Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction

<i>Crataegus monogyna</i>, commonly known as hawthorn, is a valuable plant in pharmaceutical production. Its flowers, leaves, and fruits are rich in antioxidants. This study explores the application of pulsed electric field (PEF) for enhanced extraction of bioactive compounds from <i&...

Full description

Saved in:
Bibliographic Details
Main Authors: Vasiliki Papazidou, Ioannis Makrygiannis, Martha Mantiniotou, Vassilis Athanasiadis, Eleni Bozinou, Stavros I. Lalas
Format: Article
Language:English
Published: MDPI AG 2025-07-01
Series:Plants
Subjects:
Online Access:https://www.mdpi.com/2223-7747/14/15/2262
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849770638799011840
author Vasiliki Papazidou
Ioannis Makrygiannis
Martha Mantiniotou
Vassilis Athanasiadis
Eleni Bozinou
Stavros I. Lalas
author_facet Vasiliki Papazidou
Ioannis Makrygiannis
Martha Mantiniotou
Vassilis Athanasiadis
Eleni Bozinou
Stavros I. Lalas
author_sort Vasiliki Papazidou
collection DOAJ
description <i>Crataegus monogyna</i>, commonly known as hawthorn, is a valuable plant in pharmaceutical production. Its flowers, leaves, and fruits are rich in antioxidants. This study explores the application of pulsed electric field (PEF) for enhanced extraction of bioactive compounds from <i>C. monogyna</i> leaves. The liquid-to-solid ratio, solvent composition (ethanol, water, and 50% <i>v/v</i> aqueous ethanol), and key PEF parameters—including pulse duration, pulse period, electric field intensity, and treatment duration—were investigated during the optimization process. To determine the optimal extraction conditions and their impact on antioxidant activity, response surface methodology (RSM) with a six-factor design was employed. The total polyphenol content in the optimized extract was 244 mg gallic acid equivalents/g dry weight, while individual polyphenols were analyzed using high-performance liquid chromatography coupled with a diode array detector (HPLC-DAD). Furthermore, antioxidant activity was assessed using ferric-reducing antioxidant power (FRAP) and DPPH radical scavenging assays, yielding values of 3235 and 1850 μmol ascorbic acid equivalents/g dry weight, respectively. Additionally, correlation analyses were conducted to evaluate the interactions between bioactive compounds and antioxidant capacity. Compared to other extraction techniques, PEF stands out as an eco-friendly, non-thermal standalone method, offering a sustainable approach for the rapid production of health-promoting extracts from <i>C. monogyna</i> leaves.
format Article
id doaj-art-6861a9ca4de1459f807292d1275bbe95
institution DOAJ
issn 2223-7747
language English
publishDate 2025-07-01
publisher MDPI AG
record_format Article
series Plants
spelling doaj-art-6861a9ca4de1459f807292d1275bbe952025-08-20T03:02:56ZengMDPI AGPlants2223-77472025-07-011415226210.3390/plants14152262Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted ExtractionVasiliki Papazidou0Ioannis Makrygiannis1Martha Mantiniotou2Vassilis Athanasiadis3Eleni Bozinou4Stavros I. Lalas5Department of Chemical Engineering, University of Western Macedonia, 50100 Kozani, GreeceDepartment of Food Science and Nutrition, University of Thessaly, 43100 Karditsa, GreeceDepartment of Food Science and Nutrition, University of Thessaly, 43100 Karditsa, GreeceDepartment of Food Science and Nutrition, University of Thessaly, 43100 Karditsa, GreeceDepartment of Food Science and Nutrition, University of Thessaly, 43100 Karditsa, GreeceDepartment of Food Science and Nutrition, University of Thessaly, 43100 Karditsa, Greece<i>Crataegus monogyna</i>, commonly known as hawthorn, is a valuable plant in pharmaceutical production. Its flowers, leaves, and fruits are rich in antioxidants. This study explores the application of pulsed electric field (PEF) for enhanced extraction of bioactive compounds from <i>C. monogyna</i> leaves. The liquid-to-solid ratio, solvent composition (ethanol, water, and 50% <i>v/v</i> aqueous ethanol), and key PEF parameters—including pulse duration, pulse period, electric field intensity, and treatment duration—were investigated during the optimization process. To determine the optimal extraction conditions and their impact on antioxidant activity, response surface methodology (RSM) with a six-factor design was employed. The total polyphenol content in the optimized extract was 244 mg gallic acid equivalents/g dry weight, while individual polyphenols were analyzed using high-performance liquid chromatography coupled with a diode array detector (HPLC-DAD). Furthermore, antioxidant activity was assessed using ferric-reducing antioxidant power (FRAP) and DPPH radical scavenging assays, yielding values of 3235 and 1850 μmol ascorbic acid equivalents/g dry weight, respectively. Additionally, correlation analyses were conducted to evaluate the interactions between bioactive compounds and antioxidant capacity. Compared to other extraction techniques, PEF stands out as an eco-friendly, non-thermal standalone method, offering a sustainable approach for the rapid production of health-promoting extracts from <i>C. monogyna</i> leaves.https://www.mdpi.com/2223-7747/14/15/2262hawthornantioxidantspolyphenolsHPLC-DADresponse surface methodologyextraction optimization
spellingShingle Vasiliki Papazidou
Ioannis Makrygiannis
Martha Mantiniotou
Vassilis Athanasiadis
Eleni Bozinou
Stavros I. Lalas
Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
Plants
hawthorn
antioxidants
polyphenols
HPLC-DAD
response surface methodology
extraction optimization
title Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
title_full Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
title_fullStr Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
title_full_unstemmed Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
title_short Isolation of Bioactive Compounds and Antioxidant Activity Evaluation of <i>Crataegus monogyna</i> Leaves via Pulsed Electric Field-Assisted Extraction
title_sort isolation of bioactive compounds and antioxidant activity evaluation of i crataegus monogyna i leaves via pulsed electric field assisted extraction
topic hawthorn
antioxidants
polyphenols
HPLC-DAD
response surface methodology
extraction optimization
url https://www.mdpi.com/2223-7747/14/15/2262
work_keys_str_mv AT vasilikipapazidou isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction
AT ioannismakrygiannis isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction
AT marthamantiniotou isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction
AT vassilisathanasiadis isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction
AT elenibozinou isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction
AT stavrosilalas isolationofbioactivecompoundsandantioxidantactivityevaluationoficrataegusmonogynaileavesviapulsedelectricfieldassistedextraction