Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy

This study focuses on the synthesis of sugar decorated porphyrins and their gold nanoparticle conjugates as photosensitizers for photodynamic therapy (PDT). Linking the sugar to the porphyrins imparted water solubility to the latter. The conjugation to sugar molecules enhanced the singlet oxygen qua...

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Main Authors: Thembani Silas Vukeya, Refilwe Matshitse, John Mack, Yolande Openda, Earl Prinsloo, Tebello Nyokong
Format: Article
Language:English
Published: Elsevier 2025-08-01
Series:Photodiagnosis and Photodynamic Therapy
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1572100025001905
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author Thembani Silas Vukeya
Refilwe Matshitse
John Mack
Yolande Openda
Earl Prinsloo
Tebello Nyokong
author_facet Thembani Silas Vukeya
Refilwe Matshitse
John Mack
Yolande Openda
Earl Prinsloo
Tebello Nyokong
author_sort Thembani Silas Vukeya
collection DOAJ
description This study focuses on the synthesis of sugar decorated porphyrins and their gold nanoparticle conjugates as photosensitizers for photodynamic therapy (PDT). Linking the sugar to the porphyrins imparted water solubility to the latter. The conjugation to sugar molecules enhanced the singlet oxygen quantum yield and improved the cellular uptake and therefore, their phototoxicity in some cases. The porphyrins (with or without the sugar) were linked to the Au nanoparticles (AuNPs). The activity of the synthesized complexes and conjugates with AuNPs were tested against the MDA-MB-231 breast cancer cells using the resazurin assay to monitor the cell viability. The conjugate of In porphyrin with AuNPs showed the highest PDT activity.
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institution Kabale University
issn 1572-1000
language English
publishDate 2025-08-01
publisher Elsevier
record_format Article
series Photodiagnosis and Photodynamic Therapy
spelling doaj-art-6b1e771cad3448cc892c26ea711c8a312025-08-20T04:00:40ZengElsevierPhotodiagnosis and Photodynamic Therapy1572-10002025-08-015410465810.1016/j.pdpdt.2025.104658Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapyThembani Silas Vukeya0Refilwe Matshitse1John Mack2Yolande Openda3Earl Prinsloo4Tebello Nyokong5Institute for Nanotechnology Innovation, Rhodes University, Makhanda, South AfricaInstitute for Nanotechnology Innovation, Rhodes University, Makhanda, South AfricaInstitute for Nanotechnology Innovation, Rhodes University, Makhanda, South AfricaInstitute for Nanotechnology Innovation, Rhodes University, Makhanda, South AfricaBiotechnology Innovation Centre, Rhodes University, Makhanda, South AfricaInstitute for Nanotechnology Innovation, Rhodes University, Makhanda, South Africa; Corresponding author.This study focuses on the synthesis of sugar decorated porphyrins and their gold nanoparticle conjugates as photosensitizers for photodynamic therapy (PDT). Linking the sugar to the porphyrins imparted water solubility to the latter. The conjugation to sugar molecules enhanced the singlet oxygen quantum yield and improved the cellular uptake and therefore, their phototoxicity in some cases. The porphyrins (with or without the sugar) were linked to the Au nanoparticles (AuNPs). The activity of the synthesized complexes and conjugates with AuNPs were tested against the MDA-MB-231 breast cancer cells using the resazurin assay to monitor the cell viability. The conjugate of In porphyrin with AuNPs showed the highest PDT activity.http://www.sciencedirect.com/science/article/pii/S1572100025001905Photodynamic therapyPhotosensitizerReactive oxygen speciesSinglet oxygenGold nanoparticlesSugar
spellingShingle Thembani Silas Vukeya
Refilwe Matshitse
John Mack
Yolande Openda
Earl Prinsloo
Tebello Nyokong
Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
Photodiagnosis and Photodynamic Therapy
Photodynamic therapy
Photosensitizer
Reactive oxygen species
Singlet oxygen
Gold nanoparticles
Sugar
title Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
title_full Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
title_fullStr Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
title_full_unstemmed Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
title_short Effects of central metals on sugar decorated tetrakis-(4-methylthiophenyl) porphyrin considered for use in photodynamic therapy
title_sort effects of central metals on sugar decorated tetrakis 4 methylthiophenyl porphyrin considered for use in photodynamic therapy
topic Photodynamic therapy
Photosensitizer
Reactive oxygen species
Singlet oxygen
Gold nanoparticles
Sugar
url http://www.sciencedirect.com/science/article/pii/S1572100025001905
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