Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis

Background/Objectives: Since the emergence of the COVID-19 pandemic caused by severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2), the discovery of compounds with antiviral potential from medicinal plants has been extensively researched. This study aimed to investigate plant metabolites wit...

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Main Authors: Brendo Araujo Gomes, Diégina Araújo Fernandes, Thamirys Silva da Fonseca, Mariana Freire Campos, Patrícia Alves Jural, Marcos Vinicius Toledo e Silva, Larissa Esteves Carvalho Constant, Andrex Augusto Silva da Veiga, Beatriz Ribeiro Ferreira, Ellen Santos Magalhães, Hagatha Bento Mendonça Pereira, Beatriz Graziela Martins de Mattos, Beatriz Albuquerque Custódio de Oliveira, Stephany da Silva Costa, Flavia Maria Mendonça do Amaral, Danilo Ribeiro de Oliveira, Ivana Correa Ramos Leal, Gabriel Rocha Martins, Gilda Guimarães Leitão, Diego Allonso, Simony Carvalho Mendonça, Marcus Tullius Scotti, Suzana Guimarães Leitão
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Language:English
Published: MDPI AG 2025-06-01
Series:Drugs and Drug Candidates
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Online Access:https://www.mdpi.com/2813-2998/4/2/27
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author Brendo Araujo Gomes
Diégina Araújo Fernandes
Thamirys Silva da Fonseca
Mariana Freire Campos
Patrícia Alves Jural
Marcos Vinicius Toledo e Silva
Larissa Esteves Carvalho Constant
Andrex Augusto Silva da Veiga
Beatriz Ribeiro Ferreira
Ellen Santos Magalhães
Hagatha Bento Mendonça Pereira
Beatriz Graziela Martins de Mattos
Beatriz Albuquerque Custódio de Oliveira
Stephany da Silva Costa
Flavia Maria Mendonça do Amaral
Danilo Ribeiro de Oliveira
Ivana Correa Ramos Leal
Gabriel Rocha Martins
Gilda Guimarães Leitão
Diego Allonso
Simony Carvalho Mendonça
Marcus Tullius Scotti
Suzana Guimarães Leitão
author_facet Brendo Araujo Gomes
Diégina Araújo Fernandes
Thamirys Silva da Fonseca
Mariana Freire Campos
Patrícia Alves Jural
Marcos Vinicius Toledo e Silva
Larissa Esteves Carvalho Constant
Andrex Augusto Silva da Veiga
Beatriz Ribeiro Ferreira
Ellen Santos Magalhães
Hagatha Bento Mendonça Pereira
Beatriz Graziela Martins de Mattos
Beatriz Albuquerque Custódio de Oliveira
Stephany da Silva Costa
Flavia Maria Mendonça do Amaral
Danilo Ribeiro de Oliveira
Ivana Correa Ramos Leal
Gabriel Rocha Martins
Gilda Guimarães Leitão
Diego Allonso
Simony Carvalho Mendonça
Marcus Tullius Scotti
Suzana Guimarães Leitão
author_sort Brendo Araujo Gomes
collection DOAJ
description Background/Objectives: Since the emergence of the COVID-19 pandemic caused by severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2), the discovery of compounds with antiviral potential from medicinal plants has been extensively researched. This study aimed to investigate plant metabolites with in vitro inhibitory potential against SARS-CoV-2 targets, including 3CL<sub>pro</sub>, PL<sub>pro</sub>, Spike protein, and RdRp. Methods: A systematic review was conducted following PRISMA guidelines, with literature searches performed in six electronic databases (Scielo, ScienceDirect, Scopus, Springer, Web of Science, and PubMed) from January 2020 to February 2024. Computational analyses using SwissADME, pkCSM, ADMETlab, ProTox3, Toxtree, and DataWarrior were performed to predict the absorption, distribution, metabolism, excretion, and toxicity (ADMET) profiles as well as other medicinal chemistry parameters of these compounds. Results: A total of 330 plant-derived compounds with inhibitory activities against the proposed targets were identified, with compounds showing IC<sub>50</sub> values as low as 0.01 μM. Our findings suggest that several plant metabolites exhibit significant in vitro inhibition of SARS-CoV-2 targets; however, few molecules exhibit drug development viability without further adjustments. Additionally, after these evaluations, two phenolic acids, salvianic acid A and protocatechuic acid methyl ester, stood out for their potential as candidates for developing antiviral therapies, with IC<sub>50</sub> values of 2.15 μM against 3CL<sub>pro</sub> and 3.76 μM against PL<sub>pro</sub>; respectively; and satisfactory in silico drug-likeness and ADMET profiles. Conclusions: These results reinforce the importance of plant metabolites as potential targets for antiviral drug discovery.
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spelling doaj-art-69b4e5afdf7c48c598e9d458103724252025-08-20T02:24:29ZengMDPI AGDrugs and Drug Candidates2813-29982025-06-01422710.3390/ddc4020027Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational AnalysisBrendo Araujo Gomes0Diégina Araújo Fernandes1Thamirys Silva da Fonseca2Mariana Freire Campos3Patrícia Alves Jural4Marcos Vinicius Toledo e Silva5Larissa Esteves Carvalho Constant6Andrex Augusto Silva da Veiga7Beatriz Ribeiro Ferreira8Ellen Santos Magalhães9Hagatha Bento Mendonça Pereira10Beatriz Graziela Martins de Mattos11Beatriz Albuquerque Custódio de Oliveira12Stephany da Silva Costa13Flavia Maria Mendonça do Amaral14Danilo Ribeiro de Oliveira15Ivana Correa Ramos Leal16Gabriel Rocha Martins17Gilda Guimarães Leitão18Diego Allonso19Simony Carvalho Mendonça20Marcus Tullius Scotti21Suzana Guimarães Leitão22Programa de Pós-Graduação em Biotecnologia Vegetal e Bioprocessos, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-902, RJ, BrazilInstituto de Pesquisas de Produtos Naturais, Universidade Federal do Rio de Janeiro, Centro de Ciências da Saúde, Rio de Janeiro 21941-902, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilPrograma de Pós-Graduação em Biotecnologia Vegetal e Bioprocessos, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-902, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilLaboratório de Biotecnologia e Bioengenharia Estrutural, Universidade Federal do Rio de Janeiro, Centro de Ciências da Saúde, Rio de Janeiro 21941-902, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilPrograma de Pós-Graduação em Biotecnologia Vegetal e Bioprocessos, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-902, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilLaboratório de Biotecnologia e Bioengenharia Estrutural, Universidade Federal do Rio de Janeiro, Centro de Ciências da Saúde, Rio de Janeiro 21941-902, RJ, BrazilLaboratório de Biotecnologia e Bioengenharia Estrutural, Universidade Federal do Rio de Janeiro, Centro de Ciências da Saúde, Rio de Janeiro 21941-902, RJ, BrazilDepartamento de Farmácia, Universidade Federal do Maranhão, São Luis 65085-580, MA, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Ciências Farmacêuticas, Departamento de Farmácia, Universidade de São Paulo, São Paulo 05508-900, SP, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilFaculdade de Farmácia, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-590, RJ, BrazilDepartamento de Química, Universidade Federal da Paraíba, João Pessoa 58051-970, PB, BrazilPrograma de Pós-Graduação em Biotecnologia Vegetal e Bioprocessos, Universidade Federal do Rio de Janeiro, Rio de Janeiro 21941-902, RJ, BrazilBackground/Objectives: Since the emergence of the COVID-19 pandemic caused by severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2), the discovery of compounds with antiviral potential from medicinal plants has been extensively researched. This study aimed to investigate plant metabolites with in vitro inhibitory potential against SARS-CoV-2 targets, including 3CL<sub>pro</sub>, PL<sub>pro</sub>, Spike protein, and RdRp. Methods: A systematic review was conducted following PRISMA guidelines, with literature searches performed in six electronic databases (Scielo, ScienceDirect, Scopus, Springer, Web of Science, and PubMed) from January 2020 to February 2024. Computational analyses using SwissADME, pkCSM, ADMETlab, ProTox3, Toxtree, and DataWarrior were performed to predict the absorption, distribution, metabolism, excretion, and toxicity (ADMET) profiles as well as other medicinal chemistry parameters of these compounds. Results: A total of 330 plant-derived compounds with inhibitory activities against the proposed targets were identified, with compounds showing IC<sub>50</sub> values as low as 0.01 μM. Our findings suggest that several plant metabolites exhibit significant in vitro inhibition of SARS-CoV-2 targets; however, few molecules exhibit drug development viability without further adjustments. Additionally, after these evaluations, two phenolic acids, salvianic acid A and protocatechuic acid methyl ester, stood out for their potential as candidates for developing antiviral therapies, with IC<sub>50</sub> values of 2.15 μM against 3CL<sub>pro</sub> and 3.76 μM against PL<sub>pro</sub>; respectively; and satisfactory in silico drug-likeness and ADMET profiles. Conclusions: These results reinforce the importance of plant metabolites as potential targets for antiviral drug discovery.https://www.mdpi.com/2813-2998/4/2/27natural products3CL<sub>pro</sub>PL<sub>pro</sub>Spike:ACE2RdRpADMET profiling
spellingShingle Brendo Araujo Gomes
Diégina Araújo Fernandes
Thamirys Silva da Fonseca
Mariana Freire Campos
Patrícia Alves Jural
Marcos Vinicius Toledo e Silva
Larissa Esteves Carvalho Constant
Andrex Augusto Silva da Veiga
Beatriz Ribeiro Ferreira
Ellen Santos Magalhães
Hagatha Bento Mendonça Pereira
Beatriz Graziela Martins de Mattos
Beatriz Albuquerque Custódio de Oliveira
Stephany da Silva Costa
Flavia Maria Mendonça do Amaral
Danilo Ribeiro de Oliveira
Ivana Correa Ramos Leal
Gabriel Rocha Martins
Gilda Guimarães Leitão
Diego Allonso
Simony Carvalho Mendonça
Marcus Tullius Scotti
Suzana Guimarães Leitão
Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
Drugs and Drug Candidates
natural products
3CL<sub>pro</sub>
PL<sub>pro</sub>
Spike:ACE2
RdRp
ADMET profiling
title Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
title_full Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
title_fullStr Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
title_full_unstemmed Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
title_short Plants Metabolites as In Vitro Inhibitors of SARS-CoV-2 Targets: A Systematic Review and Computational Analysis
title_sort plants metabolites as in vitro inhibitors of sars cov 2 targets a systematic review and computational analysis
topic natural products
3CL<sub>pro</sub>
PL<sub>pro</sub>
Spike:ACE2
RdRp
ADMET profiling
url https://www.mdpi.com/2813-2998/4/2/27
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