Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties

Abstract A new type of lubricating material (BTA-P4444-Lig) was synthesized by combining lignin with tetrabutylphosphorus and benzotriazole. The tribological properties, corrosion resistance, and anti-oxidation properties of BTA-P4444-Lig as a lubricant were investigated. The lubricating material ex...

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Main Authors: Chaoyang Zhang, Zhiquan Yang, Qing Huang, Xingwei Wang, Wufang Yang, Chunyu Zhou, Bo Yu, Qiangliang Yu, Meirong Cai, Feng Zhou
Format: Article
Language:English
Published: Tsinghua University Press 2022-07-01
Series:Friction
Subjects:
Online Access:https://doi.org/10.1007/s40544-022-0657-y
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author Chaoyang Zhang
Zhiquan Yang
Qing Huang
Xingwei Wang
Wufang Yang
Chunyu Zhou
Bo Yu
Qiangliang Yu
Meirong Cai
Feng Zhou
author_facet Chaoyang Zhang
Zhiquan Yang
Qing Huang
Xingwei Wang
Wufang Yang
Chunyu Zhou
Bo Yu
Qiangliang Yu
Meirong Cai
Feng Zhou
author_sort Chaoyang Zhang
collection DOAJ
description Abstract A new type of lubricating material (BTA-P4444-Lig) was synthesized by combining lignin with tetrabutylphosphorus and benzotriazole. The tribological properties, corrosion resistance, and anti-oxidation properties of BTA-P4444-Lig as a lubricant were investigated. The lubricating material exhibits excellent friction reduction and wear resistance, as well as good thermal stability and excellent oxidation resistance. Mechanistic analysis reveals that the active elements N and P in the lubricating material react with the metal substrate, and the reaction film effectively blocks direct contact between the friction pairs, affording excellent friction reduction and wear resistance. At the same time, the phenolic hydroxyl group in lignin reacts with oxygen free radicals to form a resonance-stable semi-quinone free radical, which interrupts the chain reaction and affords good anti-oxidant activity.
format Article
id doaj-art-765a46d894b14705979c68607d2c7101
institution DOAJ
issn 2223-7690
2223-7704
language English
publishDate 2022-07-01
publisher Tsinghua University Press
record_format Article
series Friction
spelling doaj-art-765a46d894b14705979c68607d2c71012025-08-20T03:19:11ZengTsinghua University PressFriction2223-76902223-77042022-07-011171239125210.1007/s40544-022-0657-yLignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological propertiesChaoyang Zhang0Zhiquan Yang1Qing Huang2Xingwei Wang3Wufang Yang4Chunyu Zhou5Bo Yu6Qiangliang Yu7Meirong Cai8Feng Zhou9State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesPetroChina Lanzhou Lubricating Oil R&D InstituteShandong Laboratory of Yantai Advanced Materials and Green ManufacturingState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesYantai Zhongke Research Institute of Advanced Materials and Green Chemical EngineeringState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesState Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Chinese Academy of SciencesAbstract A new type of lubricating material (BTA-P4444-Lig) was synthesized by combining lignin with tetrabutylphosphorus and benzotriazole. The tribological properties, corrosion resistance, and anti-oxidation properties of BTA-P4444-Lig as a lubricant were investigated. The lubricating material exhibits excellent friction reduction and wear resistance, as well as good thermal stability and excellent oxidation resistance. Mechanistic analysis reveals that the active elements N and P in the lubricating material react with the metal substrate, and the reaction film effectively blocks direct contact between the friction pairs, affording excellent friction reduction and wear resistance. At the same time, the phenolic hydroxyl group in lignin reacts with oxygen free radicals to form a resonance-stable semi-quinone free radical, which interrupts the chain reaction and affords good anti-oxidant activity.https://doi.org/10.1007/s40544-022-0657-yligninlubricationionic liquidanti-oxidant
spellingShingle Chaoyang Zhang
Zhiquan Yang
Qing Huang
Xingwei Wang
Wufang Yang
Chunyu Zhou
Bo Yu
Qiangliang Yu
Meirong Cai
Feng Zhou
Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
Friction
lignin
lubrication
ionic liquid
anti-oxidant
title Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
title_full Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
title_fullStr Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
title_full_unstemmed Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
title_short Lignin composite ionic liquid lubricants with excellent anti-corrosion, anti-oxidation, and tribological properties
title_sort lignin composite ionic liquid lubricants with excellent anti corrosion anti oxidation and tribological properties
topic lignin
lubrication
ionic liquid
anti-oxidant
url https://doi.org/10.1007/s40544-022-0657-y
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