Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges
Solid-state lithium batteries exhibit high-energy density and exceptional safety performance, thereby enabling an extended driving range for electric vehicles in the future. Solid-state electrolytes (SSEs) are the key materials in solid-state batteries that guarantee the safety performance of the ba...
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| Format: | Article |
| Language: | English |
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MDPI AG
2024-11-01
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| Series: | Nanomaterials |
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| Online Access: | https://www.mdpi.com/2079-4991/14/22/1773 |
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| author | Shun Ai Xianli Wu Jintao Wang Xu Li Xiaofeng Hao Yuezhong Meng |
| author_facet | Shun Ai Xianli Wu Jintao Wang Xu Li Xiaofeng Hao Yuezhong Meng |
| author_sort | Shun Ai |
| collection | DOAJ |
| description | Solid-state lithium batteries exhibit high-energy density and exceptional safety performance, thereby enabling an extended driving range for electric vehicles in the future. Solid-state electrolytes (SSEs) are the key materials in solid-state batteries that guarantee the safety performance of the battery. This review assesses the research progress on solid-state electrolytes, including polymers, inorganic compounds (oxides, sulfides, halides), and organic–inorganic composites, the challenges related to solid-state batteries in terms of their interfaces, and the status of industrialization research on solid-state electrolytes. For each kind of solid-state electrolytes, details on the preparation, properties, composition, ionic conductivity, ionic migration mechanism, and structure–activity relationship, are collected. For the challenges faced by solid-state batteries, the high interfacial resistance, the side reactions between solid-state electrolytes and electrodes, and interface instability, are mainly discussed. The current industrialization research status of various solid electrolytes is analyzed in regard to relevant enterprises from different countries. Finally, the potential development directions and prospects of high-energy density solid-state batteries are discussed. This review provides a comprehensive reference for SSE researchers and paves the way for innovative advancements in regard to solid-state lithium batteries. |
| format | Article |
| id | doaj-art-6af4fcaf76e944df859c0ae86b9fe3e6 |
| institution | OA Journals |
| issn | 2079-4991 |
| language | English |
| publishDate | 2024-11-01 |
| publisher | MDPI AG |
| record_format | Article |
| series | Nanomaterials |
| spelling | doaj-art-6af4fcaf76e944df859c0ae86b9fe3e62025-08-20T01:54:08ZengMDPI AGNanomaterials2079-49912024-11-011422177310.3390/nano14221773Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial ChallengesShun Ai0Xianli Wu1Jintao Wang2Xu Li3Xiaofeng Hao4Yuezhong Meng5School of Materials Science and Engineering & College of Chemistry, Zhengzhou University, Zhengzhou 450001, ChinaSchool of Materials Science and Engineering & College of Chemistry, Zhengzhou University, Zhengzhou 450001, ChinaSchool of Materials Science and Engineering & College of Chemistry, Zhengzhou University, Zhengzhou 450001, ChinaInstitute of Chemistry, Henan Academy of Sciences, Zhengzhou 450046, ChinaInstitute of Chemistry, Henan Academy of Sciences, Zhengzhou 450046, ChinaSchool of Materials Science and Engineering & College of Chemistry, Zhengzhou University, Zhengzhou 450001, ChinaSolid-state lithium batteries exhibit high-energy density and exceptional safety performance, thereby enabling an extended driving range for electric vehicles in the future. Solid-state electrolytes (SSEs) are the key materials in solid-state batteries that guarantee the safety performance of the battery. This review assesses the research progress on solid-state electrolytes, including polymers, inorganic compounds (oxides, sulfides, halides), and organic–inorganic composites, the challenges related to solid-state batteries in terms of their interfaces, and the status of industrialization research on solid-state electrolytes. For each kind of solid-state electrolytes, details on the preparation, properties, composition, ionic conductivity, ionic migration mechanism, and structure–activity relationship, are collected. For the challenges faced by solid-state batteries, the high interfacial resistance, the side reactions between solid-state electrolytes and electrodes, and interface instability, are mainly discussed. The current industrialization research status of various solid electrolytes is analyzed in regard to relevant enterprises from different countries. Finally, the potential development directions and prospects of high-energy density solid-state batteries are discussed. This review provides a comprehensive reference for SSE researchers and paves the way for innovative advancements in regard to solid-state lithium batteries.https://www.mdpi.com/2079-4991/14/22/1773solid-state electrolytesinterfacial challengesindustrialization research status |
| spellingShingle | Shun Ai Xianli Wu Jintao Wang Xu Li Xiaofeng Hao Yuezhong Meng Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges Nanomaterials solid-state electrolytes interfacial challenges industrialization research status |
| title | Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges |
| title_full | Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges |
| title_fullStr | Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges |
| title_full_unstemmed | Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges |
| title_short | Research Progress on Solid-State Electrolytes in Solid-State Lithium Batteries: Classification, Ionic Conductive Mechanism, Interfacial Challenges |
| title_sort | research progress on solid state electrolytes in solid state lithium batteries classification ionic conductive mechanism interfacial challenges |
| topic | solid-state electrolytes interfacial challenges industrialization research status |
| url | https://www.mdpi.com/2079-4991/14/22/1773 |
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