Extracting RABBITT-like phase information from time-dependent transient absorption spectra
We explore how the spectral phase of attosecond pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an atomic or molecular system governs the dynamics. As already sh...
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| Main Authors: | , , , , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
American Physical Society
2025-06-01
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| Series: | Physical Review Research |
| Online Access: | http://doi.org/10.1103/PhysRevResearch.7.023244 |
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| Summary: | We explore how the spectral phase of attosecond pulse trains influences the optical cross section in transient absorption (TA) spectroscopy. The interaction of extreme ultraviolet (XUV) and time-delayed near-infrared (NIR) fields with an atomic or molecular system governs the dynamics. As already shown in RABBITT experiments (Reconstruction of Attosecond Beating by Interference of Two-Photon Transitions), the spectral phase of the XUV pulses can be extracted from the photoionization spectrum as a function of the time delay. Similarly, this XUV phase imprints itself on delay-dependent optical cross-section oscillations. With a perturbative analytical approach and by simulating the quantum dynamics both in a few-level model and via solving the time-dependent Schrödinger equation for atomic hydrogen, we reveal the similarity between the spectral phase in RABBITT and TA spectroscopy. |
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| ISSN: | 2643-1564 |