Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices

As per the electrical properties, chromium oxide (Cr2O3) nanoparticles are categorized as semiconductors and could be used as an alternative to conventional polymer and small molecule-based semiconductor materials used in organic thin film transistors (OTFTs). In the current investigation, the perfo...

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Main Authors: Arun Singh Rathod, Abhilasha Mishra, Waseem Ahmad, Sanjay Kumar
Format: Article
Language:English
Published: Iranian Chemical Society 2025-04-01
Series:Nanochemistry Research
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Online Access:http://www.nanochemres.org/article_216708_c2da424cb15ac6f22242f0d8d4871798.pdf
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author Arun Singh Rathod
Abhilasha Mishra
Waseem Ahmad
Sanjay Kumar
author_facet Arun Singh Rathod
Abhilasha Mishra
Waseem Ahmad
Sanjay Kumar
author_sort Arun Singh Rathod
collection DOAJ
description As per the electrical properties, chromium oxide (Cr2O3) nanoparticles are categorized as semiconductors and could be used as an alternative to conventional polymer and small molecule-based semiconductor materials used in organic thin film transistors (OTFTs). In the current investigation, the performance of two bottom gate bottom contact (BGBC) OTFTs comprising pentacene and chromium oxide (Cr2O3) nanoparticles as semiconductor material, respectively, was analyzed comparatively. SILVACO TCAD simulation tool was employed to analyze OTFT structures. Performance factors such as mobility in linear regime, saturation mobility, output current, ION/IOFF ratio, trans conductance, sub-threshold slope, and threshold voltage were explored to determine the superiority of Cr2O3 nanoparticles over pentacene. The linear mobility of Cr2O3 NPs was found to be 14.46 while the pentacene linear mobility was found to be 5.79. Furthermore, the solution mobility of the Cr2O3 NPs was found to be 1.239 and the pentacene solution mobility was 0.41. The Cr2O3 nanoparticles-based device exhibited a significantly higher Ids value of 17.5136 x 10-6 µA as compare to pentacene. Additionally, the Cr2O3 nanoparticles-based device showed an increased transconductance value of 12.241277 x 10-6 µS. The obtained results offer valuable insights into performance enhancement of OTFTs using Cr2O3 nano particles as semiconductor material, without altering the dimensions or operational voltages of the OTFT structures. These findings provide valuable insights for optimizing organic thin film transistors, thereby contributing to the advancement of efficient organic electronic systems.
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spelling doaj-art-72129b829bf34c08b8c689df14e684b32025-08-20T03:14:10ZengIranian Chemical SocietyNanochemistry Research2538-42792423-818X2025-04-0110213714910.22036/NCR.2025.02.02216708Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor DevicesArun Singh Rathod0Abhilasha Mishra1Waseem Ahmad2Sanjay Kumar3Department of Electronics and Communication Engineering, Graphic Era Hill University, IndiaDepartment of Chemistry, Graphic Era deemed to be University, IndiaDepartment of Chemistry, Graphic Era deemed to be University, IndiaDepartment of Food Science and Technology, Graphic Era Deemed to Be University, Dehradun, IndiaAs per the electrical properties, chromium oxide (Cr2O3) nanoparticles are categorized as semiconductors and could be used as an alternative to conventional polymer and small molecule-based semiconductor materials used in organic thin film transistors (OTFTs). In the current investigation, the performance of two bottom gate bottom contact (BGBC) OTFTs comprising pentacene and chromium oxide (Cr2O3) nanoparticles as semiconductor material, respectively, was analyzed comparatively. SILVACO TCAD simulation tool was employed to analyze OTFT structures. Performance factors such as mobility in linear regime, saturation mobility, output current, ION/IOFF ratio, trans conductance, sub-threshold slope, and threshold voltage were explored to determine the superiority of Cr2O3 nanoparticles over pentacene. The linear mobility of Cr2O3 NPs was found to be 14.46 while the pentacene linear mobility was found to be 5.79. Furthermore, the solution mobility of the Cr2O3 NPs was found to be 1.239 and the pentacene solution mobility was 0.41. The Cr2O3 nanoparticles-based device exhibited a significantly higher Ids value of 17.5136 x 10-6 µA as compare to pentacene. Additionally, the Cr2O3 nanoparticles-based device showed an increased transconductance value of 12.241277 x 10-6 µS. The obtained results offer valuable insights into performance enhancement of OTFTs using Cr2O3 nano particles as semiconductor material, without altering the dimensions or operational voltages of the OTFT structures. These findings provide valuable insights for optimizing organic thin film transistors, thereby contributing to the advancement of efficient organic electronic systems.http://www.nanochemres.org/article_216708_c2da424cb15ac6f22242f0d8d4871798.pdfgreen synthesisnanoparticlescr2o3 npsorganic thin film transistorssilvaco tcad
spellingShingle Arun Singh Rathod
Abhilasha Mishra
Waseem Ahmad
Sanjay Kumar
Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
Nanochemistry Research
green synthesis
nanoparticles
cr2o3 nps
organic thin film transistors
silvaco tcad
title Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
title_full Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
title_fullStr Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
title_full_unstemmed Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
title_short Green Synthesis of Cr2O3 Nanoparticles for Enhanced OTFT Performance compared to Pentacene-Based Organic Thin Film Transistor Devices
title_sort green synthesis of cr2o3 nanoparticles for enhanced otft performance compared to pentacene based organic thin film transistor devices
topic green synthesis
nanoparticles
cr2o3 nps
organic thin film transistors
silvaco tcad
url http://www.nanochemres.org/article_216708_c2da424cb15ac6f22242f0d8d4871798.pdf
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AT waseemahmad greensynthesisofcr2o3nanoparticlesforenhancedotftperformancecomparedtopentacenebasedorganicthinfilmtransistordevices
AT sanjaykumar greensynthesisofcr2o3nanoparticlesforenhancedotftperformancecomparedtopentacenebasedorganicthinfilmtransistordevices