Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate

ABSTRACT Using soft chemistry methods, solid solutions of BaTi1‐xZrxO3 with 0 ≤ x ≤ 1 were obtained. The phase nature and features of the perovskite crystalline structure were established by x‐ray analysis and Fourier transform infrared (FTIR) spectroscopy. It was found that the average particle siz...

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Main Authors: Mohamed M. Salem, Aseel M. Altarawneh, Yamen A. Alibwaini, Ryad Ghazy, Osama M. Hemeda, Di Zhou, Moustafa A. Darwish, M. Khalid Hossain, Daria I. Tishkevich, Tatiana I. Zubar, Ekaterina L. Trukhanova, Alex V. Trukhanov, Sergei V. Trukhanov, Maha Mostafa
Format: Article
Language:English
Published: Wiley-VCH 2025-05-01
Series:Nano Select
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Online Access:https://doi.org/10.1002/nano.202300173
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author Mohamed M. Salem
Aseel M. Altarawneh
Yamen A. Alibwaini
Ryad Ghazy
Osama M. Hemeda
Di Zhou
Moustafa A. Darwish
M. Khalid Hossain
Daria I. Tishkevich
Tatiana I. Zubar
Ekaterina L. Trukhanova
Alex V. Trukhanov
Sergei V. Trukhanov
Maha Mostafa
author_facet Mohamed M. Salem
Aseel M. Altarawneh
Yamen A. Alibwaini
Ryad Ghazy
Osama M. Hemeda
Di Zhou
Moustafa A. Darwish
M. Khalid Hossain
Daria I. Tishkevich
Tatiana I. Zubar
Ekaterina L. Trukhanova
Alex V. Trukhanov
Sergei V. Trukhanov
Maha Mostafa
author_sort Mohamed M. Salem
collection DOAJ
description ABSTRACT Using soft chemistry methods, solid solutions of BaTi1‐xZrxO3 with 0 ≤ x ≤ 1 were obtained. The phase nature and features of the perovskite crystalline structure were established by x‐ray analysis and Fourier transform infrared (FTIR) spectroscopy. It was found that the average particle size increases with increasing content of zirconium cations. The average size of the crystallites, which are mostly irregular in shape and closely connected, is ∼43 nm. The d33 piezoelectric coefficient decreases while the concentration of zirconium cations increases. It is interesting to note that the residual polarization very strongly depends on the average crystallite size and, on the contrary, increases with increasing concentration of zirconium cations. The discovered behavior can be used in the design and production of electrostatic read‐only memory devices.
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issn 2688-4011
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series Nano Select
spelling doaj-art-6b52ef73e7394d10b8797b7af828bdbe2025-08-20T02:15:30ZengWiley-VCHNano Select2688-40112025-05-0165n/an/a10.1002/nano.202300173Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium TitanateMohamed M. Salem0Aseel M. Altarawneh1Yamen A. Alibwaini2Ryad Ghazy3Osama M. Hemeda4Di Zhou5Moustafa A. Darwish6M. Khalid Hossain7Daria I. Tishkevich8Tatiana I. Zubar9Ekaterina L. Trukhanova10Alex V. Trukhanov11Sergei V. Trukhanov12Maha Mostafa13Physics Department Faculty of Science Tanta University Tanta EgyptPhysics Department Faculty of Science Tanta University Tanta EgyptPhysics Department Faculty of Science Tanta University Tanta EgyptPhysics Department Faculty of Science Tanta University Tanta EgyptPhysics Department Faculty of Science Tanta University Tanta EgyptElectronic Materials Research Laboratory School of Electronic Science and Engineering Key Laboratory of the Ministry of Education & International Center for Dielectric Research Xi'an Jiaotong University Xi'an ChinaPhysics Department Faculty of Science Tanta University Tanta EgyptInstitute of Electronics, Atomic Energy Research Establishment Bangladesh Atomic Energy Commission Dhaka BangladeshLaboratory of Magnetic Films Physics SSPA “Scientific and Practical Materials Research Centre of NAS of Belarus” Minsk BelarusLaboratory of Magnetic Films Physics SSPA “Scientific and Practical Materials Research Centre of NAS of Belarus” Minsk BelarusLaboratory of Magnetic Films Physics SSPA “Scientific and Practical Materials Research Centre of NAS of Belarus” Minsk BelarusLaboratory of Magnetic Films Physics SSPA “Scientific and Practical Materials Research Centre of NAS of Belarus” Minsk BelarusLaboratory of Magnetic Films Physics SSPA “Scientific and Practical Materials Research Centre of NAS of Belarus” Minsk BelarusPhysics Department Faculty of Science Tanta University Tanta EgyptABSTRACT Using soft chemistry methods, solid solutions of BaTi1‐xZrxO3 with 0 ≤ x ≤ 1 were obtained. The phase nature and features of the perovskite crystalline structure were established by x‐ray analysis and Fourier transform infrared (FTIR) spectroscopy. It was found that the average particle size increases with increasing content of zirconium cations. The average size of the crystallites, which are mostly irregular in shape and closely connected, is ∼43 nm. The d33 piezoelectric coefficient decreases while the concentration of zirconium cations increases. It is interesting to note that the residual polarization very strongly depends on the average crystallite size and, on the contrary, increases with increasing concentration of zirconium cations. The discovered behavior can be used in the design and production of electrostatic read‐only memory devices.https://doi.org/10.1002/nano.202300173doped titanatesferroelectricsperovskitespiezoelectricssoft chemistry methods
spellingShingle Mohamed M. Salem
Aseel M. Altarawneh
Yamen A. Alibwaini
Ryad Ghazy
Osama M. Hemeda
Di Zhou
Moustafa A. Darwish
M. Khalid Hossain
Daria I. Tishkevich
Tatiana I. Zubar
Ekaterina L. Trukhanova
Alex V. Trukhanov
Sergei V. Trukhanov
Maha Mostafa
Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
Nano Select
doped titanates
ferroelectrics
perovskites
piezoelectrics
soft chemistry methods
title Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
title_full Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
title_fullStr Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
title_full_unstemmed Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
title_short Effect of Zr Doping on Structure and Ferroelectric Properties of Nanostructured Barium Titanate
title_sort effect of zr doping on structure and ferroelectric properties of nanostructured barium titanate
topic doped titanates
ferroelectrics
perovskites
piezoelectrics
soft chemistry methods
url https://doi.org/10.1002/nano.202300173
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