Simultaneous determination of 6 organophosphoric flame retardants in aquatic products by GC-MS/MS

A method for simultaneous determination of 6 organophosphoric flame retardants in aquatic products was developed by gas chromatogeny- tandem mass spectrometry (GC-MS/MS) with dispersive solid phase extraction (DSPE) as purification method. The samples were extracted with 0.5% formic acid-acetonitril...

Full description

Saved in:
Bibliographic Details
Main Author: QUAN Haiqian, CHEN Kun, HE Ming
Format: Article
Language:English
Published: Editorial Department of China Brewing 2024-10-01
Series:Zhongguo niangzao
Subjects:
Online Access:https://manu61.magtech.com.cn/zgnz/fileup/0254-5071/PDF/0254-5071-2024-43-10-265.pdf
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:A method for simultaneous determination of 6 organophosphoric flame retardants in aquatic products was developed by gas chromatogeny- tandem mass spectrometry (GC-MS/MS) with dispersive solid phase extraction (DSPE) as purification method. The samples were extracted with 0.5% formic acid-acetonitrile solution, after salting out and centrifugation, the supernatant was purified with 4 kinds of solid phase extractants: primary secondary amine (PSA), C18, graphitized carbon black (GCB) and silica gel. After nitrogen (N<sub>2</sub>) concentration, it was separated by DB-5ms quartz capillary- column chromatography (30 m&#x00D7;0.25 mm&#x00D7;0.25 μm), and quantified by isotope internal standard. The results showed that the 6 organophosphoric flame retardants had good linear relationship in the range of 1.0-50 μg/L (R<sup>2</sup>&gt;0.999). The average recovery rates of 6 organophosphoric flame retardants were 79.8%-97.4%, the relative standard deviation (RSD) of precision test results was 2.66%-7.98% under the standard addition 2.0 μg/kg, 4.0 μg/kg and 10.0 μg/kg. The limits of detection (LOD) was 0.6 μg/kg, and the limits of quantification (LOQ) was 2.0 μg/kg. The method had the advantages of simple operation, high sensitivity, good accuracy and precision, and could satisfy the determination requirements of 6 kinds of organophosphate ester flame retardants in aquatic products.
ISSN:0254-5071