Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation

The photocatalytic characteristics and CO2 decomposition capabilities of the TiO2:CuO heterojunction were examined using modelling and experimental methods. The simulation indicates that the TiO2:CuO heterostructure achieves a peak photocurrent density of 23.6 mA.cm-2 when the thickness of the TiO2...

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Main Authors: Thien Trinh Duc, Lam Nguyen
Format: Article
Language:English
Published: Iranian Chemical Society 2025-07-01
Series:Nanochemistry Research
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Online Access:http://www.nanochemres.org/article_220540_fa747565fa69ec03d14fc86f04dfadc8.pdf
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author Thien Trinh Duc
Lam Nguyen
author_facet Thien Trinh Duc
Lam Nguyen
author_sort Thien Trinh Duc
collection DOAJ
description The photocatalytic characteristics and CO2 decomposition capabilities of the TiO2:CuO heterojunction were examined using modelling and experimental methods. The simulation indicates that the TiO2:CuO heterostructure achieves a peak photocurrent density of 23.6 mA.cm-2 when the thickness of the TiO2 and CuO layer is 250 nm and 500 nm, respectively. The photocurrent density may vary by magnitude three times, from 8.3 mA.cm-2 when the CuO layer is first exposed to light, to 23.6 mA.cm-2 when the TiO2 layer is first exposed to light. The TiO2:CuO heterostructure was synthesized using the conventional hydrothermal method. The XRD investigation indicates the presence of two distinct phases, namely rutile TiO2 and monoclinic of CuO, in the structure. The FE-SEM images reveal a consistent structure size, with a distribution around 700 nm. The TiO2:CuO heterostructure has an enlarged absorption spectrum, reaching the wavelength of 800 nm. The evaluation of the CO2 decomposition was conducted by FTIR spectrum analysis. The presence of a distinct vibration peak at a wavelength of 1390 cm-1 in the FTIR spectrum provides that the study findings demonstrate the capacity to decompose CO2 into fuel using photocatalysis in a 1M NaOH solution.
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spelling doaj-art-7be0109245fe4c09b523b17fc611ed232025-08-20T02:50:08ZengIranian Chemical SocietyNanochemistry Research2538-42792423-818X2025-07-0110326927910.22036/ncr.2025.465846.1387220540Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and ExperimentationThien Trinh Duc0Lam Nguyen1Faculty of Physics, Hanoi National University of Education, Hanoi, VietnamFaculty of Engineering Physics and Nanotechnology, VNU-University of Engineering and Technology,The photocatalytic characteristics and CO2 decomposition capabilities of the TiO2:CuO heterojunction were examined using modelling and experimental methods. The simulation indicates that the TiO2:CuO heterostructure achieves a peak photocurrent density of 23.6 mA.cm-2 when the thickness of the TiO2 and CuO layer is 250 nm and 500 nm, respectively. The photocurrent density may vary by magnitude three times, from 8.3 mA.cm-2 when the CuO layer is first exposed to light, to 23.6 mA.cm-2 when the TiO2 layer is first exposed to light. The TiO2:CuO heterostructure was synthesized using the conventional hydrothermal method. The XRD investigation indicates the presence of two distinct phases, namely rutile TiO2 and monoclinic of CuO, in the structure. The FE-SEM images reveal a consistent structure size, with a distribution around 700 nm. The TiO2:CuO heterostructure has an enlarged absorption spectrum, reaching the wavelength of 800 nm. The evaluation of the CO2 decomposition was conducted by FTIR spectrum analysis. The presence of a distinct vibration peak at a wavelength of 1390 cm-1 in the FTIR spectrum provides that the study findings demonstrate the capacity to decompose CO2 into fuel using photocatalysis in a 1M NaOH solution.http://www.nanochemres.org/article_220540_fa747565fa69ec03d14fc86f04dfadc8.pdfheterojunctionhydrothermalphotocatalystco2 decompositionscaps-1d
spellingShingle Thien Trinh Duc
Lam Nguyen
Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
Nanochemistry Research
heterojunction
hydrothermal
photocatalyst
co2 decomposition
scaps-1d
title Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
title_full Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
title_fullStr Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
title_full_unstemmed Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
title_short Investigation of the CO2 Decomposition Capacity of the TiO2:CuO Heterojunction by Simulation and Experimentation
title_sort investigation of the co2 decomposition capacity of the tio2 cuo heterojunction by simulation and experimentation
topic heterojunction
hydrothermal
photocatalyst
co2 decomposition
scaps-1d
url http://www.nanochemres.org/article_220540_fa747565fa69ec03d14fc86f04dfadc8.pdf
work_keys_str_mv AT thientrinhduc investigationoftheco2decompositioncapacityofthetio2cuoheterojunctionbysimulationandexperimentation
AT lamnguyen investigationoftheco2decompositioncapacityofthetio2cuoheterojunctionbysimulationandexperimentation