagnetic CrSbBanik Rai0Krishnendu Patra1Satyabrata Bera2Sk Kalimuddin3Kakan Deb4Mintu Mondal5Priya Mahadevan6Nitesh Kumar7Department of Condensed Matter and Materials Physics S. N. Bose National Centre for Basic Sciences Salt Lake City Kolkata 700106 IndiaDepartment of Condensed Matter and Materials Physics S. N. Bose National Centre for Basic Sciences Salt Lake City Kolkata 700106 IndiaSchool of Physical Sciences Indian Association for the Cultivation of Science Jadavpur Kolkata 700032 IndiaSchool of Physical Sciences Indian Association for the Cultivation of Science Jadavpur Kolkata 700032 IndiaDepartment of Condensed Matter and Materials Physics S. N. Bose National Centre for Basic Sciences Salt Lake City Kolkata 700106 IndiaSchool of Physical Sciences Indian Association for the Cultivation of Science Jadavpur Kolkata 700032 IndiaDepartment of Condensed Matter and Materials Physics S. N. Bose National Centre for Basic Sciences Salt Lake City Kolkata 700106 IndiaDepartment of Condensed Matter and Materials Physics S. N. Bose National Centre for Basic Sciences Salt Lake City Kolkata 700106 IndiaAbstract CrSb has recently gained immense attention as an altermagnetic candidate. This work reports on the experimental observation of direction‐dependent conduction polarity (DDCP) in altermagnetic CrSb through Hall and Seebeck thermopower measurements. Conduction is dominated by holes along the c‐axis and by electrons in the ab‐plane of the hexagonal crystal of CrSb. Density functional theory (DFT) calculations indicate that DDCP in CrSb arises from a multicarrier mechanism, where electrons and holes living in distinct bands dominate conduction along different crystallographic directions. Furthermore, DFT predicts that DDCP exists within a narrow energy window near the Fermi level and is sensitive to small doping levels. This prediction is experimentally validated by the loss of DDCP in hole‐doped Cr0.98V0.02Sb. These findings highlight the potential for tunable electronic behavior in CrSb, offering promising avenues for applications in devices that require both p‐type and n‐type functionalities within a single material.https://doi.org/10.1002/advs.202502226altermagnetdirection‐dependent conduction polarityelectrical transportFermi surface geometrySeebeck effect
spellingShingle Banik Rai
Krishnendu Patra
Satyabrata Bera
Sk Kalimuddin
Kakan Deb
Mintu Mondal
Priya Mahadevan
Nitesh Kumar
Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
Advanced Science
altermagnet
direction‐dependent conduction polarity
electrical transport
Fermi surface geometry
Seebeck effect
title Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
title_full Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
title_fullStr Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
title_full_unstemmed Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
title_short Direction‐Dependent Conduction Polarity in Altermagnetic CrSb
title_sort direction dependent conduction polarity in altermagnetic crsb
topic altermagnet
direction‐dependent conduction polarity
electrical transport
Fermi surface geometry
Seebeck effect
url https://doi.org/10.1002/advs.202502226
work_keys_str_mv AT banikrai directiondependentconductionpolarityinaltermagneticcrsb
AT krishnendupatra directiondependentconductionpolarityinaltermagneticcrsb
AT satyabratabera directiondependentconductionpolarityinaltermagneticcrsb
AT skkalimuddin directiondependentconductionpolarityinaltermagneticcrsb
AT kakandeb directiondependentconductionpolarityinaltermagneticcrsb
AT mintumondal directiondependentconductionpolarityinaltermagneticcrsb
AT priyamahadevan directiondependentconductionpolarityinaltermagneticcrsb
AT niteshkumar directiondependentconductionpolarityinaltermagneticcrsb