Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges

Abstract Supercapacitors (SCs) are studied and used in various fields due to their high power density, fast charging/discharging rate, as well as long cycle life. Compared to other traditional electrode and electrolyte materials, supramolecular hydrogels have great advantages in the application of S...

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Main Authors: Wenshi Xu, Aibing Chen
Format: Article
Language:English
Published: Wiley 2024-10-01
Series:Aggregate
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Online Access:https://doi.org/10.1002/agt2.581
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author Wenshi Xu
Aibing Chen
author_facet Wenshi Xu
Aibing Chen
author_sort Wenshi Xu
collection DOAJ
description Abstract Supercapacitors (SCs) are studied and used in various fields due to their high power density, fast charging/discharging rate, as well as long cycle life. Compared to other traditional electrode and electrolyte materials, supramolecular hydrogels have great advantages in the application of SCs due to their excellent properties. Unlike covalent bonds, supramolecular systems are assembled through dynamic reversible bonds, including host–guest interactions, ion interactions, electrostatic interactions, hydrogen bonding, coordination interactions, etc. The resulting supramolecular hydrogels show some special functions, such as stretching, compression, adhesion, self‐healing, stimulus responsiveness, etc., making them strong candidates for the next generation of energy storage devices. This paper reviews the representative progress of electrodes, electrolytes, and SCs based on supramolecular hydrogels. Besides, the properties of supramolecular hydrogels, such as conductivity, extensibility, compressibility and elasticity, self‐healing, frost resistance, adhesion, and flexibility, are also reviewed to highlight the key role of excellent properties of hydrogel materials in SCs. In addition, this article also discusses the challenges faced by current technologies, hoping to continue promoting future research in this field.
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spelling doaj-art-72de3f39a70d4dc89d636112ca6b77c82025-08-20T01:50:45ZengWileyAggregate2692-45602024-10-0155n/an/a10.1002/agt2.581Application of supramolecular hydrogel in supercapacitors: Opportunities and challengesWenshi Xu0Aibing Chen1College of Chemical and Pharmaceutical Engineering Hebei University of Science and Technology Shijiazhuang ChinaCollege of Chemical and Pharmaceutical Engineering Hebei University of Science and Technology Shijiazhuang ChinaAbstract Supercapacitors (SCs) are studied and used in various fields due to their high power density, fast charging/discharging rate, as well as long cycle life. Compared to other traditional electrode and electrolyte materials, supramolecular hydrogels have great advantages in the application of SCs due to their excellent properties. Unlike covalent bonds, supramolecular systems are assembled through dynamic reversible bonds, including host–guest interactions, ion interactions, electrostatic interactions, hydrogen bonding, coordination interactions, etc. The resulting supramolecular hydrogels show some special functions, such as stretching, compression, adhesion, self‐healing, stimulus responsiveness, etc., making them strong candidates for the next generation of energy storage devices. This paper reviews the representative progress of electrodes, electrolytes, and SCs based on supramolecular hydrogels. Besides, the properties of supramolecular hydrogels, such as conductivity, extensibility, compressibility and elasticity, self‐healing, frost resistance, adhesion, and flexibility, are also reviewed to highlight the key role of excellent properties of hydrogel materials in SCs. In addition, this article also discusses the challenges faced by current technologies, hoping to continue promoting future research in this field.https://doi.org/10.1002/agt2.581electrodeelectrolytenoncovalent interactionssupercapacitorssupramolecular hydrogel
spellingShingle Wenshi Xu
Aibing Chen
Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
Aggregate
electrode
electrolyte
noncovalent interactions
supercapacitors
supramolecular hydrogel
title Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
title_full Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
title_fullStr Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
title_full_unstemmed Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
title_short Application of supramolecular hydrogel in supercapacitors: Opportunities and challenges
title_sort application of supramolecular hydrogel in supercapacitors opportunities and challenges
topic electrode
electrolyte
noncovalent interactions
supercapacitors
supramolecular hydrogel
url https://doi.org/10.1002/agt2.581
work_keys_str_mv AT wenshixu applicationofsupramolecularhydrogelinsupercapacitorsopportunitiesandchallenges
AT aibingchen applicationofsupramolecularhydrogelinsupercapacitorsopportunitiesandchallenges