Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery

Layer spacing of vanadium oxide can be effectively expanded by metal ion, however, its conductivity and electrochemical kinetics still require improvement. This work expands the layer spacing using manganese ion and help to improve conductivity and electrochemical kinetics by graphene. The results d...

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Main Authors: Xiaowen Niu, Jianhai Chen, Yongtao Tan
Format: Article
Language:English
Published: Elsevier 2024-10-01
Series:Next Energy
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2949821X24000851
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author Xiaowen Niu
Jianhai Chen
Yongtao Tan
author_facet Xiaowen Niu
Jianhai Chen
Yongtao Tan
author_sort Xiaowen Niu
collection DOAJ
description Layer spacing of vanadium oxide can be effectively expanded by metal ion, however, its conductivity and electrochemical kinetics still require improvement. This work expands the layer spacing using manganese ion and help to improve conductivity and electrochemical kinetics by graphene. The results demonstrate that the layer spacing can be adjusted from 12.1 Å for pristine vanadium oxide (VOH) to 13.6 Å for manganese vanadium oxide (MnVO). Due to graphene introduction, it decreases to 11.6 Å for manganese vanadium oxide/graphene composite (MnVO-0.05–8/GN-15). Notably, the optimized composite delivers higher specific capacity of 507.5 mAh g−1 for MnVO-0.05–8/GN-15 than that of MnVO (410.4 mAh g−1) and VOH (370.1 mAh g−1) at current density of 0.5 A g−1. Furthermore, the MnVO-0.05–8/GN-15 exhibits fast Zn2+ ion diffusion ability, achieving high energy density of 403.51 Wh kg−1 and retaining an excellent cycle stability of 85.7% after 2000 cycles at a current density of 3 A g−1.
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spelling doaj-art-80a7a65d492f4b7eab9d18944a9e57cf2025-08-20T02:21:04ZengElsevierNext Energy2949-821X2024-10-01510018010.1016/j.nxener.2024.100180Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion batteryXiaowen Niu0Jianhai Chen1Yongtao Tan2Ningxia Key Laboratory of Photovoltaic Materials, School of Materials and New Energy, Ningxia University, Yinchuan, 750021, PR ChinaNingxia Key Laboratory of Photovoltaic Materials, School of Materials and New Energy, Ningxia University, Yinchuan, 750021, PR ChinaCorresponding author.; Ningxia Key Laboratory of Photovoltaic Materials, School of Materials and New Energy, Ningxia University, Yinchuan, 750021, PR ChinaLayer spacing of vanadium oxide can be effectively expanded by metal ion, however, its conductivity and electrochemical kinetics still require improvement. This work expands the layer spacing using manganese ion and help to improve conductivity and electrochemical kinetics by graphene. The results demonstrate that the layer spacing can be adjusted from 12.1 Å for pristine vanadium oxide (VOH) to 13.6 Å for manganese vanadium oxide (MnVO). Due to graphene introduction, it decreases to 11.6 Å for manganese vanadium oxide/graphene composite (MnVO-0.05–8/GN-15). Notably, the optimized composite delivers higher specific capacity of 507.5 mAh g−1 for MnVO-0.05–8/GN-15 than that of MnVO (410.4 mAh g−1) and VOH (370.1 mAh g−1) at current density of 0.5 A g−1. Furthermore, the MnVO-0.05–8/GN-15 exhibits fast Zn2+ ion diffusion ability, achieving high energy density of 403.51 Wh kg−1 and retaining an excellent cycle stability of 85.7% after 2000 cycles at a current density of 3 A g−1.http://www.sciencedirect.com/science/article/pii/S2949821X24000851GrapheneManganeseVanadium oxideZinc ion battery
spellingShingle Xiaowen Niu
Jianhai Chen
Yongtao Tan
Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
Next Energy
Graphene
Manganese
Vanadium oxide
Zinc ion battery
title Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
title_full Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
title_fullStr Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
title_full_unstemmed Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
title_short Graphene-assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc-ion battery
title_sort graphene assisted improve electrochemical performance of manganese vanadium oxide for aqueous zinc ion battery
topic Graphene
Manganese
Vanadium oxide
Zinc ion battery
url http://www.sciencedirect.com/science/article/pii/S2949821X24000851
work_keys_str_mv AT xiaowenniu grapheneassistedimproveelectrochemicalperformanceofmanganesevanadiumoxideforaqueouszincionbattery
AT jianhaichen grapheneassistedimproveelectrochemicalperformanceofmanganesevanadiumoxideforaqueouszincionbattery
AT yongtaotan grapheneassistedimproveelectrochemicalperformanceofmanganesevanadiumoxideforaqueouszincionbattery