Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties

Increasing cancer mortality statistics demand more accurate and efficient treatments. Nanostructures have proved to be promising choices in this regard. Nanotubes with large surface areas can play multiple roles from drug carriers in targeted drug delivery to beam absorbers in the photothermal metho...

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Main Authors: Sara Mashhoun, Ali Tavahodi
Format: Article
Language:English
Published: Frontiers Media S.A. 2024-11-01
Series:Frontiers in Nanotechnology
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Online Access:https://www.frontiersin.org/articles/10.3389/fnano.2024.1483044/full
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author Sara Mashhoun
Ali Tavahodi
author_facet Sara Mashhoun
Ali Tavahodi
author_sort Sara Mashhoun
collection DOAJ
description Increasing cancer mortality statistics demand more accurate and efficient treatments. Nanostructures have proved to be promising choices in this regard. Nanotubes with large surface areas can play multiple roles from drug carriers in targeted drug delivery to beam absorbers in the photothermal method. While carbon nanotubes (CNTs) show cytotoxicity, Boron Nitride Nanotubes (BNNTs) offer wide bandgap and biocompatibility. In this study, we investigate the electronic and solvation properties of (5,5), (6,6), and (7,7) BNNTs computationally by the density functional theory. For multimodal therapy, we considered Iron (Fe) doping in the BNNT, which can be helpful in hyperthermia due to the magnetic moment of Fe. Our results show that doping has improved the band positions. Furthermore, we implemented an organic anticancer molecule, genistein, a metastasis inhibitor. All potent configurations connecting genistein with BNNT covalently demonstrated enhanced water solubility as compared to pristine and Fe-doped BNNTs. The results suggest that the (7,7) C3 complex is the most stable structure and the best drug carrier.
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institution Kabale University
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spelling doaj-art-6d5e1a2b030040a59e60074e4d31a9eb2024-11-15T04:46:25ZengFrontiers Media S.A.Frontiers in Nanotechnology2673-30132024-11-01610.3389/fnano.2024.14830441483044Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility propertiesSara MashhounAli TavahodiIncreasing cancer mortality statistics demand more accurate and efficient treatments. Nanostructures have proved to be promising choices in this regard. Nanotubes with large surface areas can play multiple roles from drug carriers in targeted drug delivery to beam absorbers in the photothermal method. While carbon nanotubes (CNTs) show cytotoxicity, Boron Nitride Nanotubes (BNNTs) offer wide bandgap and biocompatibility. In this study, we investigate the electronic and solvation properties of (5,5), (6,6), and (7,7) BNNTs computationally by the density functional theory. For multimodal therapy, we considered Iron (Fe) doping in the BNNT, which can be helpful in hyperthermia due to the magnetic moment of Fe. Our results show that doping has improved the band positions. Furthermore, we implemented an organic anticancer molecule, genistein, a metastasis inhibitor. All potent configurations connecting genistein with BNNT covalently demonstrated enhanced water solubility as compared to pristine and Fe-doped BNNTs. The results suggest that the (7,7) C3 complex is the most stable structure and the best drug carrier.https://www.frontiersin.org/articles/10.3389/fnano.2024.1483044/fullboron nitride nanotubes (BNNTs)nanocarrier-based cancer therapydensity functional theory (DFT)genisteindopingelectronic properties
spellingShingle Sara Mashhoun
Ali Tavahodi
Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
Frontiers in Nanotechnology
boron nitride nanotubes (BNNTs)
nanocarrier-based cancer therapy
density functional theory (DFT)
genistein
doping
electronic properties
title Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
title_full Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
title_fullStr Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
title_full_unstemmed Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
title_short Boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment: A DFT study of electronic and solubility properties
title_sort boron nitride nanotubes as carriers of genistein for multitherapeutic cancer treatment a dft study of electronic and solubility properties
topic boron nitride nanotubes (BNNTs)
nanocarrier-based cancer therapy
density functional theory (DFT)
genistein
doping
electronic properties
url https://www.frontiersin.org/articles/10.3389/fnano.2024.1483044/full
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