Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification

The aim of our current research was to synthesize some transition metal complexes of Naproxen, determine their physical properties, and examine their relative stability under various conditions. Characterizations of these complexes were done by 1H-NMR, Differential Scanning Calorimetry (DSC), FT-IR,...

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Main Authors: Md. Sharif Hasan, Ruhul Kayesh, Farida Begum, S. M. Abdur Rahman
Format: Article
Language:English
Published: Wiley 2016-01-01
Series:Journal of Analytical Methods in Chemistry
Online Access:http://dx.doi.org/10.1155/2016/3560695
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author Md. Sharif Hasan
Ruhul Kayesh
Farida Begum
S. M. Abdur Rahman
author_facet Md. Sharif Hasan
Ruhul Kayesh
Farida Begum
S. M. Abdur Rahman
author_sort Md. Sharif Hasan
collection DOAJ
description The aim of our current research was to synthesize some transition metal complexes of Naproxen, determine their physical properties, and examine their relative stability under various conditions. Characterizations of these complexes were done by 1H-NMR, Differential Scanning Calorimetry (DSC), FT-IR, HPLC, and scanning electron microscope (SEM). Complexes were subjected to acidic, basic, and aqueous hydrolysis as well as oxidation, reduction, and thermal degradation. Also the reversed phase high-performance liquid chromatography (RP-HPLC) method of Naproxen outlined in USP was verified for the Naproxen-metal complexes, with respect to accuracy, precision, solution stability, robustness, and system suitability. The melting points of the complexes were higher than that of the parent drug molecule suggesting their thermal stability. In forced degradation study, complexes were found more stable than the Naproxen itself in all conditions: acidic, basic, oxidation, and reduction media. All the HPLC verification parameters were found within the acceptable value. Therefore, it can be concluded from the study that the metal complexes of Naproxen can be more stable drug entity and offer better efficacy and longer shelf life than the parent Naproxen.
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institution Kabale University
issn 2090-8865
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series Journal of Analytical Methods in Chemistry
spelling doaj-art-6e6a2d703a7f43bfab71144a3e2ec9ac2025-08-20T03:33:54ZengWileyJournal of Analytical Methods in Chemistry2090-88652090-88732016-01-01201610.1155/2016/35606953560695Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method VerificationMd. Sharif Hasan0Ruhul Kayesh1Farida Begum2S. M. Abdur Rahman3Department of Clinical Pharmacy and Pharmacology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Pharmaceutical Chemistry, University of Dhaka, Dhaka 1000, BangladeshDepartment of Clinical Pharmacy and Pharmacology, University of Dhaka, Dhaka 1000, BangladeshDepartment of Clinical Pharmacy and Pharmacology, University of Dhaka, Dhaka 1000, BangladeshThe aim of our current research was to synthesize some transition metal complexes of Naproxen, determine their physical properties, and examine their relative stability under various conditions. Characterizations of these complexes were done by 1H-NMR, Differential Scanning Calorimetry (DSC), FT-IR, HPLC, and scanning electron microscope (SEM). Complexes were subjected to acidic, basic, and aqueous hydrolysis as well as oxidation, reduction, and thermal degradation. Also the reversed phase high-performance liquid chromatography (RP-HPLC) method of Naproxen outlined in USP was verified for the Naproxen-metal complexes, with respect to accuracy, precision, solution stability, robustness, and system suitability. The melting points of the complexes were higher than that of the parent drug molecule suggesting their thermal stability. In forced degradation study, complexes were found more stable than the Naproxen itself in all conditions: acidic, basic, oxidation, and reduction media. All the HPLC verification parameters were found within the acceptable value. Therefore, it can be concluded from the study that the metal complexes of Naproxen can be more stable drug entity and offer better efficacy and longer shelf life than the parent Naproxen.http://dx.doi.org/10.1155/2016/3560695
spellingShingle Md. Sharif Hasan
Ruhul Kayesh
Farida Begum
S. M. Abdur Rahman
Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
Journal of Analytical Methods in Chemistry
title Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
title_full Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
title_fullStr Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
title_full_unstemmed Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
title_short Transition Metal Complexes of Naproxen: Synthesis, Characterization, Forced Degradation Studies, and Analytical Method Verification
title_sort transition metal complexes of naproxen synthesis characterization forced degradation studies and analytical method verification
url http://dx.doi.org/10.1155/2016/3560695
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AT faridabegum transitionmetalcomplexesofnaproxensynthesischaracterizationforceddegradationstudiesandanalyticalmethodverification
AT smabdurrahman transitionmetalcomplexesofnaproxensynthesischaracterizationforceddegradationstudiesandanalyticalmethodverification