Strong absorption in ultra-wide band by surface nano engineering of metallic glass

Broadband light absorption is important for applications such as infrared detectors, solar energy collectors, and photothermal conversion. We propose a facile and common strategy to fabricate light absorbers with strong ultra-wideband absorption. Due to their excellent thermoplastic forming ability,...

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Main Authors: Jianan Fu, Xin Li, Zhen Li, Fei Sun, Wenxin Wen, Jinlai Zhao, Wenqing Ruan, Shuai Ren, Zhenxuan Zhang, Xiong Liang, Jiang Ma
Format: Article
Language:English
Published: KeAi Communications Co. Ltd. 2025-01-01
Series:Fundamental Research
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Online Access:http://www.sciencedirect.com/science/article/pii/S2667325822003831
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author Jianan Fu
Xin Li
Zhen Li
Fei Sun
Wenxin Wen
Jinlai Zhao
Wenqing Ruan
Shuai Ren
Zhenxuan Zhang
Xiong Liang
Jiang Ma
author_facet Jianan Fu
Xin Li
Zhen Li
Fei Sun
Wenxin Wen
Jinlai Zhao
Wenqing Ruan
Shuai Ren
Zhenxuan Zhang
Xiong Liang
Jiang Ma
author_sort Jianan Fu
collection DOAJ
description Broadband light absorption is important for applications such as infrared detectors, solar energy collectors, and photothermal conversion. We propose a facile and common strategy to fabricate light absorbers with strong ultra-wideband absorption. Due to their excellent thermoplastic forming ability, metallic glasses could be patterned into finely arranged nanowire arrays, which show extremely low reflectivity (∼0.6%) in the visible and near-infrared regimes, and a low reflectivity (∼15%) in the mid-infrared regime as caused by multiscale nano spacing, multiple reflections, and plasmonic behavior. The strong absorption at surfaces with nanowires provides excellent photothermal conversion properties. The photothermal properties show that a surface with nanowires can be rapidly heated up to ∼160 °C at a rate of 28.75 °C/s, which is 30 times higher than smooth surfaces. Meanwhile, a surface with nanowires shows a high photothermal conversion efficiency (ηPT = 56.36%). The fabricated metallic glass absorbers exhibit adaptability as they can be easily formed into various complex shapes and meet the requirements under harsh conditions. The outcomes of our research open the door to manufacturing high-performance absorbers for applications in photothermal electric power generation, desalination, and photodetectors.
format Article
id doaj-art-6cdfa4984dd545b59725602bbfeabe59
institution Kabale University
issn 2667-3258
language English
publishDate 2025-01-01
publisher KeAi Communications Co. Ltd.
record_format Article
series Fundamental Research
spelling doaj-art-6cdfa4984dd545b59725602bbfeabe592025-01-29T05:02:28ZengKeAi Communications Co. Ltd.Fundamental Research2667-32582025-01-0151307314Strong absorption in ultra-wide band by surface nano engineering of metallic glassJianan Fu0Xin Li1Zhen Li2Fei Sun3Wenxin Wen4Jinlai Zhao5Wenqing Ruan6Shuai Ren7Zhenxuan Zhang8Xiong Liang9Jiang Ma10Shenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaCollege of Materials Science and Engineering, Shenzhen Key Laboratory of Polymer Science and Technology, Guangdong Research Center for Interfacial Engineering of Functional Materials, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, ChinaShenzhen Key Laboratory of High Performance Nontraditional Manufacturing, College of Mechatronics and Control Engineering, Shenzhen University, Shenzhen 518060, China; Corresponding author.Broadband light absorption is important for applications such as infrared detectors, solar energy collectors, and photothermal conversion. We propose a facile and common strategy to fabricate light absorbers with strong ultra-wideband absorption. Due to their excellent thermoplastic forming ability, metallic glasses could be patterned into finely arranged nanowire arrays, which show extremely low reflectivity (∼0.6%) in the visible and near-infrared regimes, and a low reflectivity (∼15%) in the mid-infrared regime as caused by multiscale nano spacing, multiple reflections, and plasmonic behavior. The strong absorption at surfaces with nanowires provides excellent photothermal conversion properties. The photothermal properties show that a surface with nanowires can be rapidly heated up to ∼160 °C at a rate of 28.75 °C/s, which is 30 times higher than smooth surfaces. Meanwhile, a surface with nanowires shows a high photothermal conversion efficiency (ηPT = 56.36%). The fabricated metallic glass absorbers exhibit adaptability as they can be easily formed into various complex shapes and meet the requirements under harsh conditions. The outcomes of our research open the door to manufacturing high-performance absorbers for applications in photothermal electric power generation, desalination, and photodetectors.http://www.sciencedirect.com/science/article/pii/S2667325822003831Metallic glassNanoformingUltra-wideband absorptionPhotothermal propertiesThermoplastic forming
spellingShingle Jianan Fu
Xin Li
Zhen Li
Fei Sun
Wenxin Wen
Jinlai Zhao
Wenqing Ruan
Shuai Ren
Zhenxuan Zhang
Xiong Liang
Jiang Ma
Strong absorption in ultra-wide band by surface nano engineering of metallic glass
Fundamental Research
Metallic glass
Nanoforming
Ultra-wideband absorption
Photothermal properties
Thermoplastic forming
title Strong absorption in ultra-wide band by surface nano engineering of metallic glass
title_full Strong absorption in ultra-wide band by surface nano engineering of metallic glass
title_fullStr Strong absorption in ultra-wide band by surface nano engineering of metallic glass
title_full_unstemmed Strong absorption in ultra-wide band by surface nano engineering of metallic glass
title_short Strong absorption in ultra-wide band by surface nano engineering of metallic glass
title_sort strong absorption in ultra wide band by surface nano engineering of metallic glass
topic Metallic glass
Nanoforming
Ultra-wideband absorption
Photothermal properties
Thermoplastic forming
url http://www.sciencedirect.com/science/article/pii/S2667325822003831
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