Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents

In this study, we evaluated the cytotoxic activity and antiproliferative potency of novel octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives ( 1 – 7 ) in MCF-7 and MDA-MB-231 breast cancer cell lines. Annexin V binding assay and disruption of the mitochondrial potential were performed to deter...

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Main Authors: Agnieszka Gornowicz, Natalia Pawłowska, Anna Czajkowska, Robert Czarnomysy, Anna Bielawska, Krzysztof Bielawski, Olga Michalak, Olga Staszewska-Krajewska, Zbigniew Kałuża
Format: Article
Language:English
Published: SAGE Publishing 2017-05-01
Series:Tumor Biology
Online Access:https://doi.org/10.1177/1010428317701641
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author Agnieszka Gornowicz
Natalia Pawłowska
Anna Czajkowska
Robert Czarnomysy
Anna Bielawska
Krzysztof Bielawski
Olga Michalak
Olga Staszewska-Krajewska
Zbigniew Kałuża
author_facet Agnieszka Gornowicz
Natalia Pawłowska
Anna Czajkowska
Robert Czarnomysy
Anna Bielawska
Krzysztof Bielawski
Olga Michalak
Olga Staszewska-Krajewska
Zbigniew Kałuża
author_sort Agnieszka Gornowicz
collection DOAJ
description In this study, we evaluated the cytotoxic activity and antiproliferative potency of novel octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives ( 1 – 7 ) in MCF-7 and MDA-MB-231 breast cancer cell lines. Annexin V binding assay and disruption of the mitochondrial potential were performed to determine apoptosis. The activity of caspases 3, 8, 9, and 10 was measured after 24 h of incubation with tested compounds to explain detailed molecular mechanism of induction of apoptosis. The results from experiments were compared with effects obtained after incubation in the presence of camptothecin and etoposide. Our study demonstrated that the most active compounds in both analyzed breast cancer cell lines were compounds 3 and 4 . We also observed that all compounds induced apoptosis. We demonstrated the higher activity of caspases 3, 8, 9, and 10, which confirmed that induction of apoptosis is associated with external and internal cell death pathway. Our study revealed that the novel compounds in group of diisoquinoline derivatives are promising candidates in anticancer treatment by activation of both extrinsic and intrinsic apoptotic pathways.
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spelling doaj-art-7008c7bcda554d599ec71ea88eb0e4ba2025-08-20T02:52:34ZengSAGE PublishingTumor Biology1423-03802017-05-013910.1177/1010428317701641Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agentsAgnieszka Gornowicz0Natalia Pawłowska1Anna Czajkowska2Robert Czarnomysy3Anna Bielawska4Krzysztof Bielawski5Olga Michalak6Olga Staszewska-Krajewska7Zbigniew Kałuża8Department of Biotechnology, Medical University of Bialystok, Bialystok, PolandDepartment of Synthesis and Technology of Drugs, Medical University of Bialystok, Bialystok, PolandDepartment of Biotechnology, Medical University of Bialystok, Bialystok, PolandDepartment of Synthesis and Technology of Drugs, Medical University of Bialystok, Bialystok, PolandDepartment of Biotechnology, Medical University of Bialystok, Bialystok, PolandDepartment of Synthesis and Technology of Drugs, Medical University of Bialystok, Bialystok, PolandInstitute of Organic Chemistry, Polish Academy of Sciences, Warsaw, PolandInstitute of Organic Chemistry, Polish Academy of Sciences, Warsaw, PolandInstitute of Organic Chemistry, Polish Academy of Sciences, Warsaw, PolandIn this study, we evaluated the cytotoxic activity and antiproliferative potency of novel octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives ( 1 – 7 ) in MCF-7 and MDA-MB-231 breast cancer cell lines. Annexin V binding assay and disruption of the mitochondrial potential were performed to determine apoptosis. The activity of caspases 3, 8, 9, and 10 was measured after 24 h of incubation with tested compounds to explain detailed molecular mechanism of induction of apoptosis. The results from experiments were compared with effects obtained after incubation in the presence of camptothecin and etoposide. Our study demonstrated that the most active compounds in both analyzed breast cancer cell lines were compounds 3 and 4 . We also observed that all compounds induced apoptosis. We demonstrated the higher activity of caspases 3, 8, 9, and 10, which confirmed that induction of apoptosis is associated with external and internal cell death pathway. Our study revealed that the novel compounds in group of diisoquinoline derivatives are promising candidates in anticancer treatment by activation of both extrinsic and intrinsic apoptotic pathways.https://doi.org/10.1177/1010428317701641
spellingShingle Agnieszka Gornowicz
Natalia Pawłowska
Anna Czajkowska
Robert Czarnomysy
Anna Bielawska
Krzysztof Bielawski
Olga Michalak
Olga Staszewska-Krajewska
Zbigniew Kałuża
Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
Tumor Biology
title Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
title_full Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
title_fullStr Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
title_full_unstemmed Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
title_short Biological evaluation of octahydropyrazin[2,1-a:5,4-a′]diisoquinoline derivatives as potent anticancer agents
title_sort biological evaluation of octahydropyrazin 2 1 a 5 4 a diisoquinoline derivatives as potent anticancer agents
url https://doi.org/10.1177/1010428317701641
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