Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc

Four machine learning (ML) models including eXtreme Gradient boosting (XGBT), k-Nearest Neighbor (kNN), Gradient Boosting Decision Tree (GBDT) and Artificial Neural Network (ANN) were employed to predict saturation flux density (Bs), coercivity (Hc), grain size, magnetostriction (λ), and Curie tempe...

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Main Authors: Shengdong Tang, Rui Sun, Yifan He, Guichang Liu, Ruixuan Wang, Yuqin Liu, Chengying Tang
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Materials & Design
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Online Access:http://www.sciencedirect.com/science/article/pii/S0264127524008360
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author Shengdong Tang
Rui Sun
Yifan He
Guichang Liu
Ruixuan Wang
Yuqin Liu
Chengying Tang
author_facet Shengdong Tang
Rui Sun
Yifan He
Guichang Liu
Ruixuan Wang
Yuqin Liu
Chengying Tang
author_sort Shengdong Tang
collection DOAJ
description Four machine learning (ML) models including eXtreme Gradient boosting (XGBT), k-Nearest Neighbor (kNN), Gradient Boosting Decision Tree (GBDT) and Artificial Neural Network (ANN) were employed to predict saturation flux density (Bs), coercivity (Hc), grain size, magnetostriction (λ), and Curie temperature (Tc) of Fe-based amorphous/nanocrystalline alloys. To maximize predictive ability of ML models, grid-search and normalization were used to search the most proper parameters of ML and pre-process raw data, respectively. XGBT had best predictive and generalization ability for predicting Bs and Hc with coefficient of determination (R2) of 0.992 and 0.967, respectively. Based on the feature importance analysis from the XGBT model, the Fe85Si2B8.5P3.5C1 amorphous alloy ribbon with good magnetic properties, such as high Bs, low Hc, was designed and prepared by melt spinning. X-ray diffraction (XRD), differential scanning calorimetry (DSC), transmission electron microscopy (TEM), vibrating sample magnetometer (VSM), B–H loop tracer, and magnetostriction instrument were used to identify the phase structure and physical properties of the Fe85Si2B8.5P3.5C1 alloy. It was found that the Fe85Si2B8.5P3.5C1 alloy had good magnetic properties with Bs of 1.82 T and the Hc of 2.02 A/m after annealing at 723 K for 180 s, in good agreement with the designed results by machine learning.
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spelling doaj-art-768d05fc5c3a4dd084e7cd7c4dccf0752025-08-20T01:57:00ZengElsevierMaterials & Design0264-12752024-12-0124811346110.1016/j.matdes.2024.113461Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low HcShengdong Tang0Rui Sun1Yifan He2Guichang Liu3Ruixuan Wang4Yuqin Liu5Chengying Tang6Engineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing 100083, PR ChinaGuangxi Key Laboratory for Informational Materials & School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin, Guangxi 541004, PR ChinaGuangxi Key Laboratory for Informational Materials & School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin, Guangxi 541004, PR ChinaEngineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing 100083, PR ChinaEngineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing 100083, PR ChinaEngineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources, School of Materials Science and Technology, China University of Geosciences (Beijing), Beijing 100083, PR China; Corresponding authors.Guangxi Key Laboratory for Informational Materials & School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin, Guangxi 541004, PR China; Corresponding authors.Four machine learning (ML) models including eXtreme Gradient boosting (XGBT), k-Nearest Neighbor (kNN), Gradient Boosting Decision Tree (GBDT) and Artificial Neural Network (ANN) were employed to predict saturation flux density (Bs), coercivity (Hc), grain size, magnetostriction (λ), and Curie temperature (Tc) of Fe-based amorphous/nanocrystalline alloys. To maximize predictive ability of ML models, grid-search and normalization were used to search the most proper parameters of ML and pre-process raw data, respectively. XGBT had best predictive and generalization ability for predicting Bs and Hc with coefficient of determination (R2) of 0.992 and 0.967, respectively. Based on the feature importance analysis from the XGBT model, the Fe85Si2B8.5P3.5C1 amorphous alloy ribbon with good magnetic properties, such as high Bs, low Hc, was designed and prepared by melt spinning. X-ray diffraction (XRD), differential scanning calorimetry (DSC), transmission electron microscopy (TEM), vibrating sample magnetometer (VSM), B–H loop tracer, and magnetostriction instrument were used to identify the phase structure and physical properties of the Fe85Si2B8.5P3.5C1 alloy. It was found that the Fe85Si2B8.5P3.5C1 alloy had good magnetic properties with Bs of 1.82 T and the Hc of 2.02 A/m after annealing at 723 K for 180 s, in good agreement with the designed results by machine learning.http://www.sciencedirect.com/science/article/pii/S0264127524008360Machine learningGrid-search methodMagnetic propertiesFe-based amorphous alloysFe-based nanocrystalline alloys
spellingShingle Shengdong Tang
Rui Sun
Yifan He
Guichang Liu
Ruixuan Wang
Yuqin Liu
Chengying Tang
Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
Materials & Design
Machine learning
Grid-search method
Magnetic properties
Fe-based amorphous alloys
Fe-based nanocrystalline alloys
title Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
title_full Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
title_fullStr Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
title_full_unstemmed Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
title_short Machine learning assisted design and preparation of Fe85Si2B8.5P3.5C1 amorphous/nanocrystalline alloy with high Bs and low Hc
title_sort machine learning assisted design and preparation of fe85si2b8 5p3 5c1 amorphous nanocrystalline alloy with high bs and low hc
topic Machine learning
Grid-search method
Magnetic properties
Fe-based amorphous alloys
Fe-based nanocrystalline alloys
url http://www.sciencedirect.com/science/article/pii/S0264127524008360
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