Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K

To get a deep insight into the interactions between water (W) and acetonitrile (ACN), and to provide new data, three types of physical properties such as volumetric, transport, and acoustic properties of their binary solutions at different compositions in the whole range of concentration and at six...

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Main Authors: Sharmin Sultana, Md. Niamat Ullah, Syeda Khurshida Begum
Format: Article
Language:English
Published: Elsevier 2025-06-01
Series:Chemical Physics Impact
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Online Access:http://www.sciencedirect.com/science/article/pii/S266702242500043X
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author Sharmin Sultana
Md. Niamat Ullah
Syeda Khurshida Begum
author_facet Sharmin Sultana
Md. Niamat Ullah
Syeda Khurshida Begum
author_sort Sharmin Sultana
collection DOAJ
description To get a deep insight into the interactions between water (W) and acetonitrile (ACN), and to provide new data, three types of physical properties such as volumetric, transport, and acoustic properties of their binary solutions at different compositions in the whole range of concentration and at six different temperatures (298.15 K, 303.15 K, 308.15 K, 313.15 K, 318.15 K, and 323.15 K) at 0.1 MPa atmospheric pressure have been studied. Here, densities (ρ), viscosities (ƞ), and speeds of sound (u) were measured experimentally, and using these data some other important properties such as excess molar volumes, VmE, apparent molar volumes, Φv, thermal expansibilities, α, excess thermal expansibilities, αE, excess viscosities, ηE, relaxation times, τ, deviation in speeds of sound, ∆u, acoustic impedances, Z, deviation in acoustic impedances, ∆Z, Rao's constants, R, free volumes, Vf, and excess free volumes, VfE, were calculated. The experimental and their derived properties were fitted to appropriate polynomial equations. Analysis of the results indicates a significant interstitial accommodation of free molecules of one component into the structural network of the other, mainly at the water-rich region in the water - acetonitrile system.
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spelling doaj-art-76e069e6c5fb485d83e40f49eece50c52025-08-20T03:20:05ZengElsevierChemical Physics Impact2667-02242025-06-011010085510.1016/j.chphi.2025.100855Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15KSharmin Sultana0Md. Niamat Ullah1Syeda Khurshida Begum2Department of Chemistry, University of Chittagong, Hathazari, Chittagong 4331, BangladeshDepartment of Chemistry, University of Chittagong, Hathazari, Chittagong 4331, BangladeshCorresponding author.; Department of Chemistry, University of Chittagong, Hathazari, Chittagong 4331, BangladeshTo get a deep insight into the interactions between water (W) and acetonitrile (ACN), and to provide new data, three types of physical properties such as volumetric, transport, and acoustic properties of their binary solutions at different compositions in the whole range of concentration and at six different temperatures (298.15 K, 303.15 K, 308.15 K, 313.15 K, 318.15 K, and 323.15 K) at 0.1 MPa atmospheric pressure have been studied. Here, densities (ρ), viscosities (ƞ), and speeds of sound (u) were measured experimentally, and using these data some other important properties such as excess molar volumes, VmE, apparent molar volumes, Φv, thermal expansibilities, α, excess thermal expansibilities, αE, excess viscosities, ηE, relaxation times, τ, deviation in speeds of sound, ∆u, acoustic impedances, Z, deviation in acoustic impedances, ∆Z, Rao's constants, R, free volumes, Vf, and excess free volumes, VfE, were calculated. The experimental and their derived properties were fitted to appropriate polynomial equations. Analysis of the results indicates a significant interstitial accommodation of free molecules of one component into the structural network of the other, mainly at the water-rich region in the water - acetonitrile system.http://www.sciencedirect.com/science/article/pii/S266702242500043XBinary solutionsWaterAcetonitrileVolumetricAcousticInteractions
spellingShingle Sharmin Sultana
Md. Niamat Ullah
Syeda Khurshida Begum
Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
Chemical Physics Impact
Binary solutions
Water
Acetonitrile
Volumetric
Acoustic
Interactions
title Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
title_full Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
title_fullStr Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
title_full_unstemmed Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
title_short Volumetric and acoustic properties of binary solutions of water and acetonitrile at 298.15K, 303.15K, 308.15K, 313.15K, 318.15K, and 323.15K
title_sort volumetric and acoustic properties of binary solutions of water and acetonitrile at 298 15k 303 15k 308 15k 313 15k 318 15k and 323 15k
topic Binary solutions
Water
Acetonitrile
Volumetric
Acoustic
Interactions
url http://www.sciencedirect.com/science/article/pii/S266702242500043X
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