Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response

Abstract Cloud responses to surface‐based sources of aerosol perturbation partially depend on how turbulent transport of the aerosol to cloud base affects the spatial and temporal distribution of aerosol. Here, scenarios of plume injection below a marine stratocumulus cloud are modeled using large e...

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Main Authors: Chandru Dhandapani, Colleen M. Kaul, Kyle G. Pressel, Peter N. Blossey, Robert Wood, Gourihar Kulkarni
Format: Article
Language:English
Published: American Geophysical Union (AGU) 2025-02-01
Series:Journal of Advances in Modeling Earth Systems
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Online Access:https://doi.org/10.1029/2024MS004546
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author Chandru Dhandapani
Colleen M. Kaul
Kyle G. Pressel
Peter N. Blossey
Robert Wood
Gourihar Kulkarni
author_facet Chandru Dhandapani
Colleen M. Kaul
Kyle G. Pressel
Peter N. Blossey
Robert Wood
Gourihar Kulkarni
author_sort Chandru Dhandapani
collection DOAJ
description Abstract Cloud responses to surface‐based sources of aerosol perturbation partially depend on how turbulent transport of the aerosol to cloud base affects the spatial and temporal distribution of aerosol. Here, scenarios of plume injection below a marine stratocumulus cloud are modeled using large eddy simulations coupled to a prognostic bulk aerosol and cloud microphysics scheme. Both passive plumes, consisting of an inert tracer, and active plumes are investigated, where the latter are representative of saltwater droplet plumes such as have been proposed for marine cloud brightening. Passive plume scenarios show higher in‐plume cloud brightness (relative to out‐of‐plume) due to the predominant transport of the passive plume tracer from the near‐surface to the cloud layer within updrafts. These updrafts rise into brighter areas within the cloud deck, even in the absence of an aerosol perturbation associated with an active plume. Comparing albedo at in‐plume to out‐of‐plume locations associates the inert plume with the brightest cloud locations, without any causal effect of the plume on the cloud. Numerical sensitivities are first assessed to establish a suitable model configuration. Then sensitivity to particle injection rate is investigated. Trade‐offs are identified between the number of injected particles and the suppressive effect of droplet evaporation on plume loft and spread. Furthermore, as the near‐field in‐plume brightening effect does not depend significantly on injection rate given a suitable definition of perturbed versus unperturbed regions of the flow, plume area is a key controlling factor on the overall cloud brightening effect of an aerosol perturbation.
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spelling doaj-art-6edc0a770e5244a891a99b0e5e1bcd192025-08-20T02:16:06ZengAmerican Geophysical Union (AGU)Journal of Advances in Modeling Earth Systems1942-24662025-02-01172n/an/a10.1029/2024MS004546Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud ResponseChandru Dhandapani0Colleen M. Kaul1Kyle G. Pressel2Peter N. Blossey3Robert Wood4Gourihar Kulkarni5Pacific Northwest National Laboratory Richland WA USAPacific Northwest National Laboratory Richland WA USAPacific Northwest National Laboratory Richland WA USADepartment of Atmospheric Sciences University of Washington Seattle WA USADepartment of Atmospheric Sciences University of Washington Seattle WA USAPacific Northwest National Laboratory Richland WA USAAbstract Cloud responses to surface‐based sources of aerosol perturbation partially depend on how turbulent transport of the aerosol to cloud base affects the spatial and temporal distribution of aerosol. Here, scenarios of plume injection below a marine stratocumulus cloud are modeled using large eddy simulations coupled to a prognostic bulk aerosol and cloud microphysics scheme. Both passive plumes, consisting of an inert tracer, and active plumes are investigated, where the latter are representative of saltwater droplet plumes such as have been proposed for marine cloud brightening. Passive plume scenarios show higher in‐plume cloud brightness (relative to out‐of‐plume) due to the predominant transport of the passive plume tracer from the near‐surface to the cloud layer within updrafts. These updrafts rise into brighter areas within the cloud deck, even in the absence of an aerosol perturbation associated with an active plume. Comparing albedo at in‐plume to out‐of‐plume locations associates the inert plume with the brightest cloud locations, without any causal effect of the plume on the cloud. Numerical sensitivities are first assessed to establish a suitable model configuration. Then sensitivity to particle injection rate is investigated. Trade‐offs are identified between the number of injected particles and the suppressive effect of droplet evaporation on plume loft and spread. Furthermore, as the near‐field in‐plume brightening effect does not depend significantly on injection rate given a suitable definition of perturbed versus unperturbed regions of the flow, plume area is a key controlling factor on the overall cloud brightening effect of an aerosol perturbation.https://doi.org/10.1029/2024MS004546large eddy simulationsaerosol cloud interactionscloud microphysicsmarine cloud brighteningplume transportnumerical sensitivities
spellingShingle Chandru Dhandapani
Colleen M. Kaul
Kyle G. Pressel
Peter N. Blossey
Robert Wood
Gourihar Kulkarni
Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
Journal of Advances in Modeling Earth Systems
large eddy simulations
aerosol cloud interactions
cloud microphysics
marine cloud brightening
plume transport
numerical sensitivities
title Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
title_full Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
title_fullStr Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
title_full_unstemmed Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
title_short Sensitivities of Large Eddy Simulations of Aerosol Plume Transport and Cloud Response
title_sort sensitivities of large eddy simulations of aerosol plume transport and cloud response
topic large eddy simulations
aerosol cloud interactions
cloud microphysics
marine cloud brightening
plume transport
numerical sensitivities
url https://doi.org/10.1029/2024MS004546
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