Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light

Abstract In this study, the inactivation of various bacterial strains in a solar illuminated photocatalysis reactor with a titania photocatalyst dispersed in a geopolymer coating is studied. The modular reactor design consists of connected catalyst-coated open water carrying chutes. The cleaning eff...

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Main Authors: Lukas Dufner, Philipp Hofmann, Daniel Dobslaw, Frank Kern
Format: Article
Language:English
Published: SpringerOpen 2025-04-01
Series:Applied Water Science
Subjects:
Online Access:https://doi.org/10.1007/s13201-025-02453-x
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author Lukas Dufner
Philipp Hofmann
Daniel Dobslaw
Frank Kern
author_facet Lukas Dufner
Philipp Hofmann
Daniel Dobslaw
Frank Kern
author_sort Lukas Dufner
collection DOAJ
description Abstract In this study, the inactivation of various bacterial strains in a solar illuminated photocatalysis reactor with a titania photocatalyst dispersed in a geopolymer coating is studied. The modular reactor design consists of connected catalyst-coated open water carrying chutes. The cleaning efficiency of the process against chemical and biological water contaminants was evaluated by means of test series with methylene blue as a reference for chemical contamination and by studying the inactivation of the strains Escherichia coli, Bacillus subtilis, Pseudomonas fluorescens and an undefined mixed culture from the effluent of the secondary clarifier of a wastewater treatment plant as biological contaminants. Test series with methylene blue showed reduction efficiencies of 17–63% for non-catalyst-coated reference reactors and 55–99% for catalyst-coated reactors within 120–300 min of exposure to natural sunlight. Disinfection test series showed reduction efficiencies of 0.0–2.8 log units (without catalyst) and 0.0–4.4 log units (with catalyst) for mentioned bacteria and the mixed culture within 40–180 min of light exposure. Hence, the catalyst-coated system consistently showed a significantly higher degradation efficiency than the non-coated reference. A comparison of methylene blue degradation under natural solar irradiation and artificial UVA irradiation conditions showed that this simple reactor concept is suitable for the combined elimination of trace substances and disinfection of water even at moderate flux rates of 1000 W/m2.
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spelling doaj-art-664f3b93c6dc44bd93d7894cd152ea4d2025-08-20T03:48:18ZengSpringerOpenApplied Water Science2190-54872190-54952025-04-0115511310.1007/s13201-025-02453-xDegradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar lightLukas Dufner0Philipp Hofmann1Daniel Dobslaw2Frank Kern3Institute for Manufacturing Technologies of Ceramic Components and Composites, University of StuttgartInstitute for Manufacturing Technologies of Ceramic Components and Composites, University of StuttgartInstitute of Spatial and Regional Planning, University of StuttgartInstitute for Manufacturing Technologies of Ceramic Components and Composites, University of StuttgartAbstract In this study, the inactivation of various bacterial strains in a solar illuminated photocatalysis reactor with a titania photocatalyst dispersed in a geopolymer coating is studied. The modular reactor design consists of connected catalyst-coated open water carrying chutes. The cleaning efficiency of the process against chemical and biological water contaminants was evaluated by means of test series with methylene blue as a reference for chemical contamination and by studying the inactivation of the strains Escherichia coli, Bacillus subtilis, Pseudomonas fluorescens and an undefined mixed culture from the effluent of the secondary clarifier of a wastewater treatment plant as biological contaminants. Test series with methylene blue showed reduction efficiencies of 17–63% for non-catalyst-coated reference reactors and 55–99% for catalyst-coated reactors within 120–300 min of exposure to natural sunlight. Disinfection test series showed reduction efficiencies of 0.0–2.8 log units (without catalyst) and 0.0–4.4 log units (with catalyst) for mentioned bacteria and the mixed culture within 40–180 min of light exposure. Hence, the catalyst-coated system consistently showed a significantly higher degradation efficiency than the non-coated reference. A comparison of methylene blue degradation under natural solar irradiation and artificial UVA irradiation conditions showed that this simple reactor concept is suitable for the combined elimination of trace substances and disinfection of water even at moderate flux rates of 1000 W/m2.https://doi.org/10.1007/s13201-025-02453-xPhotocatalysisDisinfectionTiO2Solar reactorBacteria degradation
spellingShingle Lukas Dufner
Philipp Hofmann
Daniel Dobslaw
Frank Kern
Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
Applied Water Science
Photocatalysis
Disinfection
TiO2
Solar reactor
Bacteria degradation
title Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
title_full Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
title_fullStr Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
title_full_unstemmed Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
title_short Degradation of bacteria for water purification in a TiO2-coated photocatalytic reactor illuminated by solar light
title_sort degradation of bacteria for water purification in a tio2 coated photocatalytic reactor illuminated by solar light
topic Photocatalysis
Disinfection
TiO2
Solar reactor
Bacteria degradation
url https://doi.org/10.1007/s13201-025-02453-x
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AT philipphofmann degradationofbacteriaforwaterpurificationinatio2coatedphotocatalyticreactorilluminatedbysolarlight
AT danieldobslaw degradationofbacteriaforwaterpurificationinatio2coatedphotocatalyticreactorilluminatedbysolarlight
AT frankkern degradationofbacteriaforwaterpurificationinatio2coatedphotocatalyticreactorilluminatedbysolarlight