Copper(II) Complexes of Organophoshonic Acids-A Comparative Study

Polynuclear copper(II) derivatives of 1-hydroxyethylidenediphosphonic acid (HEDP), 1-aminoethylidenediphosphonic acid (AEDP, H4L), α-aminobenzylidene diphosphonic acid (ABDP, H4L), 1-amino-2-carboxyethane- 1,1-diphosphonic acid (ACEDP, H5L), 1,3 diaminopropane-1,1,3,3-tetra-phosphonic acid (DAPTP,...

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Main Authors: B. Venkateswara Rao, D. M. Puri
Format: Article
Language:English
Published: Wiley 2011-01-01
Series:E-Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2011/813586
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author B. Venkateswara Rao
D. M. Puri
author_facet B. Venkateswara Rao
D. M. Puri
author_sort B. Venkateswara Rao
collection DOAJ
description Polynuclear copper(II) derivatives of 1-hydroxyethylidenediphosphonic acid (HEDP), 1-aminoethylidenediphosphonic acid (AEDP, H4L), α-aminobenzylidene diphosphonic acid (ABDP, H4L), 1-amino-2-carboxyethane- 1,1-diphosphonic acid (ACEDP, H5L), 1,3 diaminopropane-1,1,3,3-tetra-phosphonic acid (DAPTP, H8L), Ethylenediamine-N,N'-bis (dimethyl-methylenephosphonic) acid (EDBDMPO, H4L), o-phenylene-diamine-N,N'-bis (dimethylmethylenephosphonic) acid (PDBDMPO, H4L), diethylene triamine –N,N,N',N',N"N-penta (methylene phosphonic) acid (DETAPMPO, H10L) and diethylene triamine –N,N"-bis (dimethyl methylene phosphonic) acid (DETBDMPO, H4L) have been prepared in aqueous medium. The general formula of derivatives from elemental analysis was found to be Cu2L.XH2O (in case of AEDP, ABDP, EDBDMPO, PDBDMPO, DETBDMPO), Cu5L2.XH2O (in case of ACEDP) Cu4L.XH2O, Cu2 H4L. XH2O (in case of DAPTP) and Cu5L.XH2O (in case of DETAPMPO). The electronic spectra have shown them to be six coordinated with slight distortion from octahedral geometry. Antiferromagnetism was inferred from magnetic moment data. Infrared spectral studies were carried out to determine coordination sites. EPR (Electron Paramagnetic Resonance) spectra that supports the presence of tetragonal distortion and antiferromagnetic behaviour, have also been studied.
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spelling doaj-art-76d02f756ead42e7bd02bc02220862582025-08-20T03:35:15ZengWileyE-Journal of Chemistry0973-49452090-98102011-01-018S1S271S28110.1155/2011/813586Copper(II) Complexes of Organophoshonic Acids-A Comparative StudyB. Venkateswara Rao0D. M. Puri1Department of Chemistry, Andhra Loyola College (Autonomous), Vijayawada, Andhra Pradesh, IndiaDepartment of Chemistry, Kurukshetra University, Kurukshetra, 132119, IndiaPolynuclear copper(II) derivatives of 1-hydroxyethylidenediphosphonic acid (HEDP), 1-aminoethylidenediphosphonic acid (AEDP, H4L), α-aminobenzylidene diphosphonic acid (ABDP, H4L), 1-amino-2-carboxyethane- 1,1-diphosphonic acid (ACEDP, H5L), 1,3 diaminopropane-1,1,3,3-tetra-phosphonic acid (DAPTP, H8L), Ethylenediamine-N,N'-bis (dimethyl-methylenephosphonic) acid (EDBDMPO, H4L), o-phenylene-diamine-N,N'-bis (dimethylmethylenephosphonic) acid (PDBDMPO, H4L), diethylene triamine –N,N,N',N',N"N-penta (methylene phosphonic) acid (DETAPMPO, H10L) and diethylene triamine –N,N"-bis (dimethyl methylene phosphonic) acid (DETBDMPO, H4L) have been prepared in aqueous medium. The general formula of derivatives from elemental analysis was found to be Cu2L.XH2O (in case of AEDP, ABDP, EDBDMPO, PDBDMPO, DETBDMPO), Cu5L2.XH2O (in case of ACEDP) Cu4L.XH2O, Cu2 H4L. XH2O (in case of DAPTP) and Cu5L.XH2O (in case of DETAPMPO). The electronic spectra have shown them to be six coordinated with slight distortion from octahedral geometry. Antiferromagnetism was inferred from magnetic moment data. Infrared spectral studies were carried out to determine coordination sites. EPR (Electron Paramagnetic Resonance) spectra that supports the presence of tetragonal distortion and antiferromagnetic behaviour, have also been studied.http://dx.doi.org/10.1155/2011/813586
spellingShingle B. Venkateswara Rao
D. M. Puri
Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
E-Journal of Chemistry
title Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
title_full Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
title_fullStr Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
title_full_unstemmed Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
title_short Copper(II) Complexes of Organophoshonic Acids-A Comparative Study
title_sort copper ii complexes of organophoshonic acids a comparative study
url http://dx.doi.org/10.1155/2011/813586
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