Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation

We carried out MD simulations to review the mechanisms of clay damage under hydration, the manners clays interact with water and cations, and the structures they form in between aluminosilicate sheets and offered an alternative explanation as to how clay structures become instable after certain wate...

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Main Authors: Luchao Jin, Ahmad Jamili, Liangliang Huang, Felipe Perez
Format: Article
Language:English
Published: Wiley 2017-01-01
Series:Geofluids
Online Access:http://dx.doi.org/10.1155/2017/1747068
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author Luchao Jin
Ahmad Jamili
Liangliang Huang
Felipe Perez
author_facet Luchao Jin
Ahmad Jamili
Liangliang Huang
Felipe Perez
author_sort Luchao Jin
collection DOAJ
description We carried out MD simulations to review the mechanisms of clay damage under hydration, the manners clays interact with water and cations, and the structures they form in between aluminosilicate sheets and offered an alternative explanation as to how clay structures become instable after certain water concentration. Water molecules form one, two, and sometimes three layers parallel to the clay surfaces. The cations already present in montmorillonites (the most representative of the smectites) or coming with low salinity water will either be adsorbed by the clay surfaces or become fully hydrated, detached from the surfaces, and located in the midst of the interlayer space between clay surfaces, while water molecules that do not hydrate the cations invade the clay structures, making them unstable. The driving force of this phenomenon happens to be the hydration energy of the cations in question.
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institution OA Journals
issn 1468-8115
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language English
publishDate 2017-01-01
publisher Wiley
record_format Article
series Geofluids
spelling doaj-art-7a4d60122ebd4b3ca16c1cde65a2dfd52025-08-20T02:07:37ZengWileyGeofluids1468-81151468-81232017-01-01201710.1155/2017/17470681747068Modeling the Mechanisms of Clay Damage by Molecular Dynamic SimulationLuchao Jin0Ahmad Jamili1Liangliang Huang2Felipe Perez3Mewbourne School of Petroleum and Geological Engineering, The University of Oklahoma, Norman, OK, USAMewbourne School of Petroleum and Geological Engineering, The University of Oklahoma, Norman, OK, USAGallogly College of Engineering, Chemical, Biological and Materials Engineering, The University of Oklahoma, Norman, OK, USAMewbourne School of Petroleum and Geological Engineering, The University of Oklahoma, Norman, OK, USAWe carried out MD simulations to review the mechanisms of clay damage under hydration, the manners clays interact with water and cations, and the structures they form in between aluminosilicate sheets and offered an alternative explanation as to how clay structures become instable after certain water concentration. Water molecules form one, two, and sometimes three layers parallel to the clay surfaces. The cations already present in montmorillonites (the most representative of the smectites) or coming with low salinity water will either be adsorbed by the clay surfaces or become fully hydrated, detached from the surfaces, and located in the midst of the interlayer space between clay surfaces, while water molecules that do not hydrate the cations invade the clay structures, making them unstable. The driving force of this phenomenon happens to be the hydration energy of the cations in question.http://dx.doi.org/10.1155/2017/1747068
spellingShingle Luchao Jin
Ahmad Jamili
Liangliang Huang
Felipe Perez
Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
Geofluids
title Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
title_full Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
title_fullStr Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
title_full_unstemmed Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
title_short Modeling the Mechanisms of Clay Damage by Molecular Dynamic Simulation
title_sort modeling the mechanisms of clay damage by molecular dynamic simulation
url http://dx.doi.org/10.1155/2017/1747068
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AT ahmadjamili modelingthemechanismsofclaydamagebymoleculardynamicsimulation
AT lianglianghuang modelingthemechanismsofclaydamagebymoleculardynamicsimulation
AT felipeperez modelingthemechanismsofclaydamagebymoleculardynamicsimulation