Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)

The recently discovered nonmevalonate pathway of isoprenoid biosynthesis Is a prospective target in screening of new antibiotics. Because of the absence of the pathway in the animal cells, the specific inhibitors of the pathway will be a new class of antibiotics against many pathogens (which cause e...

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Main Authors: YU. V. Ershov, K. V. Mazikin, D. N. Ostrovsky
Format: Article
Language:Russian
Published: LLC "Publishing House OKI" 2020-05-01
Series:Антибиотики и Химиотерапия
Subjects:
Online Access:https://www.antibiotics-chemotherapy.ru/jour/article/view/303
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author YU. V. Ershov
K. V. Mazikin
D. N. Ostrovsky
author_facet YU. V. Ershov
K. V. Mazikin
D. N. Ostrovsky
author_sort YU. V. Ershov
collection DOAJ
description The recently discovered nonmevalonate pathway of isoprenoid biosynthesis Is a prospective target in screening of new antibiotics. Because of the absence of the pathway in the animal cells, the specific inhibitors of the pathway will be a new class of antibiotics against many pathogens (which cause e.g. malaria, tuberculosis, etc), combining high efficiency and low toxicity. Several derivatives of 2-C-methyl-D-erythritol-2,4-cyclodiphosphate (MEC) were synthesized. 4-Phospho-methyl-D-erythritol-1,2-cyclophosphate, benzyl ether and benzyliden derivative of MEC inhibited the14C-MEC incorporation into isoprenoids of chromoplasts from red pepper with IC50 of 1.7-5 мМ. Some inhibition (about 10 %) was also observed with the use of dimethyl ether and isopropyliden derivative of MEC.
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series Антибиотики и Химиотерапия
spelling doaj-art-6a90ff74fc6543818f8592d612e2a4e62025-08-20T03:20:37ZrusLLC "Publishing House OKI"Антибиотики и Химиотерапия0235-29902020-05-01555-637302Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)YU. V. Ershov0K. V. Mazikin1D. N. Ostrovsky2A. N. Bakh Institute of BiochemistryA. N. Bakh Institute of BiochemistryA. N. Bakh Institute of BiochemistryThe recently discovered nonmevalonate pathway of isoprenoid biosynthesis Is a prospective target in screening of new antibiotics. Because of the absence of the pathway in the animal cells, the specific inhibitors of the pathway will be a new class of antibiotics against many pathogens (which cause e.g. malaria, tuberculosis, etc), combining high efficiency and low toxicity. Several derivatives of 2-C-methyl-D-erythritol-2,4-cyclodiphosphate (MEC) were synthesized. 4-Phospho-methyl-D-erythritol-1,2-cyclophosphate, benzyl ether and benzyliden derivative of MEC inhibited the14C-MEC incorporation into isoprenoids of chromoplasts from red pepper with IC50 of 1.7-5 мМ. Some inhibition (about 10 %) was also observed with the use of dimethyl ether and isopropyliden derivative of MEC.https://www.antibiotics-chemotherapy.ru/jour/article/view/303antibiotics screeningisoprenoid biosynthesis inhibitors
spellingShingle YU. V. Ershov
K. V. Mazikin
D. N. Ostrovsky
Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
Антибиотики и Химиотерапия
antibiotics screening
isoprenoid biosynthesis inhibitors
title Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
title_full Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
title_fullStr Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
title_full_unstemmed Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
title_short Screening of Potential Antibiotics, Inhibitors of the Nonmevalonate Pathway of Isoprenoid Biosynthesis (2-C-Methyl-D-Erythritol-2,4-Cyclodiphosphate Derivatives)
title_sort screening of potential antibiotics inhibitors of the nonmevalonate pathway of isoprenoid biosynthesis 2 c methyl d erythritol 2 4 cyclodiphosphate derivatives
topic antibiotics screening
isoprenoid biosynthesis inhibitors
url https://www.antibiotics-chemotherapy.ru/jour/article/view/303
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AT kvmazikin screeningofpotentialantibioticsinhibitorsofthenonmevalonatepathwayofisoprenoidbiosynthesis2cmethylderythritol24cyclodiphosphatederivatives
AT dnostrovsky screeningofpotentialantibioticsinhibitorsofthenonmevalonatepathwayofisoprenoidbiosynthesis2cmethylderythritol24cyclodiphosphatederivatives