Ultrafast all-optical generation of pure spin and valley currents

Abstract Pure currents comprise the flow of a two state quantum freedom – for example the electron spin – in the absence of charge flow. Radically different from the charge currents that underpin present day electronics, in two dimensional materials possessing additional two state freedoms such as v...

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Main Authors: D. Gill, S. Sharma, J. K. Dewhurst, S. Shallcross
Format: Article
Language:English
Published: Nature Portfolio 2025-06-01
Series:npj 2D Materials and Applications
Online Access:https://doi.org/10.1038/s41699-025-00558-0
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author D. Gill
S. Sharma
J. K. Dewhurst
S. Shallcross
author_facet D. Gill
S. Sharma
J. K. Dewhurst
S. Shallcross
author_sort D. Gill
collection DOAJ
description Abstract Pure currents comprise the flow of a two state quantum freedom – for example the electron spin – in the absence of charge flow. Radically different from the charge currents that underpin present day electronics, in two dimensional materials possessing additional two state freedoms such as valley index they offer profound possibilities for miniaturization and energy efficiency in a next generation spin- and valleytronics. Here we demonstrate a robust multi-pump lightwave protocol capable of generating both pure spin and valley currents on femtosecond times. The generation time is determined by the 2d material gap, with the creation of pure spin current in WSe2 at 40 fs and pure valley current in bilayer graphene at ~ 200 fs. Our all-optical approach demands no special material design, requiring only a gapped valley active material, and is thus applicable to a wide range of 2d materials.
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institution OA Journals
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series npj 2D Materials and Applications
spelling doaj-art-7280c8b3f70748fb8b8193b5a02d76dc2025-08-20T02:06:31ZengNature Portfolionpj 2D Materials and Applications2397-71322025-06-01911910.1038/s41699-025-00558-0Ultrafast all-optical generation of pure spin and valley currentsD. Gill0S. Sharma1J. K. Dewhurst2S. Shallcross3Max-Born-Institute for Non-Linear opticsMax-Born-Institute for Non-Linear opticsMax-Planck-Institut fur Mikrostrukturphysik Weinberg 2Max-Born-Institute for Non-Linear opticsAbstract Pure currents comprise the flow of a two state quantum freedom – for example the electron spin – in the absence of charge flow. Radically different from the charge currents that underpin present day electronics, in two dimensional materials possessing additional two state freedoms such as valley index they offer profound possibilities for miniaturization and energy efficiency in a next generation spin- and valleytronics. Here we demonstrate a robust multi-pump lightwave protocol capable of generating both pure spin and valley currents on femtosecond times. The generation time is determined by the 2d material gap, with the creation of pure spin current in WSe2 at 40 fs and pure valley current in bilayer graphene at ~ 200 fs. Our all-optical approach demands no special material design, requiring only a gapped valley active material, and is thus applicable to a wide range of 2d materials.https://doi.org/10.1038/s41699-025-00558-0
spellingShingle D. Gill
S. Sharma
J. K. Dewhurst
S. Shallcross
Ultrafast all-optical generation of pure spin and valley currents
npj 2D Materials and Applications
title Ultrafast all-optical generation of pure spin and valley currents
title_full Ultrafast all-optical generation of pure spin and valley currents
title_fullStr Ultrafast all-optical generation of pure spin and valley currents
title_full_unstemmed Ultrafast all-optical generation of pure spin and valley currents
title_short Ultrafast all-optical generation of pure spin and valley currents
title_sort ultrafast all optical generation of pure spin and valley currents
url https://doi.org/10.1038/s41699-025-00558-0
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AT ssharma ultrafastallopticalgenerationofpurespinandvalleycurrents
AT jkdewhurst ultrafastallopticalgenerationofpurespinandvalleycurrents
AT sshallcross ultrafastallopticalgenerationofpurespinandvalleycurrents