Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure

The impact resistance of four polypropylene impact copolymers (ICPs) with multi-phase structures and widely differing characteristics was related to their structure. Blends were prepared from one of them and a high-density polyethylene (HDPE) to improve impact strength further. The structure of the...

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Main Authors: Milán Ferdinánd, Michael Jerabek, Róbert Várdai, Emese Pregi, Thomas Lummerstorfer, Markus Gahleitner, Gábor Faludi, János Móczó, Béla Pukánszky
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2024-04-01
Series:eXPRESS Polymer Letters
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Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0012842&mi=cd
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author Milán Ferdinánd
Michael Jerabek
Róbert Várdai
Emese Pregi
Thomas Lummerstorfer
Markus Gahleitner
Gábor Faludi
János Móczó
Béla Pukánszky
author_facet Milán Ferdinánd
Michael Jerabek
Róbert Várdai
Emese Pregi
Thomas Lummerstorfer
Markus Gahleitner
Gábor Faludi
János Móczó
Béla Pukánszky
author_sort Milán Ferdinánd
collection DOAJ
description The impact resistance of four polypropylene impact copolymers (ICPs) with multi-phase structures and widely differing characteristics was related to their structure. Blends were prepared from one of them and a high-density polyethylene (HDPE) to improve impact strength further. The structure of the materials was characterized by microscopy and dynamic mechanical thermal analysis. Mechanical properties were determined by tensile and impact testing, while local deformation processes were followed by volume strain measurements. The results obtained in the study proved that the shear-yielding of the matrix contributes the most among local processes to the increase of impact strength, while cavitation has a small effect on this latter property since its energy absorption is negligible. Both increasing elastomer content and decreasing particle size favor shear-yielding, thus improving impact strength. Considering the importance of elastomer content and elastomer particle size, a simple but very good model was created describing the dependence of the impact strength of ICPs on these latter two factors by using linear regression analysis. Although the addition of HDPE increases the fracture resistance of ICPs further, the extent of improvement is moderate, and the approach is economically disadvantageous.
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institution Kabale University
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publishDate 2024-04-01
publisher Budapest University of Technology and Economics
record_format Article
series eXPRESS Polymer Letters
spelling doaj-art-804c98fffa9e4be5a844514d2282c5532025-08-20T03:34:02ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2024-04-0118440641910.3144/expresspolymlett.2024.30Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structureMilán FerdinándMichael JerabekRóbert VárdaiEmese PregiThomas LummerstorferMarkus GahleitnerGábor FaludiJános MóczóBéla PukánszkyThe impact resistance of four polypropylene impact copolymers (ICPs) with multi-phase structures and widely differing characteristics was related to their structure. Blends were prepared from one of them and a high-density polyethylene (HDPE) to improve impact strength further. The structure of the materials was characterized by microscopy and dynamic mechanical thermal analysis. Mechanical properties were determined by tensile and impact testing, while local deformation processes were followed by volume strain measurements. The results obtained in the study proved that the shear-yielding of the matrix contributes the most among local processes to the increase of impact strength, while cavitation has a small effect on this latter property since its energy absorption is negligible. Both increasing elastomer content and decreasing particle size favor shear-yielding, thus improving impact strength. Considering the importance of elastomer content and elastomer particle size, a simple but very good model was created describing the dependence of the impact strength of ICPs on these latter two factors by using linear regression analysis. Although the addition of HDPE increases the fracture resistance of ICPs further, the extent of improvement is moderate, and the approach is economically disadvantageous.http://www.expresspolymlett.com/letolt.php?file=EPL-0012842&mi=cd injection moulding copolymers elastomer impact behaviour failure modeling
spellingShingle Milán Ferdinánd
Michael Jerabek
Róbert Várdai
Emese Pregi
Thomas Lummerstorfer
Markus Gahleitner
Gábor Faludi
János Móczó
Béla Pukánszky
Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
eXPRESS Polymer Letters
injection moulding
copolymers
elastomer
impact behaviour
failure modeling
title Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
title_full Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
title_fullStr Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
title_full_unstemmed Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
title_short Factors and processes determining the impact resistance of PP impact copolymers with multi-phase structure
title_sort factors and processes determining the impact resistance of pp impact copolymers with multi phase structure
topic injection moulding
copolymers
elastomer
impact behaviour
failure modeling
url http://www.expresspolymlett.com/letolt.php?file=EPL-0012842&mi=cd
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