First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics

To explore the regulation mechanism of microstructure and macroscopic electrical properties of Sn-doped BaTiO3 lead- free piezoelectric ceramics. Based on density functional theory, the band structure, state density and piezoelectric properties of ceramics (BaTi1 - x Snx O3 ,abbreviated as BTSx,x =0...

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Main Authors: WANG Wanru, LI Caixia, MA Xiaoxuan, LI Chenglong, JI Nan, LI Tianqi
Format: Article
Language:zho
Published: Harbin University of Science and Technology Publications 2024-06-01
Series:Journal of Harbin University of Science and Technology
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Online Access:https://hlgxb.hrbust.edu.cn/#/digest?ArticleID=2340
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author WANG Wanru
LI Caixia
MA Xiaoxuan
LI Chenglong
JI Nan
LI Tianqi
author_facet WANG Wanru
LI Caixia
MA Xiaoxuan
LI Chenglong
JI Nan
LI Tianqi
author_sort WANG Wanru
collection DOAJ
description To explore the regulation mechanism of microstructure and macroscopic electrical properties of Sn-doped BaTiO3 lead- free piezoelectric ceramics. Based on density functional theory, the band structure, state density and piezoelectric properties of ceramics (BaTi1 - x Snx O3 ,abbreviated as BTSx,x =0 , 0. 125 , 0. 20 , 0. 25 , 0. 33 and 0. 50) were calculated by using first-principles, and the piezoelectric regulation mechanism was analyzed. The results show that the BaTiO3 ceramic band gap width is 1. 780 eV. It is found that in the range of the studied components, with the increase of Sn doping, the band gap width of BTSx ceramic samples decreases monotonically. The state density pattern shows that the hybridization between atoms makes the piezoelectric property more stable, and the B-position Sn doping enhances the room temperature piezoelectric performance of the sample.
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institution DOAJ
issn 1007-2683
language zho
publishDate 2024-06-01
publisher Harbin University of Science and Technology Publications
record_format Article
series Journal of Harbin University of Science and Technology
spelling doaj-art-6ea992ccb7794e618107ea1df1b272162025-08-20T03:17:24ZzhoHarbin University of Science and Technology PublicationsJournal of Harbin University of Science and Technology1007-26832024-06-01290313414010.15938/j.jhust.2024.03.016First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate CeramicsWANG Wanru0LI Caixia1MA Xiaoxuan2LI Chenglong3JI Nan4LI Tianqi5Physics Teaching and Experimental Center, School of Science, Harbin University of Science and Technology, Harbin 150080 , ChinaPhysics Teaching and Experimental Center, School of Science, Harbin University of Science and Technology, Harbin 150080 , ChinaCollege of Energy and Machinery, Dezhou University, Dezhou 253025 , ChinaPhysics Teaching and Experimental Center, School of Science, Harbin University of Science and Technology, Harbin 150080 , ChinaPhysics Teaching and Experimental Center, School of Science, Harbin University of Science and Technology, Harbin 150080 , ChinaPhysics Teaching and Experimental Center, School of Science, Harbin University of Science and Technology, Harbin 150080 , ChinaTo explore the regulation mechanism of microstructure and macroscopic electrical properties of Sn-doped BaTiO3 lead- free piezoelectric ceramics. Based on density functional theory, the band structure, state density and piezoelectric properties of ceramics (BaTi1 - x Snx O3 ,abbreviated as BTSx,x =0 , 0. 125 , 0. 20 , 0. 25 , 0. 33 and 0. 50) were calculated by using first-principles, and the piezoelectric regulation mechanism was analyzed. The results show that the BaTiO3 ceramic band gap width is 1. 780 eV. It is found that in the range of the studied components, with the increase of Sn doping, the band gap width of BTSx ceramic samples decreases monotonically. The state density pattern shows that the hybridization between atoms makes the piezoelectric property more stable, and the B-position Sn doping enhances the room temperature piezoelectric performance of the sample.https://hlgxb.hrbust.edu.cn/#/digest?ArticleID=2340first-principlesbatio3 ceramicselectronic structurepiezoelectricity
spellingShingle WANG Wanru
LI Caixia
MA Xiaoxuan
LI Chenglong
JI Nan
LI Tianqi
First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
Journal of Harbin University of Science and Technology
first-principles
batio3 ceramics
electronic structure
piezoelectricity
title First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
title_full First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
title_fullStr First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
title_full_unstemmed First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
title_short First-principles Calculation and Analysis of Piezoelectric Properties of Sn-doped Barium Titanate Ceramics
title_sort first principles calculation and analysis of piezoelectric properties of sn doped barium titanate ceramics
topic first-principles
batio3 ceramics
electronic structure
piezoelectricity
url https://hlgxb.hrbust.edu.cn/#/digest?ArticleID=2340
work_keys_str_mv AT wangwanru firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics
AT licaixia firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics
AT maxiaoxuan firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics
AT lichenglong firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics
AT jinan firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics
AT litianqi firstprinciplescalculationandanalysisofpiezoelectricpropertiesofsndopedbariumtitanateceramics