Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites

This study investigated the effect of polyethylene glycol (PEG) and nanosilica (NS) on the physical-mechanical properties and cure kinetics of diglycidyl ether of bisphenol-A-based epoxy (DGEBA-based EP) resin. For this purpose, tensile and viscometry tests, dynamic mechanical thermal analysis (DMTA...

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Main Authors: Haleh Nowruzi Varzeghani, Iraj Amiri Amraei, Seyed Rasoul Mousavi
Format: Article
Language:English
Published: Wiley 2020-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2020/7908343
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author Haleh Nowruzi Varzeghani
Iraj Amiri Amraei
Seyed Rasoul Mousavi
author_facet Haleh Nowruzi Varzeghani
Iraj Amiri Amraei
Seyed Rasoul Mousavi
author_sort Haleh Nowruzi Varzeghani
collection DOAJ
description This study investigated the effect of polyethylene glycol (PEG) and nanosilica (NS) on the physical-mechanical properties and cure kinetics of diglycidyl ether of bisphenol-A-based epoxy (DGEBA-based EP) resin. For this purpose, tensile and viscometry tests, dynamic mechanical thermal analysis (DMTA), and differential scanning calorimetry (DSC) were carried out under dynamic conditions. The results showed that adding NS and PEG enhances the maximum cure temperature as well as the heat of cure reaction (ΔH) in EP-NS, while it decreases in EP-PEG and EP-PEG-NS. The cure kinetic parameters of EP-PEG-NS were calculated by Kissinger, Ozawa, and KSA methods and compared with each other. The Ea calculated from the Kissinger method (96.82 kJ/mol) was found to be lower than that of the Ozawa method (98.69 kJ/mol). Also, according to the KAS method, the apparent Ea was approximately constant within the 10-90% conversion range. Tensile strength and modulus increased by adding NS, while tensile strength diminished slightly by adding PEG to EP-NS. The glass transition temperature (Tg) was calculated using DMTA which was increased and decreased by the addition of NS and PEG, respectively. The results of the viscometry test showed that the viscosity increased with the presence of both PEG and NS and it prevented the deposition of solid particles.
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series International Journal of Polymer Science
spelling doaj-art-74420aaa6f0c4af9acfc21701f8cdd7b2025-08-20T03:33:53ZengWileyInternational Journal of Polymer Science1687-94221687-94302020-01-01202010.1155/2020/79083437908343Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy CompositesHaleh Nowruzi Varzeghani0Iraj Amiri Amraei1Seyed Rasoul Mousavi2Department of Material Science and Manufacturing Technology, Malek Ashtar University of Technology, Tehran 158751774, IranDepartment of Material Science and Manufacturing Technology, Malek Ashtar University of Technology, Tehran 158751774, IranDepartment of Material Science and Manufacturing Technology, Malek Ashtar University of Technology, Tehran 158751774, IranThis study investigated the effect of polyethylene glycol (PEG) and nanosilica (NS) on the physical-mechanical properties and cure kinetics of diglycidyl ether of bisphenol-A-based epoxy (DGEBA-based EP) resin. For this purpose, tensile and viscometry tests, dynamic mechanical thermal analysis (DMTA), and differential scanning calorimetry (DSC) were carried out under dynamic conditions. The results showed that adding NS and PEG enhances the maximum cure temperature as well as the heat of cure reaction (ΔH) in EP-NS, while it decreases in EP-PEG and EP-PEG-NS. The cure kinetic parameters of EP-PEG-NS were calculated by Kissinger, Ozawa, and KSA methods and compared with each other. The Ea calculated from the Kissinger method (96.82 kJ/mol) was found to be lower than that of the Ozawa method (98.69 kJ/mol). Also, according to the KAS method, the apparent Ea was approximately constant within the 10-90% conversion range. Tensile strength and modulus increased by adding NS, while tensile strength diminished slightly by adding PEG to EP-NS. The glass transition temperature (Tg) was calculated using DMTA which was increased and decreased by the addition of NS and PEG, respectively. The results of the viscometry test showed that the viscosity increased with the presence of both PEG and NS and it prevented the deposition of solid particles.http://dx.doi.org/10.1155/2020/7908343
spellingShingle Haleh Nowruzi Varzeghani
Iraj Amiri Amraei
Seyed Rasoul Mousavi
Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
International Journal of Polymer Science
title Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
title_full Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
title_fullStr Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
title_full_unstemmed Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
title_short Dynamic Cure Kinetics and Physical-Mechanical Properties of PEG/Nanosilica/Epoxy Composites
title_sort dynamic cure kinetics and physical mechanical properties of peg nanosilica epoxy composites
url http://dx.doi.org/10.1155/2020/7908343
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AT seyedrasoulmousavi dynamiccurekineticsandphysicalmechanicalpropertiesofpegnanosilicaepoxycomposites