Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers

Biodegradable bioplastics provide a promising solution to mitigate environmental harm from petroleum-based plastics. This study focuses on optimizing bioplastic films made from oil palm trunk starch (OPTS), using glycerol (10, 20, and 30 % v/w) as a plasticizer and modified with citric-acid epoxidiz...

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Main Authors: Habib Hernando, Marpongahtun, Elisa Julianti, Arif Nuryawan, Suci Aisyah Amaturrahim, Averroes Fazlur Rahman Piliang, Muhammad Rafiq Yanhar, Ronn Goei, Nattakan Soykeabkaew, A. Muhammad Afdhal Saputra, Saharman Gea
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Case Studies in Chemical and Environmental Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666016424002330
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author Habib Hernando
Marpongahtun
Elisa Julianti
Arif Nuryawan
Suci Aisyah Amaturrahim
Averroes Fazlur Rahman Piliang
Muhammad Rafiq Yanhar
Ronn Goei
Nattakan Soykeabkaew
A. Muhammad Afdhal Saputra
Saharman Gea
author_facet Habib Hernando
Marpongahtun
Elisa Julianti
Arif Nuryawan
Suci Aisyah Amaturrahim
Averroes Fazlur Rahman Piliang
Muhammad Rafiq Yanhar
Ronn Goei
Nattakan Soykeabkaew
A. Muhammad Afdhal Saputra
Saharman Gea
author_sort Habib Hernando
collection DOAJ
description Biodegradable bioplastics provide a promising solution to mitigate environmental harm from petroleum-based plastics. This study focuses on optimizing bioplastic films made from oil palm trunk starch (OPTS), using glycerol (10, 20, and 30 % v/w) as a plasticizer and modified with citric-acid epoxidized palm oil (CEPO). The bioplastics were formed using the solution casting method and analyzed for morphology, functional groups, diffraction peaks, thermal and mechanical properties, degradation time, and compostability. The optimal conditions were achieved with 30 % glycerol (Sample ST-CEPO-GLY30). The addition of glycerol enhances the thermal and mechanical properties, improves the biodegradability, and compostability of the bioplastics.
format Article
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institution OA Journals
issn 2666-0164
language English
publishDate 2024-12-01
publisher Elsevier
record_format Article
series Case Studies in Chemical and Environmental Engineering
spelling doaj-art-82872f772dd84fa184647c2de49930fe2025-08-20T02:36:06ZengElsevierCase Studies in Chemical and Environmental Engineering2666-01642024-12-011010083910.1016/j.cscee.2024.100839Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomersHabib Hernando0 Marpongahtun1Elisa Julianti2Arif Nuryawan3Suci Aisyah Amaturrahim4Averroes Fazlur Rahman Piliang5Muhammad Rafiq Yanhar6Ronn Goei7Nattakan Soykeabkaew8A. Muhammad Afdhal Saputra9Saharman Gea10Postgraduate School, Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Jl. Bioteknologi No. 1 Medan, 20155, Indonesia; Cellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, IndonesiaCellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia; Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Jl. Bioteknologi No. 1, Medan, 20155, IndonesiaDepartment of Food and Science Technology, Faculty of Agriculture, Universitas Sumatera Utara, Padang Bulan, Medan, 20155, Sumatera Utara, IndonesiaDepartment of Forest Products Technology, Faculty of Forestry, Universitas Sumatera Utara, Jl. Tri Dharma Ujung No.1 Kampus USU Medan, 20155, North Sumatra, IndonesiaCellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia; Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Jl. Bioteknologi No. 1, Medan, 20155, IndonesiaCellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia; Department of Physics, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Medan, IndonesiaCellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia; Department of Mechanical Engineering, Faculty of Engineering, Universitas Sumatera Utara, Medan, IndonesiaSchool of Materials Science and Engineering, Nanyang Technological University, 50 Nanyang Avenue, 639798, SingaporeSchool of Science, Mae Fah Luang University, Thasud, Muang, Chiang Rai, 57100, ThailandPostgraduate School, Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Jl. Bioteknologi No. 1 Medan, 20155, Indonesia; Cellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, IndonesiaCellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia; Department of Chemistry, Faculty of Mathematics and Natural Sciences, Universitas Sumatera Utara, Jl. Bioteknologi No. 1, Medan, 20155, Indonesia; Corresponding author. Cellulosic and Functional Material Research Center, Universitas Sumatera Utara, Medan, Indonesia.Biodegradable bioplastics provide a promising solution to mitigate environmental harm from petroleum-based plastics. This study focuses on optimizing bioplastic films made from oil palm trunk starch (OPTS), using glycerol (10, 20, and 30 % v/w) as a plasticizer and modified with citric-acid epoxidized palm oil (CEPO). The bioplastics were formed using the solution casting method and analyzed for morphology, functional groups, diffraction peaks, thermal and mechanical properties, degradation time, and compostability. The optimal conditions were achieved with 30 % glycerol (Sample ST-CEPO-GLY30). The addition of glycerol enhances the thermal and mechanical properties, improves the biodegradability, and compostability of the bioplastics.http://www.sciencedirect.com/science/article/pii/S2666016424002330BioplasticCrosslinkingCitric-acidEpoxidized palm oilOil palm trunk starch
spellingShingle Habib Hernando
Marpongahtun
Elisa Julianti
Arif Nuryawan
Suci Aisyah Amaturrahim
Averroes Fazlur Rahman Piliang
Muhammad Rafiq Yanhar
Ronn Goei
Nattakan Soykeabkaew
A. Muhammad Afdhal Saputra
Saharman Gea
Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
Case Studies in Chemical and Environmental Engineering
Bioplastic
Crosslinking
Citric-acid
Epoxidized palm oil
Oil palm trunk starch
title Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
title_full Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
title_fullStr Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
title_full_unstemmed Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
title_short Impact of glycerol on oil palm trunk starch bioplastics enhanced with citric-acid epoxidized palm oil oligomers
title_sort impact of glycerol on oil palm trunk starch bioplastics enhanced with citric acid epoxidized palm oil oligomers
topic Bioplastic
Crosslinking
Citric-acid
Epoxidized palm oil
Oil palm trunk starch
url http://www.sciencedirect.com/science/article/pii/S2666016424002330
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