Glassy dynamics of SrTiO3-based two-dimensional electron gas
Abstract Electron glasses offer a convenient laboratory platform to study glassy dynamics, traditionally attributed to the interplay of long-range Coulomb interactions and disorder. Existing experimental studies on electron glass have focused on doped semiconductors, strongly correlated systems, gra...
Saved in:
| Main Authors: | , , , , , , , |
|---|---|
| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2025-04-01
|
| Series: | Communications Materials |
| Online Access: | https://doi.org/10.1038/s43246-025-00760-z |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1850284659228803072 |
|---|---|
| author | Jyotirmay Maity Shashank Kumar Ojha Prithwijit Mandal Manav Beniwal Nandana Bhattacharya Andrei Gloskovskii Christoph Schlueter Srimanta Middey |
| author_facet | Jyotirmay Maity Shashank Kumar Ojha Prithwijit Mandal Manav Beniwal Nandana Bhattacharya Andrei Gloskovskii Christoph Schlueter Srimanta Middey |
| author_sort | Jyotirmay Maity |
| collection | DOAJ |
| description | Abstract Electron glasses offer a convenient laboratory platform to study glassy dynamics, traditionally attributed to the interplay of long-range Coulomb interactions and disorder. Existing experimental studies on electron glass have focused on doped semiconductors, strongly correlated systems, granular systems, etc., which are far from the well-delocalized limit. Here, we demonstrate that the ferroelastic twin walls of well-known quantum paraelectric SrTiO3 can induce glassy electron dynamics even in a metallic phase. We show that the emergent two-dimensional electron gas at the γ-Al2O3/SrTiO3 interface exhibits long-lasting resistance relaxations and memory effects at low temperatures, hallmarks of glassiness. Moreover, the glass-like relaxations can be tuned by the application of an electric field, implying that the observed glassy dynamics relate to the development of polarity near the structural twin walls of SrTiO3 and the complex interactions among them. The observation of this glassy metal phase also contributes to the growing understanding of the fascinating and diverse emergent phenomena near the quantum critical point. |
| format | Article |
| id | doaj-art-722b246a1e7d40c98c6f62bd93f17df9 |
| institution | OA Journals |
| issn | 2662-4443 |
| language | English |
| publishDate | 2025-04-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Communications Materials |
| spelling | doaj-art-722b246a1e7d40c98c6f62bd93f17df92025-08-20T01:47:32ZengNature PortfolioCommunications Materials2662-44432025-04-01611810.1038/s43246-025-00760-zGlassy dynamics of SrTiO3-based two-dimensional electron gasJyotirmay Maity0Shashank Kumar Ojha1Prithwijit Mandal2Manav Beniwal3Nandana Bhattacharya4Andrei Gloskovskii5Christoph Schlueter6Srimanta Middey7Department of Physics, Indian Institute of ScienceDepartment of Physics, Indian Institute of ScienceDepartment of Physics, Indian Institute of ScienceDepartment of Physics, Indian Institute of ScienceDepartment of Physics, Indian Institute of ScienceDeutsches Elektronen-Synchrotron DESYDeutsches Elektronen-Synchrotron DESYDepartment of Physics, Indian Institute of ScienceAbstract Electron glasses offer a convenient laboratory platform to study glassy dynamics, traditionally attributed to the interplay of long-range Coulomb interactions and disorder. Existing experimental studies on electron glass have focused on doped semiconductors, strongly correlated systems, granular systems, etc., which are far from the well-delocalized limit. Here, we demonstrate that the ferroelastic twin walls of well-known quantum paraelectric SrTiO3 can induce glassy electron dynamics even in a metallic phase. We show that the emergent two-dimensional electron gas at the γ-Al2O3/SrTiO3 interface exhibits long-lasting resistance relaxations and memory effects at low temperatures, hallmarks of glassiness. Moreover, the glass-like relaxations can be tuned by the application of an electric field, implying that the observed glassy dynamics relate to the development of polarity near the structural twin walls of SrTiO3 and the complex interactions among them. The observation of this glassy metal phase also contributes to the growing understanding of the fascinating and diverse emergent phenomena near the quantum critical point.https://doi.org/10.1038/s43246-025-00760-z |
| spellingShingle | Jyotirmay Maity Shashank Kumar Ojha Prithwijit Mandal Manav Beniwal Nandana Bhattacharya Andrei Gloskovskii Christoph Schlueter Srimanta Middey Glassy dynamics of SrTiO3-based two-dimensional electron gas Communications Materials |
| title | Glassy dynamics of SrTiO3-based two-dimensional electron gas |
| title_full | Glassy dynamics of SrTiO3-based two-dimensional electron gas |
| title_fullStr | Glassy dynamics of SrTiO3-based two-dimensional electron gas |
| title_full_unstemmed | Glassy dynamics of SrTiO3-based two-dimensional electron gas |
| title_short | Glassy dynamics of SrTiO3-based two-dimensional electron gas |
| title_sort | glassy dynamics of srtio3 based two dimensional electron gas |
| url | https://doi.org/10.1038/s43246-025-00760-z |
| work_keys_str_mv | AT jyotirmaymaity glassydynamicsofsrtio3basedtwodimensionalelectrongas AT shashankkumarojha glassydynamicsofsrtio3basedtwodimensionalelectrongas AT prithwijitmandal glassydynamicsofsrtio3basedtwodimensionalelectrongas AT manavbeniwal glassydynamicsofsrtio3basedtwodimensionalelectrongas AT nandanabhattacharya glassydynamicsofsrtio3basedtwodimensionalelectrongas AT andreigloskovskii glassydynamicsofsrtio3basedtwodimensionalelectrongas AT christophschlueter glassydynamicsofsrtio3basedtwodimensionalelectrongas AT srimantamiddey glassydynamicsofsrtio3basedtwodimensionalelectrongas |