Connection between f-electron correlations and magnetic excitations in UTe2

Abstract The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe2 is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry Y and T points...

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Main Authors: Thomas Halloran, Peter Czajka, Gicela Saucedo Salas, Corey E. Frank, Chang-Jong Kang, J. A. Rodriguez-Rivera, Jakob Lass, Daniel G. Mazzone, Marc Janoschek, Gabriel Kotliar, Nicholas P. Butch
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:npj Quantum Materials
Online Access:https://doi.org/10.1038/s41535-024-00720-9
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author Thomas Halloran
Peter Czajka
Gicela Saucedo Salas
Corey E. Frank
Chang-Jong Kang
J. A. Rodriguez-Rivera
Jakob Lass
Daniel G. Mazzone
Marc Janoschek
Gabriel Kotliar
Nicholas P. Butch
author_facet Thomas Halloran
Peter Czajka
Gicela Saucedo Salas
Corey E. Frank
Chang-Jong Kang
J. A. Rodriguez-Rivera
Jakob Lass
Daniel G. Mazzone
Marc Janoschek
Gabriel Kotliar
Nicholas P. Butch
author_sort Thomas Halloran
collection DOAJ
description Abstract The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe2 is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry Y and T points and disperse along the crystallographic $$\hat{b}$$ b ̂ -axis. In applied magnetic fields to at least μ 0 H = 11 T along the $$\hat{c}-{\rm{axis}}$$ c ̂ − axis , the magnetism is found to be field-independent in the (h k0) plane. The scattering intensity is consistent with that expected from U3+/U4+  f-electron spins with preferential orientation along the crystallographic $$\hat{a}$$ a ̂ -axis, and a fluctuating magnetic moment of μ e f f =1.7(5) μ B . We propose interband spin excitons arising from f-electron hybridization as a possible origin of the magnetic excitations in UTe2.
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institution Kabale University
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series npj Quantum Materials
spelling doaj-art-76e2d82774c4465cb67e2323ca8644362025-01-05T12:07:50ZengNature Portfolionpj Quantum Materials2397-46482025-01-011011810.1038/s41535-024-00720-9Connection between f-electron correlations and magnetic excitations in UTe2Thomas Halloran0Peter Czajka1Gicela Saucedo Salas2Corey E. Frank3Chang-Jong Kang4J. A. Rodriguez-Rivera5Jakob Lass6Daniel G. Mazzone7Marc Janoschek8Gabriel Kotliar9Nicholas P. Butch10NIST Center for Neutron ResearchNIST Center for Neutron ResearchNIST Center for Neutron ResearchNIST Center for Neutron ResearchDepartment of Physics, Chungnam National UniversityNIST Center for Neutron ResearchLaboratory for Neutron Scattering and Imaging, Paul Scherrer InstituteLaboratory for Neutron Scattering and Imaging, Paul Scherrer InstituteLaboratory for Neutron and Muon Instrumentation, PSI Center for Neutron and Muon Sciences, Paul Scherrer InstituteDepartment of Physics and Astronomy, Rutgers UniversityNIST Center for Neutron ResearchAbstract The detailed anisotropic dispersion of the low-temperature, low-energy magnetic excitations of the candidate spin-triplet superconductor UTe2 is revealed using inelastic neutron scattering. The magnetic excitations emerge from the Brillouin zone boundary at the high symmetry Y and T points and disperse along the crystallographic $$\hat{b}$$ b ̂ -axis. In applied magnetic fields to at least μ 0 H = 11 T along the $$\hat{c}-{\rm{axis}}$$ c ̂ − axis , the magnetism is found to be field-independent in the (h k0) plane. The scattering intensity is consistent with that expected from U3+/U4+  f-electron spins with preferential orientation along the crystallographic $$\hat{a}$$ a ̂ -axis, and a fluctuating magnetic moment of μ e f f =1.7(5) μ B . We propose interband spin excitons arising from f-electron hybridization as a possible origin of the magnetic excitations in UTe2.https://doi.org/10.1038/s41535-024-00720-9
spellingShingle Thomas Halloran
Peter Czajka
Gicela Saucedo Salas
Corey E. Frank
Chang-Jong Kang
J. A. Rodriguez-Rivera
Jakob Lass
Daniel G. Mazzone
Marc Janoschek
Gabriel Kotliar
Nicholas P. Butch
Connection between f-electron correlations and magnetic excitations in UTe2
npj Quantum Materials
title Connection between f-electron correlations and magnetic excitations in UTe2
title_full Connection between f-electron correlations and magnetic excitations in UTe2
title_fullStr Connection between f-electron correlations and magnetic excitations in UTe2
title_full_unstemmed Connection between f-electron correlations and magnetic excitations in UTe2
title_short Connection between f-electron correlations and magnetic excitations in UTe2
title_sort connection between f electron correlations and magnetic excitations in ute2
url https://doi.org/10.1038/s41535-024-00720-9
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