Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS

An evaluation of the extraction of multiresidue pesticides from palm oil by liquid-liquid extraction/low-temperature purification (LLE/LTP) coupled with dispersive solid-phase extraction (d-SPE) as the cleanup procedure with the determination by liquid chromatography mass spectrometry using electros...

Full description

Saved in:
Bibliographic Details
Main Authors: Elham Sobhanzadeh, Keivan Nemati
Format: Article
Language:English
Published: Wiley 2013-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2013/915048
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850158267270955008
author Elham Sobhanzadeh
Keivan Nemati
author_facet Elham Sobhanzadeh
Keivan Nemati
author_sort Elham Sobhanzadeh
collection DOAJ
description An evaluation of the extraction of multiresidue pesticides from palm oil by liquid-liquid extraction/low-temperature purification (LLE/LTP) coupled with dispersive solid-phase extraction (d-SPE) as the cleanup procedure with the determination by liquid chromatography mass spectrometry using electrospray as the ionization source (LC-ESI-MS) was carried out. Optimization approaches were studied in terms of d-SPE to select efficiency of type and mass of adsorbents to obtain the highest recovery yield of pesticides and the lowest coextract fat residues in the final extract. The optimal conditions of d-SPE were obtained using 3 g of palm oil, 4 g anhydrous MgSO4, 150 mg of PSA, and 50 mg of GCB (PSA: GCB (3 : 1 w/w)). Recovery study was performed at three concentration levels (25, 50, and 100 ng kg−1), yielding recovery rates between 71.8 and 112.4% except diuron with relative standard deviations of 3.2–15.1%. Detection and quantification limits were lower than 2.7 and 8.2 ng kg−1, respectively. The proposed method was successfully applied to the analysis of market-purchased palm oil samples from two different brands collected in Kuala Lumpur, showing its potential applicability and revealing the presence of some of the target species in the ng g−1 range.
format Article
id doaj-art-6b1beeef37cc41579e9b6a3950d112f0
institution OA Journals
issn 2090-9063
2090-9071
language English
publishDate 2013-01-01
publisher Wiley
record_format Article
series Journal of Chemistry
spelling doaj-art-6b1beeef37cc41579e9b6a3950d112f02025-08-20T02:23:56ZengWileyJournal of Chemistry2090-90632090-90712013-01-01201310.1155/2013/915048915048Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MSElham Sobhanzadeh0Keivan Nemati1Department of Chemistry, Islamic Azad University, Masjed-Soliman Branch, Masjed-Soliman, IranDepartment of Chemistry, Islamic Azad University, Masjed-Soliman Branch, Masjed-Soliman, IranAn evaluation of the extraction of multiresidue pesticides from palm oil by liquid-liquid extraction/low-temperature purification (LLE/LTP) coupled with dispersive solid-phase extraction (d-SPE) as the cleanup procedure with the determination by liquid chromatography mass spectrometry using electrospray as the ionization source (LC-ESI-MS) was carried out. Optimization approaches were studied in terms of d-SPE to select efficiency of type and mass of adsorbents to obtain the highest recovery yield of pesticides and the lowest coextract fat residues in the final extract. The optimal conditions of d-SPE were obtained using 3 g of palm oil, 4 g anhydrous MgSO4, 150 mg of PSA, and 50 mg of GCB (PSA: GCB (3 : 1 w/w)). Recovery study was performed at three concentration levels (25, 50, and 100 ng kg−1), yielding recovery rates between 71.8 and 112.4% except diuron with relative standard deviations of 3.2–15.1%. Detection and quantification limits were lower than 2.7 and 8.2 ng kg−1, respectively. The proposed method was successfully applied to the analysis of market-purchased palm oil samples from two different brands collected in Kuala Lumpur, showing its potential applicability and revealing the presence of some of the target species in the ng g−1 range.http://dx.doi.org/10.1155/2013/915048
spellingShingle Elham Sobhanzadeh
Keivan Nemati
Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
Journal of Chemistry
title Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
title_full Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
title_fullStr Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
title_full_unstemmed Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
title_short Liquid-Liquid Extraction/Low-Temperature Purification (LLE/LTP) Followed by Dispersive Solid-Phase Extraction (d-SPE) Cleanup for Multiresidue Analysis in Palm Oil by LC-QTOF-MS
title_sort liquid liquid extraction low temperature purification lle ltp followed by dispersive solid phase extraction d spe cleanup for multiresidue analysis in palm oil by lc qtof ms
url http://dx.doi.org/10.1155/2013/915048
work_keys_str_mv AT elhamsobhanzadeh liquidliquidextractionlowtemperaturepurificationlleltpfollowedbydispersivesolidphaseextractiondspecleanupformultiresidueanalysisinpalmoilbylcqtofms
AT keivannemati liquidliquidextractionlowtemperaturepurificationlleltpfollowedbydispersivesolidphaseextractiondspecleanupformultiresidueanalysisinpalmoilbylcqtofms