Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet

Abstract Synthetic antiferromagnetics (SAF) provide an excellent platform for antiferromagnetic spintronics. Recently, the voltage-control of the Ruderman–Kittel–Kasuya–Yosida (RKKY) interaction in SAFs was studied experimentally. Optical control would offer unique opportunities for the ultrafast ma...

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Main Authors: Meiyang Ma, Jing Wu, Bo Liu, Lei Wang, Zhuoyi Li, Xuezhong Ruan, Zehua Hu, Fengqiu Wang, Xianyang Lu, Tianyu Liu, Jun Du, Ke Xia, Yongbing Xu
Format: Article
Language:English
Published: Nature Portfolio 2025-05-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-59689-z
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author Meiyang Ma
Jing Wu
Bo Liu
Lei Wang
Zhuoyi Li
Xuezhong Ruan
Zehua Hu
Fengqiu Wang
Xianyang Lu
Tianyu Liu
Jun Du
Ke Xia
Yongbing Xu
author_facet Meiyang Ma
Jing Wu
Bo Liu
Lei Wang
Zhuoyi Li
Xuezhong Ruan
Zehua Hu
Fengqiu Wang
Xianyang Lu
Tianyu Liu
Jun Du
Ke Xia
Yongbing Xu
author_sort Meiyang Ma
collection DOAJ
description Abstract Synthetic antiferromagnetics (SAF) provide an excellent platform for antiferromagnetic spintronics. Recently, the voltage-control of the Ruderman–Kittel–Kasuya–Yosida (RKKY) interaction in SAFs was studied experimentally. Optical control would offer unique opportunities for the ultrafast manipulation of spin states, however, it has yet to be demonstrated. Here, using femtosecond laser excitations in a [Co/Pt]-based perpendicular magnetic anisotropy (PMA) synthetic antiferromagnet (p-SAF), we drive a reduction of the RKKY coupling and the PMA. We attribute the reduced RKKY interaction to the optically smeared Fermi wave vector of the Ru layer, which mediates the exchange coupling between the constituent ferromagnetic layers. The PMA exhibits the same amplitude of decrease as the RKKY coupling, which we associate with electron redistributions in the 3d orbitals caused by the optically smeared Fermi level. While the pump excitation process is shown to have an influence on the modulations, thermal contributions are excluded. Our study establishes a link between the RKKY coupling and the PMA in a p-SAF structure and provides an approach to tune them in parallel.
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spelling doaj-art-76df72e6bb5b4785b111f23d63d1109d2025-08-20T03:07:56ZengNature PortfolioNature Communications2041-17232025-05-011611810.1038/s41467-025-59689-zOptical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnetMeiyang Ma0Jing Wu1Bo Liu2Lei Wang3Zhuoyi Li4Xuezhong Ruan5Zehua Hu6Fengqiu Wang7Xianyang Lu8Tianyu Liu9Jun Du10Ke Xia11Yongbing Xu12National Key Laboratory of Spintronics, Nanjing UniversitySchool of Integrated Circuits, Guangdong University of TechnologyNational Key Laboratory of Spintronics, Nanjing UniversityKey Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics, Southeast UniversityNational Key Laboratory of Spintronics, Nanjing UniversityNational Key Laboratory of Spintronics, Nanjing UniversitySchool of Electronic Science and Engineering, Nanjing UniversitySchool of Electronic Science and Engineering, Nanjing UniversityNational Key Laboratory of Spintronics, Nanjing UniversityDepartment of Physics, Nanjing UniversityDepartment of Physics, Nanjing UniversityKey Laboratory of Quantum Materials and Devices of Ministry of Education, School of Physics, Southeast UniversityNational Key Laboratory of Spintronics, Nanjing UniversityAbstract Synthetic antiferromagnetics (SAF) provide an excellent platform for antiferromagnetic spintronics. Recently, the voltage-control of the Ruderman–Kittel–Kasuya–Yosida (RKKY) interaction in SAFs was studied experimentally. Optical control would offer unique opportunities for the ultrafast manipulation of spin states, however, it has yet to be demonstrated. Here, using femtosecond laser excitations in a [Co/Pt]-based perpendicular magnetic anisotropy (PMA) synthetic antiferromagnet (p-SAF), we drive a reduction of the RKKY coupling and the PMA. We attribute the reduced RKKY interaction to the optically smeared Fermi wave vector of the Ru layer, which mediates the exchange coupling between the constituent ferromagnetic layers. The PMA exhibits the same amplitude of decrease as the RKKY coupling, which we associate with electron redistributions in the 3d orbitals caused by the optically smeared Fermi level. While the pump excitation process is shown to have an influence on the modulations, thermal contributions are excluded. Our study establishes a link between the RKKY coupling and the PMA in a p-SAF structure and provides an approach to tune them in parallel.https://doi.org/10.1038/s41467-025-59689-z
spellingShingle Meiyang Ma
Jing Wu
Bo Liu
Lei Wang
Zhuoyi Li
Xuezhong Ruan
Zehua Hu
Fengqiu Wang
Xianyang Lu
Tianyu Liu
Jun Du
Ke Xia
Yongbing Xu
Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
Nature Communications
title Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
title_full Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
title_fullStr Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
title_full_unstemmed Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
title_short Optical control of RKKY coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
title_sort optical control of rkky coupling and perpendicular magnetic anisotropy in a synthetic antiferromagnet
url https://doi.org/10.1038/s41467-025-59689-z
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